Self-Association and Microhydration of Phenol: Identification of Large-Amplitude Hydrogen Bond Librational Modes DOI Creative Commons
Dmytro Mihrin, Karen L. Feilberg, René Wugt Larsen

et al.

Molecules, Journal Year: 2024, Volume and Issue: 29(13), P. 3012 - 3012

Published: June 25, 2024

The self-association mechanisms of phenol have represented long-standing challenges to quantum chemical methodologies owing the competition between strongly directional intermolecular hydrogen bonding, weaker non-directional London dispersion forces and C-H⋯π interactions aromatic rings. present work explores these subtle relevance for biological molecular recognition processes via spectroscopic observations large-amplitude bond librational modes cluster molecules embedded in inert neon "quantum" matrices complemented by domain-based local pair natural orbital-coupled DLPNO-CCSD(T) theory. spectral signatures confirm a primarily O-H⋯H hydrogen-bonded structure dimer strengthened further cooperative contributions from inter-ring as supported DLPNO-based energy decomposition (LED) predictions. In same way, bands observed trimeric molecule pseudo-

Language: Английский

OH-Detected Aromatic Microsolvation of an Organic NO Radical: Halogenation Controls the Solvation Side DOI Creative Commons
Elisabeth Sennert, Giovanni Bistoni, Martin A. Suhm

et al.

The Journal of Physical Chemistry A, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 30, 2025

The persistent organic radical 2,2,6,6-tetramethylpiperidinyloxyl (TEMPO) protects its NO center by four methyl groups. Two of them are arranged tightly (t) on one side the six-membered puckered heterocycle, and other two more openly (o) side. It is shown OH stretching infrared spectroscopy in heated supersonic jet expansions that hydrogen bond aromatic ring a first solvating benzyl alcohol have almost no preference for either An increased t develops para-halogenated alcohols, it inverted ortho-halogenated alcohols. experimental dependence actual halogen (Cl, Br, I) weak, whereas different quantum chemical approaches predict or less pronounced trends along series. Some pre-expansion reservoir reduces TEMPO to closed-shell heterocyclic hydroxylamine TEMPO-H (1-hydroxy-2,2,6,6-tetramethylpiperidine), extent TEMPO-H···TEMPO complex observed as an impurity.

Language: Английский

Citations

0

Advancing CO2 absorbents through structural innovation: Implementation of the aromatic multi-ring based nucleophilic structure DOI
Seon Ho Kim,

Jihun Ju,

Jaehan Jo

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: 512, P. 162328 - 162328

Published: April 14, 2025

Language: Английский

Citations

0

Self-aggregation and microhydration mechanisms of monoethanolamine: Far-infrared identification of large-amplitude hydrogen bond libration DOI
Sahar Hafizi Yazdabadi, Dmytro Mihrin, Karen L. Feilberg

et al.

The Journal of Chemical Physics, Journal Year: 2024, Volume and Issue: 161(15)

Published: Oct. 15, 2024

The strong tendency for self-aggregation together with an intriguing mechanism the microhydration of monoethanolamine (MEA) have been explored by low-temperature far-infrared cluster spectroscopy in doped neon "quantum" matrices at 4 K complemented high-level quantum chemical modeling. In addition to assignment new mid-infrared perturbed intramolecular transitions, a distinct transition is unambiguously assigned concerted large-amplitude hydrogen bond librational motion MEA homodimer. This observation confirms global "head-to-head" intermolecular potential energy minimum associated formation compact doubly OH⋯N hydrogen-bonded cyclic structure, where both monomeric bonds are broken upon complexation. By means relative mixing ratio dependencies, dedicated annealing procedures, and selective complexation between isotopic H216O H218O samples, transitions intra-molecular hindered OH torsional inter-molecular H2O (hindered c-type overall rotational) monohydrate furthermore first time. These spectroscopic observations reveal metastable conformation, acts as OH⋯O donor hydroxy group instead amino cryogenic environment, strengthens due cooperativity.

Language: Английский

Citations

3

Self-Association and Microhydration of Phenol: Identification of Large-Amplitude Hydrogen Bond Librational Modes DOI Creative Commons
Dmytro Mihrin, Karen L. Feilberg, René Wugt Larsen

et al.

Molecules, Journal Year: 2024, Volume and Issue: 29(13), P. 3012 - 3012

Published: June 25, 2024

The self-association mechanisms of phenol have represented long-standing challenges to quantum chemical methodologies owing the competition between strongly directional intermolecular hydrogen bonding, weaker non-directional London dispersion forces and C-H⋯π interactions aromatic rings. present work explores these subtle relevance for biological molecular recognition processes via spectroscopic observations large-amplitude bond librational modes cluster molecules embedded in inert neon "quantum" matrices complemented by domain-based local pair natural orbital-coupled DLPNO-CCSD(T) theory. spectral signatures confirm a primarily O-H⋯H hydrogen-bonded structure dimer strengthened further cooperative contributions from inter-ring as supported DLPNO-based energy decomposition (LED) predictions. In same way, bands observed trimeric molecule pseudo-

Language: Английский

Citations

2