Regeneration of graphite from spent lithium‐ion batteries as anode materials through stepwise purification and mild temperature restoration DOI Creative Commons

Shaowen Ji,

Anlong Zhang,

Weiming Hua

et al.

Battery energy, Journal Year: 2024, Volume and Issue: 3(3)

Published: Jan. 23, 2024

Abstract Graphite is one of the most widely used anode materials in lithium‐ion batteries (LIBs). The recycling spent graphite (SG) from LIBs has attracted less attention due to its limited value, complicated contaminations, and unrestored structure. In this study, a remediation regeneration process with combined hydrothermal calcination was proposed remove different impurities as value‐added resources SG. This study focuses on application removal methods for impurity metals by acid leaching under conditions Cu, Li, Co, Mn, Ni Then, mild‐tempreture SG performed residual organic compounds. regenerated (RG) found have better morphology structure increased pore volume, which more favorable embedding desorption lithium (Li) graphite. terms electrochemical performance, first discharge‐specific capacity RG at 0.5 C 359.40 mAh/g, retention 353.49 mAh/g after 100 cycles (retention rate 98.36%). can be green efficient candidate material reduced restoration temperature, metal by‐products.

Language: Английский

Recent advances in rational design for high-performance potassium-ion batteries DOI
Yifan Xu, Yichen Du,

Han Chen

et al.

Chemical Society Reviews, Journal Year: 2024, Volume and Issue: 53(13), P. 7202 - 7298

Published: Jan. 1, 2024

The growing global energy demand necessitates the development of renewable solutions to mitigate greenhouse gas emissions and air pollution. To efficiently utilize yet intermittent sources such as solar wind power, there is a critical need for large-scale storage systems (EES) with high electrochemical performance. While lithium-ion batteries (LIBs) have been successfully used EES, surging price, coupled limited supply crucial metals like lithium cobalt, raised concerns about future sustainability. In this context, potassium-ion (PIBs) emerged promising alternatives commercial LIBs. Leveraging low cost potassium resources, abundant natural reserves, similar chemical properties potassium, PIBs exhibit excellent ion transport kinetics in electrolytes. This review starts from fundamental principles structural regulation PIBs, offering comprehensive overview their current research status. It covers cathode materials, anode electrolytes, binders, separators, combining insights full battery performance, degradation mechanisms,

Language: Английский

Citations

141

Recycling Hazardous and Valuable Electrolyte in Spent Lithium-Ion Batteries: Urgency, Progress, Challenge, and Viable Approach DOI

Bo Niu,

Zhenming Xu,

Jiefeng Xiao

et al.

Chemical Reviews, Journal Year: 2023, Volume and Issue: 123(13), P. 8718 - 8735

Published: June 20, 2023

Recycling spent lithium-ion batteries (LIBs) is becoming a hot global issue due to the huge amount of scrap, hazardous, and valuable materials associated with end-of-life LIBs. The electrolyte, accounting for 10–15 wt % LIBs, most hazardous substance involved in recycling Meanwhile, components, especially Li-based salts, make economically beneficial. However, studies electrolyte still account only small fraction number LIB papers. On other hand, many more about have been published Chinese but are not well-known worldwide limitations language. To build bridge between Western academic achievements on treatments, this Review first illustrates urgency importance analyzes reason its neglect. Then, we introduce principles processes collection methods including mechanical processing, distillation freezing, solvent extraction, supercritical carbon dioxide. We also discuss separation regeneration an emphasis recovering lithium salts. advantages, disadvantages, challenges processes. Moreover, propose five viable approaches industrialized applications efficiently recycle electrolytes that combine different processing steps, ranging from heat mechanochemistry situ catalysis, discharging dioxide extraction. conclude discussion future directions recycling. This will contribute efficiently, environmentally friendly, economically.

Language: Английский

Citations

73

A Review of Lithium-Ion Battery Recycling: Technologies, Sustainability, and Open Issues DOI Creative Commons
Alessandra Zanoletti, Eleonora Carena, Chiara Ferrara

et al.

Batteries, Journal Year: 2024, Volume and Issue: 10(1), P. 38 - 38

Published: Jan. 22, 2024

Lithium-ion batteries (LIBs) are a widely used energy storage technology as they possess high density and characterized by the reversible intercalation/deintercalation of Li ions between electrodes. The rapid development LIBs has led to increased production efficiency lower costs for manufacturers, resulting in growing demand their application across various industries, particularly different types vehicles. In order meet while minimizing climate-impacting emissions, reuse, recycling, repurposing is critical step toward achieving sustainable battery economy. This paper provides comprehensive review lithium-ion covering topics such current recycling technologies, technological advancements, policy gaps, design strategies, funding pilot projects, strategy recycling. Additionally, this emphasizes challenges associated with developing LIB opportunities arising from these challenges, potential innovation creation more circular environmental implications also evaluated methodologies able provide sustainability analysis selected technology. aims enhance comprehension trade-offs encourage discussion on determining “best” route when targets conflict.

Language: Английский

Citations

62

Recycling of spent lithium-ion batteries for a sustainable future: recent advancements DOI Creative Commons
Basanta Kumar Biswal, Bei Zhang, Phuong Thi Minh Tran

et al.

Chemical Society Reviews, Journal Year: 2024, Volume and Issue: 53(11), P. 5552 - 5592

Published: Jan. 1, 2024

A critical review of the recent developments in recycling spent Li-ion batteries using five major technologies (direct recycling, pyrometallurgy, hydrometallurgy, bioleaching and electrometallurgy) evaluation their sustainability.

Language: Английский

Citations

62

Pyrometallurgical recycling of spent lithium-ion batteries from conventional roasting to synergistic pyrolysis with organic wastes DOI
Chao Pan, Yafei Shen

Journal of Energy Chemistry, Journal Year: 2023, Volume and Issue: 85, P. 547 - 561

Published: July 25, 2023

Language: Английский

Citations

51

Non–closed–loop recycling strategies for spent lithium–ion batteries: Current status and future prospects DOI
Haoxuan Yu,

Haitao Yang,

Kechun Chen

et al.

Energy storage materials, Journal Year: 2024, Volume and Issue: 67, P. 103288 - 103288

Published: Feb. 21, 2024

Language: Английский

Citations

31

Bubbles to batteries: A review of froth flotation for sustainably recycling spent lithium-ion batteries DOI
Sabereh Nazari, Ali Behrad Vakylabad,

Kaveh Asgari

et al.

Journal of Energy Storage, Journal Year: 2024, Volume and Issue: 84, P. 110702 - 110702

Published: Feb. 15, 2024

Language: Английский

Citations

24

A review of lithium-ion battery recycling for enabling a circular economy DOI Creative Commons

Mina Rezaei,

Atiyeh Nekahi,

Anil Kumar M R

et al.

Journal of Power Sources, Journal Year: 2025, Volume and Issue: 630, P. 236157 - 236157

Published: Jan. 8, 2025

Language: Английский

Citations

5

Recycling technologies of spent lithium-ion batteries and future directions: A review DOI Open Access
Xuesong Gao, Meng Wu,

Guangjin Zhao

et al.

Transactions of Nonferrous Metals Society of China, Journal Year: 2025, Volume and Issue: 35(1), P. 271 - 295

Published: Jan. 1, 2025

Language: Английский

Citations

4

Direct regeneration and flash upcycling of mixed spent graphite with a uniform energy-storage property DOI
Zhen Shang,

Zhang Naizhe,

Zhiwen Ying

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 159132 - 159132

Published: Jan. 1, 2025

Language: Английский

Citations

2