Controlled Self‐Assembly and Photo‐Thermal Activation of Viologen‐Based 2D Semiconductors for Dual‐Function Energy Management in All‐Weather Applications
Advanced Science,
Journal Year:
2025,
Volume and Issue:
unknown
Published: Feb. 8, 2025
Solar
thermal
technology
offers
a
promising
solution
to
water
scarcity;
however,
the
continuous
operation
of
solar
evaporators
remains
challenging
due
sunlight's
intermittent
availability.
Herein,
an
alternative
strategy
is
proposed
achieve
dual-functional
energy
management
photo-thermoactivated
viologen
T
semiconductors
for
enhanced
evaporation,
water-enabled
electricity
generation,
and
electrothermal
evaporation.
A
sequential
cyanide-bridged
layer-directed
intercalation
approach
developed,
where
infinitely
π-stacked,
redox-active
N-methyl
bipyridinium
cations
with
near-planar
structures
are
sandwiched
between
MnII-FeIII.
The
extended
absorption
range
95%
achieved
through
radical-π
interactions
that
occur
within
continuously
π-stacked
units
upon
activation.
MnII-FeIII
compounds
anchored
charcoal
mask
(MnII-FeIII@CM)
sided
evaporation
structure
controllable
transfer,
offering
high
rate
2.39
kg
m-2
h-1
under
one
sun
(1
kW
m-2)
illumination.
As
nanogenerator,
output
voltage
current
MnII-FeIII@CM
can
reach
up
≈480
mV
≈60
µA
cm-2
ambient
conditions.
Furthermore,
storage
electrical
from
using
devices
expected
enable
all-weather
by
electric
heating
unsustainable
sunlight,
providing
unique
seawater
desalination
offshore
work
platform
access.
Language: Английский
Engineering wood-MOF networks to realize multilevel weak water interactions for highly-efficient solar water-power cogeneration
Hongbin Li,
No information about this author
Rongcui Fan,
No information about this author
Fudong Zhang
No information about this author
et al.
Chemical Engineering Journal,
Journal Year:
2025,
Volume and Issue:
unknown, P. 161332 - 161332
Published: March 1, 2025
Language: Английский
Efficient interfacial solar-driven evaporation and hydroelectric co-generation by Al-Fum metal-organic framework-derived porous carbon
Erhui Xu,
No information about this author
Weikang Han,
No information about this author
Guixin Hu
No information about this author
et al.
Sustainable materials and technologies,
Journal Year:
2025,
Volume and Issue:
unknown, P. e01356 - e01356
Published: March 1, 2025
Language: Английский
Flexible and transparent bamboo composites Enabled by a Dual-Resin blending strategy
Chemical Engineering Journal,
Journal Year:
2025,
Volume and Issue:
unknown, P. 161256 - 161256
Published: March 1, 2025
Language: Английский
Polymer semiconductor-coated 3D bilayer cellulose nanofiber/polydimethylsiloxane aerogel for enhanced solar-driven interfacial water evaporation
Desalination,
Journal Year:
2025,
Volume and Issue:
unknown, P. 118947 - 118947
Published: April 1, 2025
Language: Английский
MXene/Bacterial Cellulose Hybrid Materials for Sustainable Soft Electronics
Materials,
Journal Year:
2024,
Volume and Issue:
17(22), P. 5513 - 5513
Published: Nov. 12, 2024
This
work
evaluated
bacterial
cellulose
(BC)
as
a
possible
biodegradable
soft
electronics
substrate
in
comparison
to
polyethylene
terephthalate
(PET),
while
also
focusing
on
evaluating
hybrid
MXene/BC
material
potential
flexible
electronic
sensor.
Material
characterization
studies
revealed
that
the
BC
structure
consists
of
nanofibers
with
diameters
ranging
from
70
140
nm,
stacked
layer-by-layer.
samples
produced
are
sensitive
post-treatment
isopropanol
resulting
change
structural
and
mechanical
properties.
The
viscoelastic
properties
substrates
have
been
studied
experimentally
PET
film.
Aged
showcased
similar
stability,
exhibiting
better
above
°C,
total
storage
modulus
−15%
loss
21%.
MXenes
prepared
using
Minimally
Intensive
Layer
Delamination
(MILD)
method
were
screen-printed
onto
films
form
(MX/BC)
MXene/PET
(MX/PET)
devices.
electrical
results
different
resistive
behavior
both
impedance
moduli.
MX/PET
presented
lower
sheet
resistance
around
156
Ω·sq−1,
MX/BC
was
2733
Ω·sq−1.
Finally,
devices
subjected
repeatable
quasi-static
load
tests
piezoresistive
sensing
has
reported.
Language: Английский