Published: Jan. 1, 2024
Language: Английский
Published: Jan. 1, 2024
Language: Английский
Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 493, P. 152558 - 152558
Published: May 25, 2024
Language: Английский
Citations
29ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(27), P. 35400 - 35409
Published: June 25, 2024
A series of dual-band photomultiplication (PM)-type organic photodetectors (OPDs) were fabricated by employing a donor(s)/acceptor (100:1, wt/wt) mixed layer and an ultrathin Y6 as the active layers, well using PNDIT-F3N interfacial near indium tin oxide (ITO) electrode. The PM-type OPDs exhibit response range 330–650 nm under forward bias 650–850 reverse bias. tunable spectral or can be explained from trapped electron distribution electrodes. dark current density (JD) efficiently suppressed anode special layers with hole-only transport characteristics. light (JL) slightly increased incorporating wide-bandgap polymer P-TPDs relatively large hole mobility (μh) in layers. signal-to-noise ratios optimized reach 100,980 −50 V white illumination intensity 1.0 mW·cm–2, benefiting ultralow JD buffer JL appropriate P-TPD
Language: Английский
Citations
28Advanced Materials, Journal Year: 2024, Volume and Issue: 36(21)
Published: Feb. 9, 2024
Abstract Ternary strategyopens a simple avenue to improve the power conversion efficiency (PCE) of organic solar cells (OSCs). The introduction wide bandgap polymer donors (PDs) as third component canbetter utilize sunlight and mechanical thermal stability active layer. However, efficient ternary OSCs (TOSCs) with two PDs are rarely reported due inferior compatibility shortage match acceptors. Herein, PDs‐(PBB‐F PBB‐Cl) adopted in dual‐PDs systems explore underlying mechanisms their photovoltaic performance. findings demonstrate that components exhibit excellent miscibility PM6 embedded host donor form alloy‐like phase. A more profound mechanism for enhancing through dual mechanisms, guest energy transfer charge transport at donor/acceptor interface, has been proposed. Consequently, PM6:PBB‐Cl:BTP‐eC9 TOSCs achieve PCE over 19%. Furthermore, better than binary reduction spatial site resistance resulting from tightly entangled long‐chain structure. This work not only provides an effective approach fabricate high‐performance TOSCs, but also demonstrates importance developing compatible PD materials.
Language: Английский
Citations
27Joule, Journal Year: 2024, Volume and Issue: 8(8), P. 2250 - 2264
Published: June 12, 2024
Language: Английский
Citations
23Journal of Semiconductors, Journal Year: 2024, Volume and Issue: 45(5), P. 050201 - 050201
Published: May 1, 2024
Language: Английский
Citations
8Nano-Micro Letters, Journal Year: 2024, Volume and Issue: 17(1)
Published: Nov. 27, 2024
Abstract Trap-assisted charge recombination is one of the primary limitations restricting performance organic solar cells. However, effectively reducing presence traps in photoactive layer remains challenging. Herein, wide bandgap polymer donor PTzBI-dF demonstrated as an effective modulator for enhancing crystallinity bulk heterojunction active layers composed D18 derivatives blended with Y6, leading to dense and ordered molecular packings, thus, improves photoluminescence quenching properties. As a result, photovoltaic devices exhibit reduced trap-assisted losses, achieving optimized power conversion efficiency over 19%. Besides enhancement, comprised third component simultaneously attain decreased current leakage, improved carrier mobilities, suppressed bimolecular recombination, energy losses. The advanced crystalline structures induced by its characteristics, such well-aligned level, complementary absorption spectra, are ascribed promising improvements. Our findings suggest that phase engineering feasible approach tuning packings layer, providing guidelines designing morphology modulators high-performance
Language: Английский
Citations
8Advanced Energy Materials, Journal Year: 2024, Volume and Issue: unknown
Published: Sept. 13, 2024
Abstract All‐polymer systems are promising for commercial applications because the lower diffusivity of polymers helps to inhibit large‐scaled phase separation and obtain excellent stability. Achieving a fine‐tuned morphology active layer with an appropriate vertical has long been major goal in obtaining efficient all‐polymer solar cells (all‐PSCs). Herein, through synergistic effect layer‐by‐layer (LBL) structure dual donor strategy, high performance stable all‐PSCs prepared by constructing interpenetrating network. The introduction third component PTzBI‐dF suppresses excessive aggregation reduces exciton recombination. formation favorable p‐i‐n adjust distribution improve Ultimately, fine optimization, PBQx‐T‐Cl:PTzBI‐dF/PY‐IT achieves PCE 18.83%. This research demonstrates simple effective way construct high‐performance OSCs desirable distribution.
Language: Английский
Citations
7Journal of Energy Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 1, 2025
Language: Английский
Citations
1ChemSusChem, Journal Year: 2024, Volume and Issue: 17(16)
Published: March 21, 2024
The large open circuit voltage (V
Language: Английский
Citations
5Cell Reports Physical Science, Journal Year: 2025, Volume and Issue: 6(1), P. 102390 - 102390
Published: Jan. 1, 2025
Language: Английский
Citations
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