Facilitating CO2–CH4 Reforming Into Syngas and Useful Chemicals by Water‐Cooled Dielectric Barrier Discharge Plasma: Effect of Discharge Power, Gas Mixing, and Mechanism Insight DOI
Tian Chang, Xiangpeng Chang,

Abdelkader Labidi

et al.

Plasma Processes and Polymers, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 3, 2024

ABSTRACT CO 2 reforming of CH 4 to syngas (H and CO) has emerged as one the attractive options for mitigating carbon emissions. Here, a water‐cooled dielectric barrier discharge plasma reactor been constructed –CH produce value‐added chemicals. The effects main parameters (i.e., power, /CO molar ratio, gas flow rate) on were investigated. highest conversion rate was found be 40.57% 27.15%, respectively, with H selectivity 56.07% 43.71%, respectively. total energy efficiency achieved 0.28 mmol/kJ. C 6 hydrocarbon product. Lastly, mechanism proposed in terms active species products.

Language: Английский

Plasma Catalysis for Hydrogen Production: A Bright Future for Decarbonization DOI Creative Commons
Ni Wang, Hope O. Otor,

Gerardo Rivera-Castro

et al.

ACS Catalysis, Journal Year: 2024, Volume and Issue: 14(9), P. 6749 - 6798

Published: April 16, 2024

Thermal approaches have played a dominant role in driving chemical reactions within the chemicals and fuels industries, benefiting from ongoing enhancements efficiency via heat integration, catalyst development, process intensification. Nevertheless, these traditional thermal remain heavily reliant on fossil fuels, there exists an urgent demand for implementation of renewable energy technologies to synthesize commodity chemicals, specialty chemicals. Nonthermal plasmas gained considerable attention recent years as promising solution, prospects combining with suitable catalysts become even more appealing. Moreover, evolution nonthermal plasma catalysis generation clean hydrogen could be transformative reducing greenhouse gas emissions. This comprehensive review highlights influential contributions production, discusses advancements, provides future researchers aiming advance production hydrogen.

Language: Английский

Citations

21

Plasma-based dry reforming of CH4: Plasma effects vs. thermal conversion DOI
Joachim Slaets, Björn Loenders, Annemie Bogaerts

et al.

Fuel, Journal Year: 2023, Volume and Issue: 360, P. 130650 - 130650

Published: Dec. 15, 2023

Language: Английский

Citations

11

Plasma-based conversion of martian atmosphere into life-sustaining chemicals: The benefits of utilizing martian ambient pressure DOI Creative Commons
Seán Kelly,

Elizabeth Mercer,

Yury Gorbanev

et al.

Journal of CO2 Utilization, Journal Year: 2024, Volume and Issue: 80, P. 102668 - 102668

Published: Jan. 9, 2024

We explored the potential of plasma-based In-Situ Resource Utilization (ISRU) for Mars through conversion Martian atmosphere (∼96% CO2, 2% N2, and Ar) into life-sustaining chemicals. As surface pressure is about 1% Earth's pressure, it an ideal environment gas using microwave reactors. At 1000 W 10 Ln/min (normal liters per minute), we produced ∼76 g/h O2 ∼3 NOx a 2.45 GHz waveguided reactor at 25 mbar, which ∼3.5 times ambient pressure. The energy cost required to produce was ∼0.013 kWh/g, very promising compared recently concluded MOXIE experiments on surface. This marks crucial step towards realizing extension human exploration.

Language: Английский

Citations

4

Microwave plasma-assisted hydrogen production via conversion of CO2–CH4 mixture DOI
Dariusz Czylkowski, Bartosz Hrycak, Robert Miotk

et al.

International Journal of Hydrogen Energy, Journal Year: 2024, Volume and Issue: 78, P. 421 - 432

Published: June 27, 2024

Language: Английский

Citations

4

Electrifying the dry reforming of methane. Shall we target the chemistry or the heat supply? DOI Creative Commons
Tomasz Kotkowski, Robert Cherbański, Andrzej Stankiewicz

et al.

Chemical Engineering and Processing - Process Intensification, Journal Year: 2024, Volume and Issue: 202, P. 109875 - 109875

Published: June 29, 2024

The principles of sustainable development require decarbonization the chemical sector. An example implementation this strategy is electrification Dry Reforming Methane (DRM). In work, five electricity-based DRM technologies targeting chemistry (photocatalysis and plasma) heat supply (microwaves, Joule heating induction heating) are analyzed compared. following issues discussed for all technologies: feasibility large-scale reactor design operation, reactants conversion syngas production rates, energy consumption/efficiency, coking, process economy safety. On short term, appears to be most promising reviewed, due its relative simplicity, high methane conversions electricity-to-heat efficiency.

Language: Английский

Citations

4

Combined excitation of microwave thermal field and electric field on doped ferroelectric catalyst of MgFe-LiNbO3 for lignin depolymerization DOI
Wenkang Wang,

Junhao Cui,

Zhonglei Zhang

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 163256 - 163256

Published: April 1, 2025

Language: Английский

Citations

0

Synergistic Catalytic Effects of Nickel-Based Catalysts on Calcium Aluminate Supports in Methane Dry and Combined Reforming Processes DOI
Ehsan Akbari, Mehran Rezaei, Zahra Montazeri

et al.

Process Safety and Environmental Protection, Journal Year: 2025, Volume and Issue: unknown, P. 106903 - 106903

Published: Feb. 1, 2025

Language: Английский

Citations

0

Research Progress on Plasma-Assisted Catalytic Dry Reforming of Methane DOI Creative Commons
Τao Zhu, Chen Li, Xueli Zhang

et al.

Atmosphere, Journal Year: 2025, Volume and Issue: 16(4), P. 376 - 376

Published: March 26, 2025

With the significant consumption of traditional fossil fuels, emissions greenhouse gases such as methane (CH4) and carbon dioxide (CO2) continue to rise, requiring effective treatment methods. The dry reforming (DRM) offers a promising pathway for gas mitigation by converting CH4 CO2 into high-value syngas. However, thermal catalysis is prone catalyst deactivation due high-temperature sintering deposition caused side reactions. introduction non-thermal plasma (NTP) provides mild reaction environment, effectively mitigating deposition, extending lifespan, reducing energy consumption, significantly enhancing performance efficiency. This paper reviews recent progress in plasma-assisted DRM, focusing on different discharge types materials. synergistic effects between catalysts challenges prospects DRM technology are discussed.

Language: Английский

Citations

0

Progress and Future of CO2 Conversion Based on Plasma Catalysis DOI Creative Commons

Lefei Cao,

Fei Qi, Nan Zhang

et al.

DeCarbon, Journal Year: 2025, Volume and Issue: unknown, P. 100109 - 100109

Published: April 1, 2025

Language: Английский

Citations

0

Development and Validation of a Detailed Mechanism Generated by the Reaction Mechanism Generator for High-Temperature Ethane Dry Reforming DOI

Woorin Kang,

Moon Soo Bak

Journal of the Korean Society of Combustion, Journal Year: 2025, Volume and Issue: 30(1), P. 10 - 17

Published: March 31, 2025

Language: Английский

Citations

0