Toward Intrinsically Stretchable OLEDs with High Efficiency DOI Creative Commons
Huanyu Zhou, Hyun‐Wook Kim, Woo‐Jin Jeong

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 21, 2025

Wearable electronics require stretchable displays that can withstand large and repeated mechanical deformation without failure. Intrinsically organic light-emitting diodes (ISOLEDs) operate under DC voltage provide promising candidates for wearable display applications. However, the lack of sophisticated materials processing techniques suitable ISOLEDs results in a significant deficit efficiency state-of-the-art compared to industrial standards. The design conducting semiconducting poses challenge because trade-off relationships between stretchability properties such as conductivity charge carrier mobility. To increase meet standards, strategies overcome these trade-offs must be developed. This perspective discusses recent progress challenges designing electrodes, materials, transport potential applications ISOLEDs. It provides useful guide this field develop efficient system-level integration.

Language: Английский

Functionalization of Hydrophilic and Amphiphilic Carbon Dots with Polyethylene Glycol for Electroluminescent Devices DOI Creative Commons
Mikhail D. Miruschenko, Kseniia D. Kosolapova, Ivan A. Aleinik

et al.

Small Structures, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 17, 2025

Carbon dots (CDs) are fluorescent carbon nanomaterials that considered for applications in optoelectronics, sensorics, and biofields due to their low‐cost robust synthesis, versatile optical properties. Herein, it is demonstrated how chemical functionalization of hydrophilic or amphiphilic CDs with polyethylene glycol influences energy level structure hence the emission Functionalization results an increase quantum yield: from 30% 75% 20% 25% CDs. The estimated absolute values levels, including highest occupied molecular orbital lowest unoccupied energies, dependent on composition size Moreover, glycol‐functionalized CD can form good quality films based composite polyvinylcarbazole (PVK), together intense crucial light‐emitting diode (LED) fabrication. By studying spectral properties fabricated CD‐LEDs, shown electroluminescence (EL) originates mixed levels PVK composite, resulting shifting EL maximum blue green during several seconds LED operation. optimized CD‐LEDs show brightness up 2600 cd m −2 .

Language: Английский

Citations

1

Sustainable cross-linked poly(glycerol–co–δ–valerolactone) urethane substrates and multipurpose transparent electrodes for wearable electronics DOI Creative Commons
Pulikanti Guruprasad Reddy, Amit Barua, Timo Laukkanen

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 495, P. 153531 - 153531

Published: June 27, 2024

Substrates form the backbone of most flexible electronic devices. This study reports sustainable substrates based on a new class cross-linked poly(glycerol-co-δ-valerolactone) urethanes for and stretchable A cost-effective method is described preparing these via thermal cross-linking polymerization triol with diisocyanates glass mold. The developed display high flexibility, stretchability (∼673 %), transparency (∼90 stability (∼300 °C), degradability, essential next-generation Using synthesized polymers as substrates, we develop transparent conducting electrodes (TCEs). An innovative fabrication technique involves applying thin electrospun polyvinyl alcohol (PVA) nanofiber mat wet film leveling agent to enhance adhesion even distribution sprayed silver nanowires. Through heat pressure-based nanowelding nanowire junctions, create TCEs uniform conductivity, low sheet resistance (∼40 Ω sq−1), good (∼70 %). To demonstrate versatility TCEs, fabricated devices like capacitive sensors, curvature strain heaters. TCE sensor exhibits creep consistent performance from 5–45 % strain, maintaining signal over 200 cycles at 10 kPa. pressure responds pressures 0.5–300 kPa maximum sensitivity 2.43 kPa−1 least 2600 cycles. shows increased capacitance curvatures up 600 m−1. heater reaches 85 °C in under s 5.5 V rapidly 0–35 strain. These effectively detect human motion, serving wearable sensors heaters cold conditions, demonstrating real-life applicability.

Language: Английский

Citations

8

Advanced visual components inspired by animal eyes DOI Creative Commons
Sehui Chang, Duk‐Jo Kong, Young Min Song

et al.

Nanophotonics, Journal Year: 2024, Volume and Issue: 13(6), P. 859 - 879

Published: Feb. 29, 2024

Artificial vision systems pervade our daily lives as a foremost sensing apparatus in various digital technologies, from smartphones to autonomous cars and robotics. The broad range of applications for conventional requires facile adaptation under extreme dynamic visual environments. However, these current needs have complicated individual components high-quality image acquisition processing, which indeed leads decline efficiency the overall system. Here, we review recent advancements high-performance processing based on strategies biological eyes that execute diverse imaging functionalities sophisticated processes with simple concise ocular structures. This first covers structures functions (i.e., single-lens compound eyes), contain micro-optic nanophotonic After that, focus their inspirations optics/photonics, light-trapping filtering components, retinomorphic devices. We discuss remaining challenges notable waiting be implemented.

Language: Английский

Citations

5

Effective Strategy for High‐Performance Organic Photodetectors with Significantly Suppressed Dark Current and Improved Responsivity DOI
Shuai Zhang, Tong Liu, Jianxiao Wang

et al.

Advanced Optical Materials, Journal Year: 2024, Volume and Issue: 12(19)

Published: May 11, 2024

Abstract Organic photodetectors (OPDs) have attracted immense interest as solution‐processable optical signal‐capturing devices due to their various advantages, such adjustable response range, excellent weak light response, lightweight, flexibility, and ease of processing on diverse substrates. Low dark current density ( J d ) high responsivity R are key requirements necessary for achieving a specific detectivity D *). Here, an effective strategy preparing high‐performance OPDs with potential micro p‐i‐n structure by introducing insulating poly(aryl ether) (PAEN) into the organic photosensitive layer is reported. The PM6:PC 71 BM‐based capable significantly suppressing while increasing , which can be attributed multiple optimizations morphology charge transport caused addition PAEN. As result, value (3.63 × 10 −10 A cm −2 two orders magnitude lower than that device without PAEN (1.00 −8 at −1 V bias. Combined increased 0.376 W optimized achieves *of 3.45 13 Jones (−1 620 nm). demonstrate performance comparable commercial Si (Hamamatsu S1133), paving way direct market development this cost‐effective photodetection technology.

Language: Английский

Citations

5

Short-Wave Infrared Light-Emitting Diodes Using Colloidal CuInS2 Quantum Dots with ZnI2 Dual-Passivation DOI

Zhenyang Liu,

Chaoqi Hao,

Yejing Liu

et al.

ACS Nano, Journal Year: 2024, Volume and Issue: 18(32), P. 21523 - 21533

Published: July 26, 2024

Short-wave infrared (SWIR) light-emitting diodes (LEDs) have emerged as promising technologies for diverse applications such optical communication, biomedical imaging, surveillance, and machine vision. Colloidal quantum dots (QDs) are particularly attractive SWIR LEDs due to their solution processability, compatibility with flexible substrates, tunable absorption luminescence. However, the presence of toxic elements or precious metals in most SWIR-emitting QDs poses health, environmental, cost challenges. In this context, CuInS2 (CIS) known low toxicity, cost-effective fabrication, SWIR-light emitting capability. CIS not yet been directly utilized fabricate date, which is particle stability, inefficient charge carrier recombination, significantly blue-shifted luminescence after integrating into LED devices. To address challenges, we propose a dual-passivation strategy using ZnI2 chemical additive enhance both property plain recombination upon device implementation. The resulting CIS-QD-based exhibit stable electroluminescence (EL) peak (over 1000 nm) high EL radiance record external efficiency region. Our study represents significant step forward SWIR-QLED technology, offering pathway development high-performance, low-cost, nontoxic light sources.

Language: Английский

Citations

5

Inspiration from Visual Ecology for Advancing Multifunctional Robotic Vision Systems: Bio‐inspired Electronic Eyes and Neuromorphic Image Sensors DOI
Changsoon Choi, Gil Ju Lee, Sehui Chang

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 14, 2024

In robotics, particularly for autonomous navigation and human-robot collaboration, the significance of unconventional imaging techniques efficient data processing capabilities is paramount. The unstructured environments encountered by robots, coupled with complex missions assigned to them, present numerous challenges necessitating diverse visual functionalities, consequently, development multifunctional robotic vision systems has become indispensable. Meanwhile, rich diversity inherent in animal systems, honed over evolutionary epochs meet their survival demands across varied habitats, serves as a profound source inspirations. Here, recent advancements drawing inspiration from natural ocular structures perception mechanisms are delineated. First, unique functionalities eyes terrestrial, aerial, aquatic habitats signal mechanism humans explored. Then, designs bio-inspired electronic explored, engineered mimic key components underlying optical principles eyes. Furthermore, neuromorphic image sensors discussed, emulating functional properties synapses, neurons, retinas thereby enhancing accuracy efficiency tasks. Next, integration examples mobile robotic/biological introduced. Finally, forward-looking outlook on provided.

Language: Английский

Citations

5

Applied research and recent advances in the development of flexible sensing hydrogels from cellulose: A review DOI
Jinru Liu, Shenghua Lv, Yanlu Mu

et al.

International Journal of Biological Macromolecules, Journal Year: 2024, Volume and Issue: 281, P. 136100 - 136100

Published: Oct. 24, 2024

Language: Английский

Citations

5

Bio-inspired tunable optics and photonics: bridging the gap between nature and technology DOI Creative Commons
Do Hyeon Kim,

Jeong Jin Kim,

Duk‐Jo Kong

et al.

International Journal of Optomechatronics, Journal Year: 2024, Volume and Issue: 18(1)

Published: April 14, 2024

In the realm of optical technologies, integration nature's designs and modern engineering has paved way for groundbreaking innovations. Bio-inspired tunable optics photonics, drawing from intricate mechanisms found in biological systems, offer a new frontier adaptive efficient light management. Here, this review presents comprehensive examination principles, advancements, applications natural light-manipulation adaptation mechanisms, highlighting their translation into artificial photonic structures. Emphasizing remarkable potential bio-inspired particularly those emulating functionalities eyes skins, it explores current state devices. Our categorizes these systems two foundational mechanisms: light-adaptation, illustrating wide-ranging implications consumer electronics to next-generation technologies. This also highlights challenges prospects photonics. It emphasizes role promoting properties multifunctional devices, providing revolutionary opportunities across various sectors, including military everyday life, thus surpassing cutting-edge

Language: Английский

Citations

4

Improved Mobility–Stretchability Properties of Diketopyrrolopyrrole‐Based Conjugated Polymers with Diastereomeric Conjugation Break Spacers DOI

Pin‐Hong Chen,

Hiroya Shimizu,

Megumi Matsuda

et al.

Macromolecular Rapid Communications, Journal Year: 2024, Volume and Issue: 45(16)

Published: June 14, 2024

Stretchable conjugated polymers with conjugation break spacers (CBSs) synthesized via random terpolymerization have gained considerable attention because of their efficacy in modulating mobility and stretchability. This study incorporates a series dianhydrohexitol diastereomers isosorbide (ISB) isomannide (IMN) units into the diketopyrrolopyrrole-based backbone as CBSs. It is found that distorted CBS improves mobility-stretchability properties polymer highly coplanar backbone, whereas extended enhances those noncoplanar backbone. Additionally, different configurations ISB IMN sufficiently affect solid-state packing, aggregation capabilities, crystallographic parameters, polymer. The IMN-based exhibit highest 1.69 cm

Language: Английский

Citations

4

Advances in Flexible, Foldable, and Stretchable Quantum Dot Light-Emitting Diodes: Materials and Fabrication Strategies DOI

Taewoo Park,

Ji Su Kim,

Daewon Ko

et al.

Korean Journal of Chemical Engineering, Journal Year: 2024, Volume and Issue: 41(13), P. 3517 - 3543

Published: July 30, 2024

Language: Английский

Citations

4