Surfaces and Interfaces, Journal Year: 2023, Volume and Issue: 39, P. 102937 - 102937
Published: May 7, 2023
Language: Английский
Surfaces and Interfaces, Journal Year: 2023, Volume and Issue: 39, P. 102937 - 102937
Published: May 7, 2023
Language: Английский
Applied Catalysis B Environment and Energy, Journal Year: 2023, Volume and Issue: 333, P. 122780 - 122780
Published: April 25, 2023
Language: Английский
Citations
153Separation and Purification Technology, Journal Year: 2023, Volume and Issue: 315, P. 123708 - 123708
Published: March 30, 2023
Language: Английский
Citations
121International Journal of Hydrogen Energy, Journal Year: 2023, Volume and Issue: 52, P. 804 - 818
Published: Sept. 22, 2023
Language: Английский
Citations
112Journal of Material Science and Technology, Journal Year: 2023, Volume and Issue: 160, P. 214 - 239
Published: April 23, 2023
Language: Английский
Citations
103Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 467, P. 143450 - 143450
Published: May 11, 2023
Language: Английский
Citations
69Journal of environmental chemical engineering, Journal Year: 2023, Volume and Issue: 11(5), P. 110393 - 110393
Published: June 19, 2023
Language: Английский
Citations
59Separation and Purification Technology, Journal Year: 2023, Volume and Issue: 312, P. 123398 - 123398
Published: Feb. 11, 2023
Language: Английский
Citations
58Materials Today Chemistry, Journal Year: 2023, Volume and Issue: 30, P. 101603 - 101603
Published: June 1, 2023
Language: Английский
Citations
46Chemosphere, Journal Year: 2023, Volume and Issue: 337, P. 139397 - 139397
Published: July 3, 2023
Language: Английский
Citations
43ACS Catalysis, Journal Year: 2024, Volume and Issue: 14(3), P. 1951 - 1961
Published: Jan. 22, 2024
Photocatalytic conversion of CO2 into valuable hydrocarbon fuels holds great promise in addressing emerging energy shortages and environmental crises while fulfilling pressing societal national development demands. Nonetheless, its efficiency is hindered by restricted chemisorption, rapid electron–hole recombination, weak redox capability. Drawing inspiration from the distinctive characteristics Schiff-based covalent organic frameworks (COFs), including substantial specific surface area, unique pore structure, an abundance weakly alkaline nitrogen elements, we employ TPA-COF to enhance chemisorption activation acidic molecules, as validated CO2-temperature-programmed desorption analysis. Furthermore, anchoring CsPbBr3 quantum dots (QDs) onto COF facilitates effective spatial separation photoinduced charge carriers with strong capability, resulting formation S-scheme heterojunctions between QDs substantiated situ irradiation X-ray photoelectron spectroscopy, femtosecond transient absorption density functional theory simulations. As anticipated, optimized COF/QDs heterostructures exhibit remarkable enhancements photoreduction performance absence any molecule cocatalyst or scavenger, yielding CO CH4 at rates 41.2 13.7 μmol g–1, respectively. This work provides insights novel organic/inorganic heterojunction photocatalysts separation, offering potential for sustainable artificial photosynthesis.
Language: Английский
Citations
38