The Science of The Total Environment,
Journal Year:
2025,
Volume and Issue:
962, P. 178436 - 178436
Published: Jan. 1, 2025
The
widespread
occurrence
of
new
and
emerging
persistent
organic
pollutants
(NEPs
POPs)
in
surface
water
poses
a
risk
to
drinking
supply
consequently
human
health.
aim
this
work
was
investigate
the
potential
transport
42
target
NEPs
POPs
(including
per-and
polyfluoroalkyl
substances
(PFAS),
pharmaceuticals,
pesticides
bisphenols)
along
rural
urban
environments
three
rivers
England.
type
concentrations
varied
between
sampling
days
points.
Two
pharmaceuticals
(diclofenac
ibuprofen),
two
(diethyl-meta-toluamide
(DEET)
prosulfocarb)
range
PFAS
were
detected
above
method
detection
limit.
observed
include
restricted
perfluorooctanoic
acid
(PFOA),
perfluorooctanesulfonic
(PFOS)
newer
generation
substitute
6:2
fluorotelomer
sulfonate
(6:2
FTS).
levels
PFOS
diclofenac
all
studied
exceeded
European
environmental
quality
standard
(EQS).
high
frequency
river
Ouse
suggests
their
persistence
contaminate
connecting
tributaries.
An
assessment
ecological
prosulfocarb
samples
from
Ouse,
using
quotient
method,
showed
algae,
planktonic
crustaceans,
fish.
Our
results
suggest
that
presence
12
POPs,
could
potentially
be
influenced
by
anthropogenic
activities
across
rivers.
study
highlights
need
for
continuous
monitoring
new-generation
chemicals
waters
understand
impact
on
ecosystem
public
This
study
evaluated
PFAS
occurrence
in
rural
well
water
and
surface
relative
to
land
application
of
biosolids
a
tile-drained
agriculture-dominated
watershed.
Spatial
data
were
used
identify
potentially
vulnerable
wells
based
on
their
proximity
biosolid-permitted
location
with
respect
groundwater
flow.
Water
was
collected
from
103
private
Greater
Tippecanoe
County
Indiana
168
locations
within
the
Region
Great
Bend
Wabash
River
Overall,
results
indicate
that
(∑PFAS
≤
169.4
ng/L)
is
more
contamination
than
15.7
ng/L).
Short-chain
perfluoroalkyl
acids
made
up
72%
∑PFAS
both
sources.
Nonetheless,
long-chain
homologues
detected
frequently
(94%)
(82%).
Hierarchical
cluster
analysis
identified
biosolid-applied
fields,
WTTPs,
industrial
discharges
as
sources
first-order
streams
high
∑PFAS.
Temporal
trends
revealed
an
inverse
relationship
between
streamflow
concentrations
sites
impacted
by
point
vice
versa
for
diffuse
sources,
thereby
providing
complementary
evidence
potential
The
set
did
not
show
distinct
spatial
trend
distance
biosolid
or
characteristics.
Environmental Health,
Journal Year:
2023,
Volume and Issue:
22(1)
Published: Aug. 21, 2023
Abstract
Background
Over
40%
of
the
six
million
dry
metric
tons
sewage
sludge,
often
referred
to
as
biosolids,
produced
annually
in
United
States
is
land
applied.
Biosolids
serve
a
sink
for
emerging
pollutants
which
can
be
toxic
and
persist
environment,
yet
their
fate
after
application
impacts
on
human
health
have
not
been
well
studied.
These
gaps
our
understanding
are
exacerbated
by
absence
systematic
monitoring
programs
defined
standards
protection.
Methods
The
purpose
this
paper
call
critical
attention
knowledge
that
currently
exist
regarding
biosolids
underscore
need
evidence-based
testing
regulatory
frameworks
protection
when
A
scoping
review
methodology
was
used
identify
research
conducted
within
last
decade,
current
standards,
government
publications
applied
biosolids.
Results
Current
indicates
persistent
organic
compounds,
or
pollutants,
found
pharmaceuticals
personal
care
products,
microplastics,
per-
polyfluoroalkyl
substances
(PFAS)
potential
contaminate
ground
surface
water,
uptake
these
from
soil
amended
result
contamination
food
sources.
Advanced
technologies
remove
contaminants
wastewater
treatment
plant
influent,
effluent,
destined
along
with
tools
detect
quantify
Conclusions
To
address
risks,
there
needs
significant
investment
ongoing
infrastructure
support
advancements
treatment;
expanded
manufacture
use
sustainable
products;
increased
public
communication
risks
associated
overuse
plastics;
development
implementation
regulations
protective
environment.
Environmental Health Perspectives,
Journal Year:
2023,
Volume and Issue:
131(7)
Published: July 1, 2023
Per-
and
polyfluoroalkyl
substances
(PFAS)
are
ubiquitous
in
the
environment
have
been
shown
to
cause
various
adverse
health
impacts.
In
animals,
sex-
species-specific
differences
PFAS
elimination
half-lives
linked
activity
of
kidney
transporters.
However,
molecular
interactions
with
transporters
still
not
fully
understood.
Moreover,
impact
disease
on
remains
unclear.This
state-of-the-science
review
integrated
current
knowledge
assess
how
changes
function
transporter
expression
from
could
affect
toxicokinetics
identified
priority
research
gaps
that
should
be
addressed
advance
knowledge.We
searched
for
studies
measured
uptake
by
transporters,
quantified
transporter-level
associated
status,
developed
pharmacokinetic
models.
We
then
used
two
databases
identify
untested
potential
transport
based
their
endogenous
substrates.
Finally,
we
an
existing
model
perfluorooctanoic
acid
(PFOA)
male
rats
explore
influence
levels,
glomerular
filtration
rate
(GFR),
serum
albumin
half-lives.The
literature
search
nine
human
eight
rat
were
previously
investigated
ability
PFAS,
as
well
seven
three
confirmed
specific
PFAS.
proposed
a
candidate
list
transport.
Model
results
indicated
PFOA
more
influenced
GFR
than
expression.Studies
additional
particularly
efflux
especially
current-use
needed
better
cover
role
across
class.
Remaining
states
limit
effectiveness
risk
assessment
prevent
identification
vulnerable
populations.
https://doi.org/10.1289/EHP11885.
Environmental Pollution,
Journal Year:
2024,
Volume and Issue:
346, P. 123575 - 123575
Published: Feb. 14, 2024
We
have
investigated
the
occurrence,
distribution,
and
biomagnification
of
per-
polyfluoroalkyl
substances
(PFAS)
in
two
tropical
lakes
(Asejire
Eleyele)
Southwestern
Nigeria,
with
contrasting
urban
intensities.
Over
an
8-month
period,
we
sampled
sediment
fish
species
(Clarias
gariepinus:
CIG;
Oreochromis
niloticus:
ON;
Coptodon
guineensis:
CG;
Sarotherodon
melanotheron:
SM)
across
trophic
levels,
analyzed
various
PFAS
congeners,
addition
to
a
select
group
toxicological
responses.
While
herbivores
(SM)
benthic
omnivores
(CIG)
at
Asejire
exhibited
elevated
levels
PFBS
PFOS,
pelagic
(ON)
showed
dominance
PFDA,
PFHxDA
EtFOSE
muscle.
At
Eleyele
lake,
patterns
was
dominated
by
PFBS,
EtFOSE,
PFPeS,
PFOcDA
PFOS
(SM,
CG),
omnivore
(ClG).
The
estimated
factor
(BMF)
analysis
for
both
indicated
level
increase
PFUnA
PFDA
suburban
while
biomagnified
lake.
detected
occurrence
diSAMPAP
9CL-PF3ONS,
novel
compounds
not
commonly
reported,
studies
lakes.
studied
responses
varied
groups
probable
modulations
environmental
conditions,
structure,
relative
exposures
present
study
documents,
first
time
or
any
other
African
country,
role
urbanization
on
contaminant
load
into
environment
their
implications
dynamics
within
ecosystem
aquatic
food
safety.