MXene‐Supported Single‐Atom Electrocatalysts DOI Creative Commons

Jianan He,

Joshua D. Butson, R. Gu

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: March 27, 2025

MXenes, a novel member of the 2D material family, shows promising potential in stabilizing isolated atoms and maximizing atom utilization efficiency for catalytic applications. This review focuses on role MXenes as support single-atom catalysts (SACs) various electrochemical reactions, namely hydrogen evolution reaction (HER), oxygen (OER), reduction (ORR), carbon dioxide (CO2RR), nitrogen (NRR). First, state-of-the-art characterization synthesis methods MXene-supported SACs are discussed, highlighting how unique structure tunable functional groups enhance performance pristine contribute to SAs. Then, recent studies different electrocatalytic areas examined, including experimental theoretical studies. Finally, this discusses challenges outlook field electrocatalysis.

Language: Английский

The Loss of Interfacial Water-Adsorbate Hydrogen Bond Connectivity Position Surface-Active Hydrogen as a Crucial Intermediate to Enhance Nitrate Reduction Reaction DOI

Shisheng Zheng,

X. Yang,

Zhong-Zhang Shi

et al.

Journal of the American Chemical Society, Journal Year: 2024, Volume and Issue: unknown

Published: Sept. 20, 2024

The electrochemical nitrate reduction reaction (NO

Language: Английский

Citations

9
Structure properties and industrial applications of anion exchange resins for the removal of electroactive nitrate ions from contaminated water DOI Creative Commons

Mohammad Faraz Ahmer,

Mohammad Kashif Uddin

RSC Advances, Journal Year: 2024, Volume and Issue: 14(45), P. 33629 - 33648

Published: Jan. 1, 2024

A review of the properties anion exchange resins and their industrial applications for adsorption electroactive nitrate ions.

Language: Английский

Citations

6
Ab Initio Study of a Tandem PdCu Catalyst Supported on Carbon Nitride Nanosheets for Nitrate-to-Ammonia Electrochemical Reduction DOI
Zhe Xue, Rui Tan,

Jinzhong Tian

et al.

ACS Applied Nano Materials, Journal Year: 2025, Volume and Issue: 8(4), P. 1709 - 1717

Published: Jan. 15, 2025

Electrochemical conversion of nitrate offers an efficient approach to mitigate pollution and ammonia synthesis but is still challenged by the slow kinetics selectivity issues active sites. Herein, performing density functional theory (DFT) calculations, we report a double-atom catalyst PdCu–C7N6 incorporating Pd Cu together embedded in C7N6 frameworks, which not only shows outstanding catalytic performance with low limiting potential 0.36 V, also can effectively inhibit competing hydrogen evolution reactions. The high NO3RR activity on well explained polarizable bond length as asymmetric charge distribution Pd–Cu dual This DFT work opens avenue for developing highly multicomponent electrocatalysts.

Language: Английский

Citations

0
Advances in electrocatalytic nitrate reduction to ammonia over Cu-based catalysts DOI
Zhibin Zhang, Kailun Yu, Hui Wang

et al.

Environmental Research, Journal Year: 2025, Volume and Issue: unknown, P. 121123 - 121123

Published: Feb. 1, 2025

Language: Английский

Citations

0
Surface reconstruction induced Cu2O/FeO heterojunction towards efficient nitrate-containing wastewater remediation DOI

Le Ding,

Haosheng Lan,

Xin Li

et al.

Journal of Colloid and Interface Science, Journal Year: 2025, Volume and Issue: unknown, P. 137318 - 137318

Published: March 1, 2025

Language: Английский

Citations

0
MXene‐Supported Single‐Atom Electrocatalysts DOI Creative Commons

Jianan He,

Joshua D. Butson, R. Gu

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: March 27, 2025

MXenes, a novel member of the 2D material family, shows promising potential in stabilizing isolated atoms and maximizing atom utilization efficiency for catalytic applications. This review focuses on role MXenes as support single-atom catalysts (SACs) various electrochemical reactions, namely hydrogen evolution reaction (HER), oxygen (OER), reduction (ORR), carbon dioxide (CO2RR), nitrogen (NRR). First, state-of-the-art characterization synthesis methods MXene-supported SACs are discussed, highlighting how unique structure tunable functional groups enhance performance pristine contribute to SAs. Then, recent studies different electrocatalytic areas examined, including experimental theoretical studies. Finally, this discusses challenges outlook field electrocatalysis.

Language: Английский

Citations

0