Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: May 2, 2025

Abstract Single‐atom catalysts (SACs) have garnered significant attention in the applications of environmental remediation based on Fenton‐like systems. Current research single‐atom catalysis often emphasizes catalytic activity and mechanism regulation, while paying limited to simultaneous enhancement both stability—a critical factor for practical scale‐up SACs. This review systematically summarizes recent advances synchronization strategies improving stability catalysis, with a focus design principles mechanisms four key strategies: coordination engineering, confinement effects, carrier substitution, module design. To best knowledge, this represents first comprehensive from perspective concurrent optimization stability. Additionally, auxiliary role machine learning lifecycle assessment (LCA) is evaluated advancing these strategies. By investigating interplay among different support materials, configurations, reaction environments, as well enlarged modules, factors governing stability/activity SACs are highlighted, future directions proposed developing next‐generation high efficiency long‐term durability remediation.

Language: Английский