Nano Energy, Journal Year: 2022, Volume and Issue: 103, P. 107753 - 107753
Published: Aug. 27, 2022
Language: Английский
EnergyChem, Journal Year: 2022, Volume and Issue: 5(2), P. 100091 - 100091
Published: Sept. 6, 2022
Language: Английский
Citations
102
Advanced Science, Journal Year: 2022, Volume and Issue: 10(4)
Published: Dec. 8, 2022
The conversion of biomass is a favorable alternative to the fossil energy route solve crisis and environmental pollution. As one most versatile platform compounds, 5-hydroxymethylfural (HMF) can be transformed various value-added chemicals via electrolysis combining with renewable energy. Here, recent advances in electrochemical oxidation HMF, from reaction mechanism reactor design are reviewed. First, pathway summarized systematically. Second, parameters easy ignored emphasized discussed. Then, electrocatalysts reviewed comprehensively for different products reactors introduced. Finally, future efforts on exploring mechanism, electrocatalysts, prospected. This review provides deeper understanding electrocatalyst reactor, which expected promote economical efficient industrial applications.
Language: Английский
Citations
100
Advanced Materials, Journal Year: 2022, Volume and Issue: 34(52)
Published: March 25, 2022
Abstract Electrocatalysts are the core components of many sustainable energy conversion technologies that considered most potential solution to worldwide and environmental crises. The reliability structure composition pledges electrocatalysts can achieve predictable stable performance. However, during electrochemical reaction, influenced directly by applied potential, electrolyte, adsorption/desorption reactive species, triggering structural compositional corrosion, which affects catalytic behaviors (performance degradation or enhancement) invalidates established structure–activity relationship. Therefore, it is necessary elucidate corrosion behavior mechanism formulate targeted corrosion‐resistant strategies use reconstruction synthesis techniques guide preparation efficient electrocatalysts. Herein, recent developments in electrocatalyst chemistry outlined, including mechanisms, mitigation strategies, syntheses/reconstructions based on typical materials important electrocatalytic reactions. Finally, opportunities challenges also proposed foresee possible development this field. It believed contribution will raise more awareness regarding nanomaterial beyond.
Language: Английский
Citations
96
Advanced Energy Materials, Journal Year: 2022, Volume and Issue: 12(39)
Published: Aug. 23, 2022
Abstract Single‐atom‐alloys (SAAs), as an emerging kind of materials, combine the advantages alloy and single‐atom catalysts. The full atomic utilization active sites well‐defined bonding environments in SAAs lead to superior electrocatalytic performance give a deep insight into structural–activity relationship. In this review, recent advances various electrochemical reactions are highlighted for further designing highly effective electrocatalysts. This review starts with introduction fundamental concepts several effects, which influence activities. Then preparation characterization methods on listed compared. Next, hydrogen evolution reaction, oxygen reduction alcohol/hydrogen/formic acid oxidation carbon dioxide etc. illustrated discussed detail. Finally, challenges suggestions future development energy‐conversion electrocatalysis presented.
Language: Английский
Citations
94
Nano Energy, Journal Year: 2022, Volume and Issue: 103, P. 107753 - 107753
Published: Aug. 27, 2022
Language: Английский
Citations
88