Boosting Photocatalytic Performance of Polymeric Carbon Nitride by Adjusting its D-A Structure Via Group Modification Strategy DOI
Bei Wang,

Mingxiu Huang,

Meng Jiang

et al.

Published: Jan. 1, 2023

A new kind of group-modified polymeric carbon nitride (PCN) photocatalyst was synthetized with urea and 4-Nitro-o-phenylenediamine (NPD) by one-pot method applied to degrade bisphenol (BPA) in aqueous solution. The light response range had been extended a lot due conjugation electron withdrawing properties nitrobenzene. introduction nitrobenzene changed nanostructures PCN led an increased specific surface area. XPS EPR results proved that more sp2 N vacancies were introduced grafting Theoretical simulation demonstrated this group modification on beneficial for enhanced Donor-Acceptor (D-A) structures thus promotional charge separation. photocatalytic performance BPA degradation promoted 10 times than unmodified PCN. To verify the universality strategies, we prepared other two kinds photocatalysts via electron-withdrawing strategy their all improved obviously.

Language: Английский

Study on the performance and mechanism of photocatalytic reduction of Cr(VI) through Boron-doped g-C3N4 under visible Light DOI
Yuhang Gao,

Lijun Nie,

Na Zheng

et al.

Optical Materials, Journal Year: 2025, Volume and Issue: unknown, P. 116889 - 116889

Published: March 1, 2025

Language: Английский

Citations

0
Strategic nitrogen defect engineering for optimizing the photocatalytic performance of polymerized carbon nitride: Identification, synthesis, and mechanism DOI

Zhangkai Chen,

Meifang Li, Xinjiang Hu

et al.

Journal of environmental chemical engineering, Journal Year: 2023, Volume and Issue: 11(5), P. 111121 - 111121

Published: Sept. 26, 2023

Language: Английский

Citations

5
Synthesis of lamellar O-doped ZnIn2S4 on layered g-C3N4 for boosted charge transfer and photocatalytic performances DOI

Yan Xu,

Mengxia Ma,

Yanli Mao

et al.

New Journal of Chemistry, Journal Year: 2023, Volume and Issue: 47(34), P. 16235 - 16244

Published: Jan. 1, 2023

The formation schematic is representative of the CN/O-doped ZIS composite. First, pure g-C 3 N 4 powder was prepared by directly calcining melamine in a muffle furnace. Then composites were via hydrothermal method.

Language: Английский

Citations

4
Preparation of organic compounds/g-C3N4 composites and their applications in photocatalysis DOI

Jun Wu,

Xingchen Ding, Xiashi Zhu

et al.

Materials Chemistry Frontiers, Journal Year: 2024, Volume and Issue: 8(23), P. 3859 - 3876

Published: Jan. 1, 2024

This review mainly summarises the progress in preparation methods of organic compound/g-C 3 N 4 . Various materials such as different types composites and their related energy environmental applications are discussed.

Language: Английский

Citations

0
The n–π* electronic transition induced by nitrogen vacancies enhances photocatalytic hydrogen production in carbon nitride DOI

Zhili Xu,

Jing Li,

Deyi Zhan

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 501, P. 157670 - 157670

Published: Nov. 14, 2024

Language: Английский

Citations

0
Ascorbic Acid Enhanced Cufe2o4-Catalyzed Heterogeneous Photo-Fenton-Like Degradation of Phenol DOI
Junrui Feng, Ying Zhang

Published: Jan. 1, 2023

CuFe2O4 particles were synthesized using the sol-gel self-combustion method and characterized for their compositional surface morphology crystal structure. In comparison to photo-Fenton system without ascorbic acid (AA), presence of AA resulted in significantly enhanced catalytic degradation phenol CuFe2O4. The highest efficiency was achieved at an concentration 1 mM/L, resulting up 99.4% elimination just 40 min. reaction rate found be 31.7 times higher than that AA. mechanism enhancement further investigated. Two key factors contribute enhancing introduction system. First, promoted Cu/Fe redox cycle on catalyst surface, leading a more efficient generation reactive species which are responsible degradation. Second, accelerated leaching metal ions from assisting homogenous Fenton effect. bimetallic offers new perspectives effective design crucial insights reductant-enhanced activation.

Language: Английский

Citations

0
Boosting Photocatalytic Performance of Polymeric Carbon Nitride by Adjusting its D-A Structure Via Group Modification Strategy DOI
Bei Wang,

Mingxiu Huang,

Meng Jiang

et al.

Published: Jan. 1, 2023

A new kind of group-modified polymeric carbon nitride (PCN) photocatalyst was synthetized with urea and 4-Nitro-o-phenylenediamine (NPD) by one-pot method applied to degrade bisphenol (BPA) in aqueous solution. The light response range had been extended a lot due conjugation electron withdrawing properties nitrobenzene. introduction nitrobenzene changed nanostructures PCN led an increased specific surface area. XPS EPR results proved that more sp2 N vacancies were introduced grafting Theoretical simulation demonstrated this group modification on beneficial for enhanced Donor-Acceptor (D-A) structures thus promotional charge separation. photocatalytic performance BPA degradation promoted 10 times than unmodified PCN. To verify the universality strategies, we prepared other two kinds photocatalysts via electron-withdrawing strategy their all improved obviously.

Language: Английский

Citations

0