
Green Chemical Engineering, Journal Year: 2024, Volume and Issue: unknown
Published: Sept. 1, 2024
Language: Английский
Green Chemical Engineering, Journal Year: 2024, Volume and Issue: unknown
Published: Sept. 1, 2024
Language: Английский
Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: 95, P. 636 - 643
Published: April 26, 2024
Language: Английский
Citations
9Advanced Functional Materials, Journal Year: 2024, Volume and Issue: 34(46)
Published: Aug. 9, 2024
Abstract Carbon materials are of great significance in state‐of‐the‐art electrochemical CO 2 reduction (ECR) as key components such electrocatalysts, gas diffusion electrodes, and current collectors. Notably, dimensionalities carbons related manipulations play vital roles boosting ECR performance, e.g., mass/charge transfer dynamics, exposure active sites, reaction space, product's Faradaic efficiency/selectivity, durability. Here, recent endeavors dimensionality engineering toward advanced carbon‐based for is first summarized, including pure (e.g., carbon nanotube graphene) composites, highlight the dimensionality‐dependent properties performance. Various strategies referring to modulation integration have been top‐down, bottom‐up, soft chemical approaches. Design principles dimensionality‐varied elaborated, impacts surface chemistry functional group, wettability, electronic structure) on kinetics product‐targeted mechanisms also scrutinized. Some insights into how manipulation elevates performance acceleration, kinetics, product selectivity provided. At last, a perspective challenges future development discussed. This review aims at providing guidance customizable construction with dependence green energy‐saving electrosynthesis systems.
Language: Английский
Citations
8Journal of Rare Earths, Journal Year: 2025, Volume and Issue: unknown
Published: Feb. 1, 2025
Language: Английский
Citations
1Science China Chemistry, Journal Year: 2024, Volume and Issue: 67(10), P. 3209 - 3222
Published: Aug. 14, 2024
Language: Английский
Citations
6Green Energy & Environment, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 1, 2025
Language: Английский
Citations
0Hybrid Advances, Journal Year: 2025, Volume and Issue: unknown, P. 100411 - 100411
Published: Feb. 1, 2025
Language: Английский
Citations
0Journal of Energy Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: March 1, 2025
Language: Английский
Citations
0Advanced Functional Materials, Journal Year: 2025, Volume and Issue: unknown
Published: April 16, 2025
Abstract The efficient electrocatalytic conversion of CO 2 to formate is often impeded by the high energy requirements oxygen evolution reaction (OER) and limited activity selectivity reduction (CO RR). Herein, a novel strategy enhance production substituting OER with methanol oxidation (MOR) optimizing cathodic microenvironment interfacial Cl − ions presented. Through theoretical analysis, binder‐free Bi NiOOH electrodes that achieve remarkable Faradaic efficiencies (FE ) exceeding 90% at current densities 50–250 mA·cm −2 for RR MOR, respectively, are identified. These combined experimental investigations demonstrate enrichment on electrode modulates local electronic structure, fostering conducive RR. Bi–NiOOH full cell maintains FE above industry‐level (100–300 ), enabling concurrent electrosynthesis both electrodes. This work highlights critical role anion environments in electrocatalysis provides strategic framework synergistic engineering electrochemical systems.
Language: Английский
Citations
0Journal of Energy Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: April 1, 2025
Language: Английский
Citations
0Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: unknown, P. 124822 - 124822
Published: Nov. 1, 2024
Language: Английский
Citations
2