Stochastic Environmental Research and Risk Assessment, Journal Year: 2024, Volume and Issue: 38(7), P. 2693 - 2709
Published: April 2, 2024
Language: Английский
Stochastic Environmental Research and Risk Assessment, Journal Year: 2024, Volume and Issue: 38(7), P. 2693 - 2709
Published: April 2, 2024
Language: Английский
Atmospheric Environment, Journal Year: 2024, Volume and Issue: 323, P. 120390 - 120390
Published: Feb. 3, 2024
The Yangtze River Economic Belt (YREB) in China is one of the most populated regions world with fast growth economy and pollutant emissions from human activity, which has contributed to severe air-quality issues detrimental impact on health. China's measures control spread COVID-19 appear have resulted reductions energy consumption air emissions. However, there a scarcity studies that examine how natural meteorological socioeconomic factors collectively influence temporal spatial variations pollution YREB before during lockdown. In this study, we analyze spatiotemporal evolution pollutants period 2015–2022, estimate their dependence, clustering characteristics, spillover effects, response multiple variables. Significant decreasing trends were observed for major except O3. Although 24.44% reduction PM2.5 exposure outbreak 7.60% due clean measures, O3 warm seasons (April–September) increased by 13.74% 9.29% outbreak. At level, highest concentrations six recorded urban agglomerations lower or middle reaches River. A significant autocorrelation annual average was detected Meteorological conditions activities potentially had impacts concentrations. Prior implementation both dominated quality changes YREB. following epidemic, far outweighed index. finding study profound implications formulating emission policies customized China.
Language: Английский
Citations
3Atmosphere, Journal Year: 2022, Volume and Issue: 13(11), P. 1834 - 1834
Published: Nov. 4, 2022
Nowadays, many cities in China are suffering from both fine particulate matter (PM2.5, with an aerodynamic diameter smaller than 2.5 µm) and ozone (O3) pollution. Secondary organic aerosol (SOA) is important component of PM2.5 closely related to the oxidation processes. To investigate characteristics formation pathways SOA during different types haze pollution episodes, carbonaceous components volatile compounds (VOCs) were monitored continuously Chengdu April 2019, when experienced not only (SPP) but also a complex O3 (CoP). In CoP episode, concentrations increased by 51.2% as compared SPP, positively correlated mass concentrations. These suggest that drove increase levels event some extent. The preliminary VOC source analysis based on feature ratio showed vehicle emission fuel volatilization sources main VOCs at this urban site. addition, coal emissions biomass burning contributors. High-carbon alkanes aromatic hydrocarbons significantly contributed formation. results provide understanding episodes Chengdu, which can help us further understand air typical region.
Language: Английский
Citations
13Atmosphere, Journal Year: 2023, Volume and Issue: 14(2), P. 292 - 292
Published: Feb. 1, 2023
In recent years, ozone and PM2.5 pollution has often occured in the Fenwei Plain due to heavy emission favorable geographical conditions. this study, we used weather research forecasting/chemistry (WRF-Chem) model reproduce complex air of (FWP) from 20 May 29 2015. By comparing simulation results with observed data, found that although some cities there was a bias between simulated values captured trend pollutants generally. Moreover, according assessment parameters, validated deviations are acceptable. However, these WRF-Chem performed better on rather than PM2.5. Based validation, further analyzed pollutant distribution during contaminated period. Generally speaking, polluted area is mainly located Shanxi province Henan province. time period, occurred 27 28 May. addition, different formation conditions pollution, characteristics two were also be different. Ozone north FWP prevailing wind chemistry production. As for PM2.5, at night FWP. Furthermore, high areas closed sources FWP, showing correlation primary emissions.
Language: Английский
Citations
7Atmosphere, Journal Year: 2023, Volume and Issue: 14(4), P. 609 - 609
Published: March 23, 2023
Ozone (O3) is becoming an increasingly concerning air quality problem in China, and previous O3 control strategies focused primarily on reducing anthropogenic volatile organic compounds (AVOCs), while neglecting the role of biogenic VOCs (BVOCs) formation. In this study, a field campaign was conducted at suburban site Pearl River Delta region China with high BVOC emissions from 29 August to 3 September 2020. An empirical kinetic modelling approach (EKMA) showed that VOC-limited dominant feature for formation site. The relative incremental reactivity (RIR) values calculated by box model (AtChem2-MCM) revealed isoprene, formaldehyde, methylglyoxal acetaldehyde had highest RIRs. Simulation results also isoprene played substantial secondary carbonyls, especially contributing 32–92% formaldehyde production rate. Box simulations further during pollution period emissions, only near zero AVOC could prevent if levels nitrogen oxides (NOx) remained unchanged. suggest presence can greatly impact efforts AVOCs, particularly regions relatively NOx (up 51 ppbv study). long term, it may be essential choose low BVOC-emitting tree species urban planning address issue, as are projected become more significant source reactive enhanced AVOCs.
Language: Английский
Citations
7Stochastic Environmental Research and Risk Assessment, Journal Year: 2024, Volume and Issue: 38(7), P. 2693 - 2709
Published: April 2, 2024
Language: Английский
Citations
2