Journal of Materials Science Materials in Electronics, Journal Year: 2025, Volume and Issue: 36(5)
Published: Feb. 1, 2025
Language: Английский
Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: 94, P. 302 - 331
Published: March 8, 2024
Language: Английский
Citations
61
Advanced Science, Journal Year: 2024, Volume and Issue: 11(25)
Published: April 22, 2024
Abstract High‐entropy oxides (HEOs) have garnered significant attention within the realm of rechargeable batteries owing to their distinctive advantages, which encompass diverse structural attributes, customizable compositions, entropy‐driven stabilization effects, and remarkable superionic conductivity. Despite brilliance HEOs in energy conversion storage applications, there is still lacking a comprehensive review for both entry‐level experienced researchers, succinctly encapsulates present status challenges inherent HEOs, spanning features, intrinsic properties, prevalent synthetic methodologies, diversified applications batteries. Within this review, endeavor distill characteristics, ionic conductivity, entropy explore practical (lithium‐ion, sodium‐ion, lithium‐sulfur batteries), including anode cathode materials, electrolytes, electrocatalysts. The seeks furnish an overview evolving landscape HEOs‐based cell component shedding light on progress made hurdles encountered, as well serving guidance compositions design optimization strategy enhance reversible stability, electrical electrochemical performance conversion.
Language: Английский
Citations
26
Rare Metals, Journal Year: 2024, Volume and Issue: 43(10), P. 4639 - 4776
Published: Aug. 28, 2024
Language: Английский
Citations
21
Materials Today Catalysis, Journal Year: 2024, Volume and Issue: 4, P. 100039 - 100039
Published: Jan. 17, 2024
Electrocatalysis plays a crucial role in the conversion and storage of renewable energy, offering significant potential for addressing energy crisis environmental concerns. High-entropy oxides (HEOs), class emerging functional materials, have gained increasing attention electrocatalysis due to their stable crystal structure, exceptional geometric compatibility, unique electronic balance factors, abundant active sites. In this comprehensive review, we present recent advancements utilizing HEOs as catalysts various energy-based electrocatalytic reactions. We begin with an overview that includes definitions, fundamental properties, theoretical investigations. Subsequently, describe different synthetic methods while highlighting two newly-developed techniques. Furthermore, extensively discuss developments HEO-based electrocatalysts diverse structures such rock-salt-type, rutile-type, spinel-type, perovskite-type, other specially-structured HEOs. Special emphasis is placed on designed strategies aimed at enhancing performance exploring correlations between structure/ composition performance. Finally, provide concluding remarks along perspectives future opportunities exciting field.
Language: Английский
Citations
19
Advanced Fiber Materials, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 2, 2025
Language: Английский
Citations
2
Journal of Alloys and Compounds, Journal Year: 2023, Volume and Issue: 969, P. 172232 - 172232
Published: Sept. 20, 2023
Language: Английский
Citations
30
Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: 98, P. 441 - 471
Published: July 4, 2024
Language: Английский
Citations
14
Energy storage materials, Journal Year: 2024, Volume and Issue: 72, P. 103750 - 103750
Published: Aug. 26, 2024
Language: Английский
Citations
12
Journal of Advanced Ceramics, Journal Year: 2024, Volume and Issue: 13(8), P. 1093 - 1118
Published: May 24, 2024
The coordinated development of new energy vehicles and the storage industry has become inevitable to reduce carbon emissions. cathode material is key that determines density cost a power battery, while currently developed applied can not meet requirements high specific capacity, low cost, safety good stability. High-entropy type single-phase composed multiple principal elements in equimolar or near-equimolar ratios. interaction between play an important role improving comprehensive properties material, which expected solve limitations battery materials practical applications. Based on this, this review provides overview current status modification strategies batteries (lithium-ion sodium-ion battery), proposes high-entropy design strategy, analyzes structure-activity relationship effect performance. Finally, future research topics are proposed, including computational guide design, synthesis methods, electrochemistry high-throughput databases. This aims provide guidance for next-generation batteries.
Language: Английский
Citations
11
Materials Futures, Journal Year: 2024, Volume and Issue: 3(4), P. 042103 - 042103
Published: Oct. 8, 2024
Abstract High-entropy oxides (HEOs), with their multi-principal-element compositional diversity, have emerged as promising candidates in the realm of energy materials. This review encapsulates progress harnessing HEOs for conversion and storage applications, encompassing solar cells, electrocatalysis, photocatalysis, lithium-ion batteries, solid oxide fuel cells. The critical role theoretical calculations simulations is underscored, highlighting contribution to elucidating material stability, deciphering structure-activity relationships, enabling performance optimization. These computational tools been instrumental multi-scale modeling, high-throughput screening, integrating artificial intelligence design. Despite promise, challenges such fabrication complexity, cost, hurdles impede broad application HEOs. To address these, this delineates future research perspectives. include innovation cost-effective synthesis strategies, employment situ characterization micro-chemical insights, exploration unique physical phenomena refine performance, enhancement models precise structure-performance predictions. calls interdisciplinary synergy, fostering a collaborative approach between materials science, chemistry, physics, related disciplines. Collectively, these efforts are poised propel towards commercial viability new technologies, heralding innovative solutions pressing environmental challenges.
Language: Английский
Citations
10