Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 157783 - 157783
Published: Nov. 1, 2024
Language: Английский
Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 157783 - 157783
Published: Nov. 1, 2024
Language: Английский
ACS Catalysis, Journal Year: 2024, Volume and Issue: unknown, P. 13697 - 13722
Published: Aug. 30, 2024
Electrocatalytic carbon dioxide reduction (CO2RR) over Cu-based catalysts has emerged as a promising strategy for value-added artificial cycling, addressing the current climate and energy challenges. However, product selectivity long-term stability of are limited by their instability at constant potential. Recent advancements in pulsed techniques aim to overcome these limitations, enhancing industrial feasibility CO2RR systems. This review critically examines recent research progress catalysts, offering comprehensive synthesis findings. Key pulse parameters characterization strategies explored uncover mechanisms behind enhanced performance. The focus is on surface reconstruction, encompassing regeneration stabilization Cu oxidation states alongside morphological evolution, while also discussing microenvironment changes, including local CO2 concentration, pH, ionic arrangement. intricate modulation mode, potential, duration performance elucidated, highlighting interconnections. Finally, we identify prevailing challenges propose future directions achieving environmentally friendly economically viable cycling. By providing insightful perspectives optimizing CO2RR, this paves way developing more efficient robust catalytic
Language: Английский
Citations
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Language: Английский
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1Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 157783 - 157783
Published: Nov. 1, 2024
Language: Английский
Citations
0