A framework for automated multimodal HDX-MS analysis DOI Creative Commons
Lisa M. Tuttle, Rachel E. Klevit, Miklós Guttman

et al.

bioRxiv (Cold Spring Harbor Laboratory), Journal Year: 2025, Volume and Issue: unknown

Published: March 15, 2025

ABSTRACT We present pyHXExpress, a customizable codebase for automated high-throughput multimodal analysis of all spectra generated from HDX-MS experiments. The workflow was validated against synthetic test dataset to the fitting algorithms and confirm statistical outputs. further establish framework determination multimodality throughout protein system by rigorous evaluation fits across peptide spectra. demonstrate this approach using entire datasets detect multimodality, conformational heterogeneity, characterize dynamics small heat shock HSPB5 two disease mutants.

Language: Английский

Kingfisher: An open‐sourced web‐based platform for the analysis of hydrogen exchange mass spectrometry data DOI

Nathan McLaughlin,

Juan P. Rincon Pabon, Samantha Gies

et al.

Protein Science, Journal Year: 2025, Volume and Issue: 34(4)

Published: March 18, 2025

Abstract Hydrogen–deuterium exchange mass spectrometry (HDX‐MS) is now a critical tool in molecular biology and structural proteomics. It routinely used to probe protein conformational dynamics through well‐established experiment where amide hydrogens with deuterium atoms buffer containing D 2 O. Although there have been numerous advances the field, data analysis still poses challenges mainly due need for manual curation of lack standardized statistics accessible software. In response, we developed Kingfisher, an open‐source, user‐friendly, web‐based solution that facilitates downstream using provides advanced high‐resolution representations HDX results. Kingfisher able read directly as exported from common software packages usually takes less than minute run analysis, without download raw code or install any We foresee valuable both newcomers experts field Hydrogen Exchange Mass Spectrometry. available all users interactive web application at https://kingfisher.wustl.edu/ .

Language: Английский

Citations

0

A framework for automated multimodal HDX-MS analysis DOI Creative Commons
Lisa M. Tuttle, Rachel E. Klevit, Miklós Guttman

et al.

bioRxiv (Cold Spring Harbor Laboratory), Journal Year: 2025, Volume and Issue: unknown

Published: March 15, 2025

ABSTRACT We present pyHXExpress, a customizable codebase for automated high-throughput multimodal analysis of all spectra generated from HDX-MS experiments. The workflow was validated against synthetic test dataset to the fitting algorithms and confirm statistical outputs. further establish framework determination multimodality throughout protein system by rigorous evaluation fits across peptide spectra. demonstrate this approach using entire datasets detect multimodality, conformational heterogeneity, characterize dynamics small heat shock HSPB5 two disease mutants.

Language: Английский

Citations

0