Comparison of rhodamine B adsorption and desorption on the aged non-degradable and degradable microplastics: Effects of charge-assisted hydrogen bond and underline mechanism DOI Creative Commons
Kangkang Wang,

Yuli Kou,

Changyan Guo

et al.

Environmental Technology & Innovation, Journal Year: 2024, Volume and Issue: 35, P. 103739 - 103739

Published: July 3, 2024

The accumulation of microplastics (MPs) in the environment and their role as carriers for ionic organic pollutants are increasingly attracting attention. This study evaluated adsorption-desorption characteristics cationic pollutant on virgin UV-aged non-degradable polystyrene (PS) well degradable poly(butylene succinate) (PBS) adipate-co-terephthalate) (PBAT) MPs. results showed that aging treatment made surface MPs rougher more porous, causing adsorption to shift from monolayer multilayer adsorption. Aging increased oxygen-containing groups MPs, significantly enhancing H bond (HB) donor capabilities aged PBS PBAT, thereby improving by than 10 times. significant increase is mainly due combined effects strong HB (including ordinary (OHB) charge-assisted (CAHB)), electrostatic interactions, π-π interactions. Notably, stronger enabled PBAT achieve efficient stable rhodamine B over a wide pH range, with desorption hysteresis (HI > 1.80). indicates can act long-distance transport. total simulated animal gastrointestinal fluids confirmed greater environmental hazards work first demonstrate unique donors, primarily adsorb through (CAHB OHB), which helps assess fate biodegradable aquatic systems.

Language: Английский

From organic fertilizer to the soils: What happens to the microplastics? A critical review DOI
Shengwei Zhang, Yanxia Li, Linshu Jiang

et al.

The Science of The Total Environment, Journal Year: 2024, Volume and Issue: 919, P. 170217 - 170217

Published: Feb. 1, 2024

Language: Английский

Citations

26

Research progress on the role of biofilm in heavy metals adsorption-desorption characteristics of microplastics: A review DOI

Haixia Pan,

Xin Zhao,

Xiuyan Zhou

et al.

Environmental Pollution, Journal Year: 2023, Volume and Issue: 336, P. 122448 - 122448

Published: Aug. 26, 2023

Language: Английский

Citations

29

Biodegradable microplastics interaction with pollutants and their potential toxicity for aquatic biota: a review DOI
Wajid Ali, Haksoo Jeong, Jae‐Seong Lee

et al.

Environmental Chemistry Letters, Journal Year: 2024, Volume and Issue: 22(3), P. 1185 - 1220

Published: Feb. 27, 2024

Language: Английский

Citations

12

Accelerated aging behavior of degradable and non-degradable microplastics via advanced oxidation and their adsorption characteristics towards tetracycline DOI Creative Commons
Xinfeng Cheng, Shihao Wang, Xin Zhang

et al.

Ecotoxicology and Environmental Safety, Journal Year: 2024, Volume and Issue: 284, P. 116864 - 116864

Published: Aug. 12, 2024

The increasing global utilization of biodegradable plastics due to stringent regulations on traditional has caused a significant rise in microplastic (MPs) pollution aquatic ecosystems from products. However, the environmental behavior MPs remains inadequately elucidated. This study explored aging processes polylactic acid (PLA) and polystyrene (PS) under heat-activated potassium persulfate (K

Language: Английский

Citations

11

Embedding an esterase mimic inside polyesters to realize rapid and complete degradation without compromising their utility DOI Creative Commons

Yanfen Wu,

Jing Tian,

Minmin Sun

et al.

Green Chemistry, Journal Year: 2024, Volume and Issue: 26(5), P. 2851 - 2857

Published: Jan. 1, 2024

This work presents an innovative method to manage post-consumer biodegradable plastics by embedding a molecular mimic of esterase into poly(butylene terephthalate/adipate), which holds the potential elevate composting efficiency and capacity.

Language: Английский

Citations

10

Effects of biodegradable microplastics on arsenic migration and transformation in paddy soils: a comparative analysis with conventional microplastics DOI

Qiuying An,

Zhuo Zhen,

Nijing Zhong

et al.

Journal of Hazardous Materials, Journal Year: 2024, Volume and Issue: 469, P. 134053 - 134053

Published: March 15, 2024

Language: Английский

Citations

10

Exploring Environmental Behaviors and Health Impacts of Biodegradable Microplastics DOI
Yuhao Yan, Jun Cheng, Jie Gao

et al.

Environmental Science & Technology, Journal Year: 2025, Volume and Issue: unknown

Published: March 21, 2025

Biodegradable plastics (BPs) are promoted as eco-friendly alternatives to conventional plastics. However, compared microplastics (MPs), they degrade rapidly into biodegradable (BMPs), which may lead a more significant accumulation of BMPs in the environment. This review systematically compares and MPs, summarizes current knowledge on their environmental behaviors impacts ecosystems human health, offers recommendations for future research. detected water, sediments, indoor dust, food, marine organisms, samples. Compared prone transformations, such photodegradation biodegradation, results shorter migration distance across different matrices. Like can adsorb pollutants transport them enhancing toxicity health risks through Trojan horse effect. Studies indicate that negatively impact terrestrial aquatic than MPs by disrupting nutrient cycling inhibiting plant animal growth. In vivo vitro research also shows BMP degradation products increase bioavailability, exacerbating neurotoxicity overall toxicity. findings BMPs' effects remain inconsistent. Further evaluation trade-offs between biodegradability is needed address these uncertainties.

Language: Английский

Citations

1

Comprehensive understanding of the aging and biodegradation of polystyrene-based plastics DOI

Dazhuang Dong,

Zhi Guo,

Xue Yang

et al.

Environmental Pollution, Journal Year: 2023, Volume and Issue: 342, P. 123034 - 123034

Published: Nov. 26, 2023

Language: Английский

Citations

22

Effects of humic acids on the adsorption of Pb(II) ions onto biofilm-developed microplastics in aqueous ecosystems DOI
Qiongjie Wang, Yangyang Zhang, Huijuan Chen

et al.

The Science of The Total Environment, Journal Year: 2023, Volume and Issue: 882, P. 163466 - 163466

Published: April 23, 2023

Language: Английский

Citations

18

Exploring the hidden environmental pollution of microplastics derived from bioplastics: A review DOI
I. D. U. H. Piyathilake, Chuxia Lin, Nanthi Bolan

et al.

Chemosphere, Journal Year: 2024, Volume and Issue: 355, P. 141773 - 141773

Published: March 26, 2024

Language: Английский

Citations

8