Enhanced Degradation of Levofloxacin through Visible-Light-Driven Peroxymonosulfate Activation over CuInS2/g-C3N4 Heterojunctions DOI Creative Commons
Xin Zhong, Meihuan Ji, Wenxin Wu

et al.

Nanomaterials, Journal Year: 2023, Volume and Issue: 14(1), P. 74 - 74

Published: Dec. 26, 2023

In this work, the heterojunctions of CuInS2 embedded in g-C3N4 materials (xCuInS2/g-C3N4, abbreviated as xCIS/GCN) was successfully prepared for peroxymonosulfate (PMS) activation under visible light. The catalysts are characterized by different techniques, such XRD, FTIR, SEM, TEM, and UV-vis. unique heterojunction composites can suppress recombination photogenerated pairs. catalytic results showed that 3CIS/GCN exhibited excellent levofloxacin (LVF) degradation efficiency, while more than 98.9% LVF removed 60 min over a wide pH range. SO4•−, O2•−, OH•, 1O2 were verified main reactive species via quenching experiments electron paramagnetic resonance technology (EPR). synergetic effect xCIS/GCN, PMS, light irradiation discussed. possible pathway proposed through byproducts analysis (LC-MS). Moreover, 3CIS/GCN/vis-PMS system has very low metal leaching. Owing to xCIS/GCN having good properties PMS activation, it potential applications or other hazardous pollutants degradation.

Language: Английский

Pilot-scale sulfate radical-based advanced oxidation for wastewater reuse: simultaneous disinfection, removal of contaminants of emerging concern, and antibiotic resistance genes DOI
Sonia Guerra-Rodríguez, María Jesús Abeledo-Lameiro, María Inmaculada Polo-López

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 477, P. 146916 - 146916

Published: Oct. 24, 2023

Language: Английский

Citations

24

Catalytic-separation technology for highly efficient removal of emerging pollutants, desalination, and antimicrobials: A new strategy for complex wastewater treatment DOI

Ming Yi,

Qi Xia,

Jiale Tan

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 493, P. 152568 - 152568

Published: May 26, 2024

Language: Английский

Citations

9

The Convergence of Antibiotic Contamination, Resistance, and Climate Dynamics in Freshwater Ecosystems DOI Open Access
Marcelo Pedrosa Gomes

Water, Journal Year: 2024, Volume and Issue: 16(18), P. 2606 - 2606

Published: Sept. 14, 2024

The convergence of antibiotic contamination, antimicrobial resistance (AMR), and climate dynamics poses a critical environmental public health challenge. Freshwater ecosystems are increasingly threatened by the persistent presence antibiotics, which, coupled with rising global temperatures, accelerate development spread AMR. This review examines sources, pathways, mechanisms through which antibiotics enter freshwater systems how change exacerbates these processes. discusses this convergence’s ecological human impacts, highlighting implications for biodiversity health. It also explored current monitoring mitigation strategies, including advanced oxidation processes, natural-based solutions, policy interventions. Finally, identifies research gaps proposes future directions managing intertwined threats resistance, change. emphasizes need integrated, multidisciplinary approaches to protect resources in an volatile environment.

Language: Английский

Citations

9

Bibliometric analysis of Advanced Oxidation Processes studies with a focus on Life Cycle Assessment and Costs DOI
Isadora Luiza Clímaco Cunha, Pedro Gerber Machado, Celma de Oliveira Ribeiro

et al.

Environmental Science and Pollution Research, Journal Year: 2024, Volume and Issue: 31(15), P. 22319 - 22338

Published: March 2, 2024

Language: Английский

Citations

5

CO2(OH)2CO3 and Fe doped Co2(OH)2CO3 prepared as efficient and stable catalysts for activation of PMS: Two systems comparison and key role of high-valent metal-oxo species in mechanism revealing DOI
Peng Cheng,

Qiongfang Wang,

Xin Zhang

et al.

Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 129980 - 129980

Published: Oct. 1, 2024

Language: Английский

Citations

4

Construction of CoFe2O4/TiO2@C S-scheme heterojunction and removal of phenol by activated peroxymonosulfate DOI
Zichu Hu, Wanqi Zhang,

Zhechen Liu

et al.

Journal of Alloys and Compounds, Journal Year: 2025, Volume and Issue: 1022, P. 179992 - 179992

Published: March 31, 2025

Language: Английский

Citations

0

Developing a β-cyclodextrin modified nanoconfined channels catalyst for efficient activation of peroxymonosulfate: Enhancing non-radical pathways and electron transfer DOI
Jun Cai, Jinquan Wan, Yan Wang

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2025, Volume and Issue: unknown, P. 125401 - 125401

Published: April 1, 2025

Language: Английский

Citations

0

Asymmetric Pulsed Janus Filter Cathode Enables Effective and Sustainable Electro-Fenton: Overlooked Interfacial Electronic Interaction and Competitive Effect DOI
Gengbo Ren, Jie Zhang,

Tiantong Rao

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2025, Volume and Issue: unknown, P. 125349 - 125349

Published: April 1, 2025

Language: Английский

Citations

0

Life cycle assessment to evaluate the integral water cycle in industrial supply: A real case study DOI Creative Commons
Jorge Rodríguez‐Chueca,

Asier Criado Bañuelos,

Javier Pérez

et al.

The Science of The Total Environment, Journal Year: 2024, Volume and Issue: 931, P. 172891 - 172891

Published: May 1, 2024

Wastewater recycling technologies are developed in areas where the necessity of water resources cannot be satisfied by natural sources. Nevertheless, nowadays trends and European Union Plans show an increasing interest on using these to reduce environmental impacts. This manuscript aims address question real results differences between each specific case Life Cycle Assessment (LCA) methodology. A study is analyzed answer this question: integral cycle a northern Spain, comparing traditional supply system (system I), alternative wastewater regeneration plant II). System II presents higher impact for all categories (between 1.2 37 times higher), except land use, it reduced 53 %. These larger produced due energy chemical product consumption. Energy consumption main factor causing highest most both studied systems, including one associated resource It accounts at least 50 % total 7 16 evaluated categories. In terms climate change, not particularly significant I, but II, represents around that impact. determined consumption, waste discharge treatment relevant factors. sense, paper highlights importance analysing specifically underscores usefulness LCA methodology as tool improve decision-making management, with emerging crucial focal point.

Language: Английский

Citations

2

Environmental life cycle assessment of UV-C LEDs vs. mercury lamps and oxidant selection for diclofenac degradation DOI Creative Commons
Angela Raffaella Pia Pizzichetti, Mario Martín-Gamboa, Cristina Pablos

et al.

Sustainable materials and technologies, Journal Year: 2024, Volume and Issue: 41, P. e01002 - e01002

Published: June 3, 2024

This study is the first environmental comparison between a UV-C LED lamp (emitting at 265 nm) and mercury lamps employed in lab-scale photoreactor for water treatment purification purposes, using removal of diclofenac as case study. Ex-ante life cycle assessment (LCA) methodology was used robust method to identify hotspots recommendations early stage LEDs technology. The functional unit defined "the 1 L polluted with 20 mg L-1 achieve 90% contaminant", while system boundaries include production operation photoreactors, following cradle-to-gate approach. Several scenarios were explored, overall, shows promising performance, less or similar potential impacts than 16 categories selected from Environmental Footprint (EF) method. In particular, it reveals impact "human toxicity non-cancer" "resource use minerals metals" presents electricity main source impact. Given higher efficacy UV-driven advanced oxidation processes compared UV irradiation alone, since no studies have previously been conducted on sustainability free chlorine (FC) an oxidant treatment, UV-C, UV-C/H2O2, UV-C/FC employing nm also assessed. UV-C/H2O2 more sustainable same time, but both led overall reduction 35% 30%, respectively. To increase sustainability, cleaner energy sources such photovoltaic wind resulted 80% 93% "climate change" category. Overall, this demonstrates that oxidants beneficial encourages scale-up system.

Language: Английский

Citations

2