International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: unknown, P. 141261 - 141261
Published: Feb. 1, 2025
Language: Английский
International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: unknown, P. 141261 - 141261
Published: Feb. 1, 2025
Language: Английский
Progress in Materials Science, Journal Year: 2024, Volume and Issue: 144, P. 101288 - 101288
Published: March 21, 2024
Language: Английский
Citations
26Small, Journal Year: 2023, Volume and Issue: 20(23)
Published: Dec. 26, 2023
Abstract Whereas thermal comfort and healthcare management during long‐term wear are essentially required for wearable system, simultaneously achieving them remains challenge. Herein, a highly comfortable breathable smart textile personal is developed, via assembling stimuli‐responsive core–sheath dual network that silver nanowires(AgNWs) core interlocked graphene sheath induced by MXene. Small MXene nanosheets with abundant groups proposed as novel “dispersant” to according “like dissolves like” theory, while acting “cross‐linker” between AgNWs networks filling the voids them. The heterogeneous conductive fiber “cross‐linking” exhibits reliable response various mechanical/electrical/light stimuli, even under large mechanical deformations(100%). fiber‐enabled can adapt movements of human body seamlessly, convert these deformations into character signals accurate monitoring rapid response(440 ms). Moreover, excellent Joule heating photothermal effect instant energy harvesting/storage stimuli‐response process, which be developed self‐powered dynamic camouflage when integrated phase change thermochromic layer. fibers/textiles structures hold great promise in personalized management.
Language: Английский
Citations
29Advanced Functional Materials, Journal Year: 2023, Volume and Issue: 34(11)
Published: Dec. 3, 2023
Abstract The cracks in flexible triboelectric nanogenerators (TENG) cannot naturally repair themselves during low‐temperature operation, which significantly restricts their practical applications. Yet, the development of elastomers capable self‐repair at low temperatures has remained a formidable challenge. In this study, dual dynamic cross‐linking network using multiple hydrogen bonds and β ‐hydroxy esters is constructed to fabricate fully bio‐based elastomer known as PLMBE. This can be stretched up an impressive 1200% its original length possesses remarkable autonomous self‐healing capability even under harsh conditions, including (−10 °C, 12 h, with 75% efficiency rate) exposure supercooled, high‐concentration saline (10% NaCl solution −10 64% rate). These properties are attributed elastomer's glass transition temperature (Tg) −30 °C abundance hydrogen‐bonded supramolecular interactions. Importantly, highly suitable layer for creating TENG (Bio‐TENG) . results demonstrate that Bio‐TENG achieve output power density 2.4 W m −2 , voltage recovers 95% after °C. Consequently, these have promising applications various fields, energy storage devices.
Language: Английский
Citations
27Polymers, Journal Year: 2023, Volume and Issue: 15(22), P. 4383 - 4383
Published: Nov. 11, 2023
Since the invention of triboelectric nanogenerator (TENG), porous polymer materials (PPMs), with different geometries and topologies, have been utilized to enhance output performance expand functionality TENGs. In this review, basic characteristics preparation methods various PPMs are introduced, along their applications in TENGs on basis roles as electrodes, surfaces, structural materials. According pore size dimensionality, types that built hydrogels, aerogels, foams, fibrous media classified advantages disadvantages analyzed. To deepen understanding future development trend, intelligent multifunctional human–machine interfaces, smart wearable devices, self-powering sensors introduced. Finally, directions challenges explored provide possible guidance TENG-based devices systems.
Language: Английский
Citations
25Nano Energy, Journal Year: 2024, Volume and Issue: 126, P. 109675 - 109675
Published: April 24, 2024
Language: Английский
Citations
10ACS Applied Polymer Materials, Journal Year: 2023, Volume and Issue: 5(10), P. 8720 - 8734
Published: Oct. 3, 2023
Although some progress has been achieved in flexible strain sensors, it is still a big challenge to develop sensors with excellent self-healing capability, adhesive, and recyclable properties for enhanced lifespan, facile operation, decreased waste pollution the electronic field. In this study, we successfully synthesized pyrene-terminated multifunctional polyurethane elastomer called PMFPU based on dynamic covalent bond noncovalent hydrogen bonds, which integrates exceptional tough mechanical (the tensile toughness of 168.4 MJ/m3), performance (healing efficiency 96%), superior adhesive property (shear strength as high 1.46 MPa), well-performed reprocessability (more than five cycles). Furthermore, applied fabrication stretchable π–π stacking interactions between pyrene carbon nanotubes (CNTs). Based unique design, obtained can dissolve THF DMF solvents, enabling reprocessing ability avoiding pollution. The could detect human movements facial expressions. Moreover, restore stable sensing capabilities even after repaired process or process, significant importance development environmentally friendly high-performance sensors. these functional holds broad application prospects fields such medical monitoring, human–machine interaction, skin.
Language: Английский
Citations
19ACS Applied Materials & Interfaces, Journal Year: 2023, Volume and Issue: 15(42), P. 49689 - 49700
Published: Oct. 12, 2023
In nature, living organisms, such as octopuses, cabrito, and frogs, have already evolved admirable adhesive abilities for better movement predation in response to the surroundings. Inspired by biological structures, researchers made enormous efforts developing actuators that can respond external stimuli, while property is very desired, yet there still limited research responsive hydrogel actuators. Here, a bilayer actuator with high stretchability robust interface bonding presented, which has smart adhesion thermoreception function. The system consists of an passive layer copolymerized amphoteric ([2-(methacryloyloxy) ethyl] dimethyl-(3-sulfopropyl), SBMA) acrylic acid (AA), active composed poly(N-isopropylacrylamide) (PNIPAm) containing polydopamine-modified MXene (P-MXene) calcium chloride (CaCl2). coordination carboxylate Ca2+ at two layers enhances interfacial from 14 30 N m–1, facilitates withstanding large strain preventing stratification. resulting bend approximately 360° mere 10 s, exhibiting excellent photothermal effect, angle bending deformation, ultrafast photoresponsive ability. As proof concept, are programmed present various shapes grab objects. Importantly, exhibits remarkable capabilities toward diverse substrates, maximum peel force up 280 m–1. Relying on their own photoresponse properties, these flexible show outstanding gripping capability, enabling them grip release objects different weights. More interestingly, adjustable capability temperatures, enables it gripper recognize temperature signals through real-time feedback actions based its adhesion. This study presents innovative insights into biomimetic actuators, providing new opportunities intelligent soft robots multiple functions.
Language: Английский
Citations
17Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 158871 - 158871
Published: Dec. 1, 2024
Language: Английский
Citations
7SusMat, Journal Year: 2024, Volume and Issue: 4(3)
Published: May 27, 2024
Abstract Spider silk, possessing exceptional combination properties, is classified as a bio‐gel fiber. Thereby, it serves valuable origin of inspiration for the advancement various artificial gel fiber materials with distinct functionalities. Gel fibers exhibit promising potential utilization in diverse fields, including smart textiles, muscle, tissue engineering, and strain sensing. However, there are still numerous challenges improving performance functionalizing applications spider silk‐inspired fibers. Thus, to gain penetrating insight into bioinspired fibers, this review provided comprehensive overview encompassing three key aspects: fundamental design concepts implementing strategies properties strengthening functionalities application prospects In particular, multiple toughening mechanisms were introduced at micro, nano, molecular‐level structures Additionally, existing summarized. This aims offer significant guidance development inspire further research field high‐performance
Language: Английский
Citations
6Nano Energy, Journal Year: 2023, Volume and Issue: 118, P. 108950 - 108950
Published: Sept. 28, 2023
Language: Английский
Citations
14