Journal of Materials Chemistry B,
Journal Year:
2020,
Volume and Issue:
8(16), P. 3171 - 3191
Published: Jan. 1, 2020
Stimuli-responsive
hydrogel
strain
sensors
that
synergize
the
advantages
of
both
and
smart
functional
materials
have
attracted
increasing
interest
from
material
design
to
emerging
applications
in
health
monitors
human–machine
interfaces.
Advanced Functional Materials,
Journal Year:
2020,
Volume and Issue:
30(25)
Published: April 20, 2020
Abstract
Wearable
and
implantable
bioelectronics
are
receiving
a
great
deal
of
attention
because
they
offer
huge
promise
in
personalized
healthcare.
Currently
available
generally
rely
on
external
aids
to
form
an
attachment
the
human
body,
which
leads
unstable
performance
practical
applications.
Self‐adhesive
highly
desirable
for
ameliorating
these
concerns
by
offering
reliable
conformal
contact
with
tissue,
stability
fidelity
signal
detection.
However,
achieving
adequate
long‐term
self‐adhesion
soft
wet
biological
tissues
has
been
daunting
challenge.
Recently,
mussel‐inspired
hydrogels
have
emerged
as
promising
candidates
design
self‐adhesive
bioelectronics.
In
addition
self‐adhesiveness,
chemistry
offers
unique
pathway
integrating
multiple
functional
properties
all‐in‐one
bioelectronic
devices,
implications
healthcare
this
report,
recent
progress
area
is
highlighted
specifically
discussing:
1)
adhesion
mechanism
mussels,
2)
repeatable
adhesion,
3)
advance
development
hydrogel
reconciling
self‐adhesiveness
additional
including
conductivity,
toughness,
transparency,
self‐healing,
antibacterial
properties,
tolerance
extreme
environment,
4)
challenges
prospects
future
Small,
Journal Year:
2021,
Volume and Issue:
18(5)
Published: Oct. 17, 2021
Abstract
Conductive
hydrogels
can
be
prepared
by
incorporating
various
conductive
materials
into
polymeric
network
hydrogels.
In
recent
years,
have
been
developed
and
applied
in
the
field
of
strain
sensors
owing
to
their
unique
properties,
such
as
electrical
conductivity,
mechanical
self‐healing,
anti‐freezing
properties.
These
remarkable
properties
allow
hydrogel‐based
show
excellent
performance
for
identifying
external
stimuli
detecting
human
body
movement,
even
at
subzero
temperatures.
This
review
summarizes
application
fabrication
working
different
modes.
Finally,
a
brief
prospectus
development
future
is
provided.
ACS Materials Letters,
Journal Year:
2020,
Volume and Issue:
2(10), P. 1287 - 1301
Published: Aug. 25, 2020
Conductive
hydrogels
are
widely
used
in
various
applications,
such
as
artificial
skin,
flexible
and
implantable
bioelectronics,
tissue
engineering.
However,
it
is
still
a
challenge
to
formulate
with
high
electrical
conductivity
without
compromising
their
physicochemical
properties
(e.g.,
toughness,
stretchability,
biocompatibility).
Additionally,
incorporating
other
functions,
self-healing,
shape
memory,
wet
adhesion,
into
conductive
critical
many
practical
applications
of
hydrogel
bioelectronics.
In
this
Review,
we
highlight
recent
progress
the
development
functional
hydrogels.
We,
then,
discuss
potential
challenges
faced
by
areas
wearable/implantable
electronics
cell/tissue
can
serve
an
important
building
block
for
bioelectronic
devices
personalized
healthcare
bioengineering
areas.
Advanced Functional Materials,
Journal Year:
2020,
Volume and Issue:
30(48)
Published: Sept. 18, 2020
Abstract
Conductive
hydrogels
are
promising
interface
materials
utilized
in
bioelectronics
for
human–machine
interactions.
However,
the
low‐temperature
induced
freezing
problem
and
water
evaporation‐induced
structural
failures
have
significantly
hindered
their
practical
applications.
To
address
these
problems,
herein,
an
elaborately
designed
nanocomposite
organohydrogel
is
fabricated
by
introducing
highly
conductive
MXene
nanosheets
into
a
tannic
acid‐decorated
cellulose
nanofibrils/polyacrylamide
hybrid
gel
network
infiltrated
with
glycerol
(Gly)/water
binary
solvent.
Owing
to
introduction
of
Gly,
as‐prepared
demonstrates
outstanding
flexibility
electrical
conductivity
under
wide
temperature
spectrum
(from
−36
60
°C),
exhibits
long‐term
stability
open
environment
(>7
days).
Additionally,
dynamic
catechol‐borate
ester
bonds,
along
readily
formed
hydrogen
bonds
between
Gly
molecules,
further
endow
excellent
stretchability
(≈1500%
strain),
high
tissue
adhesiveness,
self‐healing
properties.
The
favorable
environmental
broad
working
strain
range
(≈500%
strain);
together
sensitivity
(gauge
factor
8.21)
make
this
candidate
both
large
subtle
motion
monitoring.
ACS Nano,
Journal Year:
2021,
Volume and Issue:
15(2), P. 1960 - 2004
Published: Feb. 3, 2021
Patient-friendly
medical
diagnostics
and
treatments
have
been
receiving
a
great
deal
of
interest
due
to
their
rapid
cost-effective
health
care
applications
with
minimized
risk
infection,
which
has
the
potential
replace
conventional
hospital-based
procedures.
In
particular,
integration
recently
developed
materials
into
devices
allows
development
point-of-care
(POC)
sensing
platforms
implantable
special
functionalities.
this
review,
recent
advances
in
biosensors
for
patient-friendly
diagnosis
treatment
are
discussed.
Comprehensive
analysis
portable
wearable
biosensing
monitoring
disease
is
provided,
including
topics
such
as
selection,
device
structure
integration,
biomarker
detection
strategies.
Moreover,
specific
challenges
related
each
biological
fluid
biosensor-based
POC
presented.
Also,
devices,
wireless
communication
strategies,
Furthermore,
various
surgical
approaches
reviewed,
minimally
invasive
insertion
mounting,
vivo
electrical
optical
modulations,
post-operation
monitoring.
Finally,
future
perspectives
toward
provided.
ACS Applied Bio Materials,
Journal Year:
2020,
Volume and Issue:
4(1), P. 85 - 121
Published: Aug. 17, 2020
Natural
biopolymer-based
conductive
hydrogels,
which
combine
inherent
renewable,
nontoxic
features,
biocompatibility
and
biodegradability
of
biopolymers,
excellent
flexibility
conductivity
exhibit
great
potential
in
applications
wearable
stretchable
sensing
devices.
Compared
to
traditional
flexible
substrates
deriving
from
petro-materials-derived
polymers,
hydrogels
consisting
continuous
cross-linked
polymer
networks
a
large
amount
water
more
fantastic
combination
stretchability
because
their
endow
the
with
mechanical
offers
them
consecutive
ionic
transport
property.
Different
biopolymers
that
are
extracted
bioresource
intrinsic
commonly
considered
as
appropriate
candidates
for
constructing
For
example,
such
cellulose,
chitosan,
silk
fibroin
usually
chosen
promising
construct
endowing
enhanced
properties
remarkable
biocompatibility.
This
review
summarizes
recent
progress
natural
utilized
electrical
devices
series
typical
including
fibroin,
gelatin.
The
chemical
structures
physicochemical
four
demonstrated,
diverse
hydrogel
sensors
discussed
detail.
Finally,
remaining
challenges
expectations
discussed.
Advanced Functional Materials,
Journal Year:
2021,
Volume and Issue:
31(24)
Published: April 9, 2021
Abstract
Stretchable
self‐healing
supercapacitors
(SCs)
can
operate
under
extreme
deformation
and
restore
their
initial
properties
after
damage
with
considerably
improved
durability
reliability,
expanding
opportunities
in
numerous
applications,
including
smart
wearable
electronics,
bioinspired
devices,
human–machine
interactions,
etc.
It
is
challenging,
however,
to
achieve
mechanical
stretchability
self‐healability
energy
storage
technologies,
wherein
the
key
issue
lies
exploitation
of
ideal
electrode
electrolyte
materials
exceptional
ability
besides
conductivity.
Conductive
hydrogels
(CHs)
possess
unique
hierarchical
porous
structure,
high
electrical/ionic
conductivity,
broadly
tunable
physical
chemical
through
molecular
design
structure
regulation,
holding
tremendous
promise
for
stretchable
SCs.
Hence,
this
review
innovatively
constructed
a
focus
on
CH
based
electrodes
electrolytes
First,
common
synthetic
approaches
CHs
are
introduced;
then
stretching
strategies
involved
systematically
elaborated;
followed
by
an
explanation
conductive
mechanism
CHs;
focusing
CH‐based
SCs;
subsequently,
application
SCs
electronics
discussed;
finally,
conclusion
drawn
along
views
challenges
future
research
directions
regarding
field