Molecular interactions between bovine serum albumin (BSA) and trihalophenol: Insights from spectroscopic, calorimetric and molecular modeling studies DOI
Wenjie Liang, Zhenxuan Zhang, Qingyao Zhu

et al.

Spectrochimica Acta Part A Molecular and Biomolecular Spectroscopy, Journal Year: 2022, Volume and Issue: 287, P. 122054 - 122054

Published: Oct. 28, 2022

Language: Английский

Identification of Toxicity Forcing Agents from Individual Aliphatic and Aromatic Disinfection Byproducts Formed in Drinking Water: Implications and Limitations DOI
Yuru Chen,

Qiuhong Liang,

Wenjie Liang

et al.

Environmental Science & Technology, Journal Year: 2023, Volume and Issue: 57(3), P. 1366 - 1377

Published: Jan. 12, 2023

Recently, a study found that aromatic DBP fractions dominate the overall toxicity of chlorinated drinking water. However, key drivers have not been reported via comprehensive evaluation based on formation aliphatic and DBPs in In this study, occurrence 37 19 samples with different water characteristics collected Chinese megacity was explored. According to individual concentrations cytotoxicity potencies as well "TIC-Tox" method, haloacetonitriles halonitrophenols were be among measured DBPs, respectively. when are taken into consideration together, calculated present higher contribution than which is inconsistent previous study. TOX showed significant positive correlations most but no sample concentrates significantly related total suggesting current selected insufficient represent DBPs. UV

Language: Английский

Citations

33

Unraveling the Pollution and Discharge of Aminophenyl Sulfone Compounds, Sulfonamide Antibiotics, and Their Acetylation Products in Municipal Wastewater Treatment Plants DOI

Yilin Xiao,

Qing Zhang, Yingying Yang

et al.

Environmental Science & Technology, Journal Year: 2024, Volume and Issue: 58(26), P. 11695 - 11706

Published: June 15, 2024

Aminophenyl sulfone compounds (ASCs) are widely used in various fields, such as the pharmaceutical and textile industries. ASCs their primary acetylation products inevitably discharged into environment. However, high toxicity of could be released from deacetylation products. Still, occurrence ecological risks remain largely unknown. Here, we integrated all existing based on core structure, together with potential products, to establish a database covering 1105 compounds. By combining R programming, 45 ASCs, sulfonamides, were identified influent effluent 19 municipal wastewater treatment plants 4 cities China. 13 them detected for first time aquatic environment, 12 newly identified. The cumulative concentrations range 231-9.96 × 10

Language: Английский

Citations

11

Cytotoxicity of emerging halophenylacetamide disinfection byproducts in drinking water: Mechanism and prediction DOI
Shaoyang Hu, Xiangxiang Li, Falin He

et al.

Water Research, Journal Year: 2024, Volume and Issue: 256, P. 121562 - 121562

Published: April 1, 2024

Language: Английский

Citations

8

Health risk assessment via ingestion of disinfection by-products in drinking water DOI Creative Commons
Lei Wang, Zisi Fang, Xiaocong Zhou

et al.

Scientific Reports, Journal Year: 2025, Volume and Issue: 15(1)

Published: Jan. 13, 2025

Disinfection is a critical process to ensure the safety of drinking water. To curb spread various bacteria and viruses, disinfectants are extensively employed in communities, hospitals, sewage treatment plants, other settings. However, can produce disinfection by-products (DBPs) that threaten human health. Despite their importance, research systematic analyses these risks remain limited. This study monitored DBPs water across 13 districts counties Hangzhou, conducting risk assessment based on health model recommended by United States Environmental Protection Agency. Concentrations 12 ranged from 0.01 µg/L 120 µg/L, with levels 2020–2022 generally exceeding those 2018–2019. Notably, median concentrations trichloromethane peaked at 18.00 2021. Most detected higher central northern parts. spatial distribution was determined be random. The associated most were 2021 compared years. Cancer between 10− 6 4 noncarcinogenic below 1. demonstrates increased disinfectant use during may elevates concentrations.

Language: Английский

Citations

1

Strategies for mitigating chlorinated disinfection byproducts in wastewater treatment plants DOI Creative Commons
Sofía Albolafio, Alicia Marín, Ana Allende

et al.

Chemosphere, Journal Year: 2021, Volume and Issue: 288, P. 132583 - 132583

Published: Oct. 18, 2021

A case study of 15 wastewater treatment plants (WWTPs) at a full-scale was assessed for the risks disinfection byproduct (DBP) formation, mainly regulated trihalomethanes (THMs) and haloacetic acids (HAAs) chlorate as an inorganic recently in EU. Raw from large, medium/small urban areas were treated with single or combined processes (i.e., chlorine, peracetic acid (PAA) ultraviolet (UV) radiation). Sampling executed once month over seven months WWTPs twice large ones. Due to potential risk SARS-CoV-2 contaminated wastewater, several inactivation methods examined before DBP analysis. step, stability THM4 HAA9 suffered reductions, monitoring their presence only effluents after treatments. In contrast, levels remained unchanged treatment; thus both raw occurrence Results showed that residues varied greatly undetected high 42.2 mg L−1. As continuous DBPs performed, positive correlation chlorine chlorine/UV found. Changes physicochemical parameters indicated quality considerably depending on WWTPs, it influenced formation. all alone UV significantly increased THMs, HAAs, effluents. When same changed PAA PAA/UV, diminished completely. This highlights during pandemic. It also how chemical formation could be reduced by changing chlorinated technologies particularly if reclaimed water is intended agricultural irrigation minimize residues.

Language: Английский

Citations

52

Impacts of COVID-19 pandemic on the aquatic environment associated with disinfection byproducts and pharmaceuticals DOI Open Access
Zhong Zhang, Yang Zhou, Lanfang Han

et al.

The Science of The Total Environment, Journal Year: 2021, Volume and Issue: 811, P. 151409 - 151409

Published: Nov. 4, 2021

Language: Английский

Citations

48

Spatial variation of dissolved organic nitrogen in Wuhan surface waters: Correlation with the occurrence of disinfection byproducts during the COVID-19 pandemic DOI Open Access
Leyun Wang, Xian Zhang, Shanshan Chen

et al.

Water Research, Journal Year: 2021, Volume and Issue: 198, P. 117138 - 117138

Published: April 11, 2021

Language: Английский

Citations

41

Nanocomposite Polymeric Membranes for Organic Micropollutant Removal: A Critical Review DOI Creative Commons
Yichen Wu, Ming Chen, Hye-Jin Lee

et al.

ACS ES&T Engineering, Journal Year: 2022, Volume and Issue: 2(9), P. 1574 - 1598

Published: Aug. 23, 2022

The prevalence of organic micropollutants (OMPs) and their persistence in water supplies have raised serious concerns for drinking safety public health. Conventional treatment technologies, including adsorption biological treatment, are known to be insufficient treating OMPs demonstrated poor selectivity toward a wide range OMPs. Pressure-driven membrane filtration has the potential remove many detected with high as membrane's molecular weight cutoff (MWCO), surface charge, hydrophilicity can easily tailored targeted OMP's size, charge octanol-water partition coefficient (K

Language: Английский

Citations

36

Formation of disinfection by-products from microplastics, tire wear particles, and other polymer-based materials DOI
Mahyar Ghanadi, Mélanie Kah, Rai S. Kookana

et al.

Water Research, Journal Year: 2022, Volume and Issue: 230, P. 119528 - 119528

Published: Dec. 23, 2022

Language: Английский

Citations

36

Formation and Cytotoxicity of Halophenylacetamides: A New Group of Nitrogenous Aromatic Halogenated Disinfection Byproducts in Drinking Water DOI
Shaoyang Hu, Han Yeong Kaw, Lizhong Zhu

et al.

Environmental Science & Technology, Journal Year: 2022, Volume and Issue: 56(5), P. 3181 - 3192

Published: Feb. 17, 2022

Nitrogenous aromatic halogenated disinfection byproducts (DBPs) in drinking water have received considerable attention recently owing to their relatively high toxicity. In this study, a new group of nitrogenous byproducts, halophenylacetamides (HPAcAms), were successfully identified for the first time both laboratory experiments and realistic water. The formation mechanism HPAcAms during chlorination phenylalanine presence Br– I–, occurrence frequencies, concentrations authentic investigated, quantitative structure–activity relationship (QSAR) model was developed based on acquired cytotoxicity data. results demonstrated that could be formed from via electrophilic substitution, decarboxylation, hydrochloric acid elimination, hydrolysis. HPAcAm yields significantly affected by contact time, pH, chlorine dose, temperature. Nine with range 0.02–1.54 ng/L detected samples. Most tested showed higher compared dichloroacetamide, which is most abundant aliphatic haloacetamide DBP. QSAR cellular uptake efficiency polarized distributions electrons play essential roles mechanisms.

Language: Английский

Citations

35