Abstract.
This
study
reports
the
contribution
of
fire
emissions
on
ozone
(O₃)
pollution
in
Arizona
compared
to
local
and
regional
anthropogenic
emissions.
Using
WRF-Chem
modeling
system
with
different
O₃
CO
tags,
we
quantified
contributions
these
levels
during
June
2021,
a
period
when
region
was
experiencing
both
drought
conditions
extreme
heat.
Our
findings
indicate
that
background
accounted
for
about
50
%
total
O₃,
contributing
between
24
40
%.
During
peak
smoky
time
period,
fire-contributed
significant
across
Phoenix
metropolitan
area,
ranging
from
5
23
ppb
or
21
levels,
an
average
15
We
verify
tags
by
conducting
model
sensitivity
test
excluded
emissions,
which
showed
strong
agreement
spatiotemporal
pattern
due
although
magnitude
is
underestimated
factor
1.4.
further
demonstrates
wildfires
exacerbate
exceedances
over
urban
areas.
analysis
also
Yuma
are
significantly
influenced
transboundary
California
Mexico,
whereas
Phoenix's
mainly
driven
much
smaller
external
sources
period.
Consistent
previous
reports,
our
highlight
role
confounding
assessment
environments,
especially
dry
extremely
hot
summer
semi-arid/arid
regions.
Frontiers in Science,
Journal Year:
2024,
Volume and Issue:
2
Published: April 4, 2024
Global
warming
and
climate
change
have
increased
the
pollen
burden
frequency
intensity
of
wildfires,
sand
dust
storms,
thunderstorms,
heatwaves—with
concomitant
increases
in
air
pollution,
heat
stress,
flooding.
These
environmental
stressors
alter
human
exposome
trigger
complex
immune
responses.
In
parallel,
pollutants,
allergens,
other
factors
increase
risks
skin
mucosal
barrier
disruption
microbial
dysbiosis,
while
a
loss
biodiversity
reduced
exposure
to
diversity
impairs
tolerogenic
development.
The
resulting
dysregulation
is
contributing
an
immune-mediated
diseases
such
as
asthma
allergic
diseases,
autoimmune
cancer.
It
now
abundantly
clear
that
multisectoral,
multidisciplinary,
transborder
efforts
based
on
Planetary
Health
One
approaches
(which
consider
dependence
health
environment
natural
ecosystems)
are
urgently
needed
adapt
mitigate
effects
change.
Key
actions
include
reducing
emissions
improving
quality
(through
fossil
fuel
use),
providing
safe
housing
(e.g.,
weatherization),
diets
(i.e.,
diversity)
agricultural
practices,
increasing
green
spaces.
There
also
pressing
need
for
collaborative,
multidisciplinary
research
better
understand
pathophysiology
context
New
data
science
techniques,
biomarkers,
economic
models
should
be
used
measure
impact
disease,
inform
mitigation
adaptation
efforts,
evaluate
their
effectiveness.
Justice,
equity,
diversity,
inclusion
(JEDI)
considerations
integral
these
address
disparities
Thorax,
Journal Year:
2025,
Volume and Issue:
unknown, P. thorax - 222709
Published: March 31, 2025
Introduction
Ambient
formaldehyde
(HCHO)
is
globally
distributed,
posing
significant
exposure
to
vast
populations,
particularly
vulnerable
demographics
such
as
children.
Investigations
into
the
correlation
between
ambient
HCHO
and
children’s
respiratory
ailments
are
deficient.
Methods
was
retrieved
from
TROPOspheric
Monitoring
Instrument.
A
two-stage
time-series
analysis
conducted
examine
relationship
hospital
admission
of
diseases
among
198
704
children
in
Jiangsu
Province,
China,
2019
2021.
Additionally,
12
patterns
were
defined
further
discern
potential
synergistic
effects
high
temperature
combined
exposure.
Results
After
controlling
for
relevant
covariates,
our
findings
revealed
associated
with
respiratory-related
admissions.
Specifically,
we
identified
a
pronounced
effect
at
lag
3
day,
demonstrating
1.14%
increase
(95%
CI:
0.60%,
1.69%).
Subgroup
analyses
that
warm
season,
3–7
years
old
group
disadvantaged
economic
areas
showed
higher
risk.
Moreover,
found
would
trigger
elevated
risk
admission.
Notably,
specific
scenarios,
cumulative
relative
reached
up
1.051
1.025,
1.078),
highlighting
on
health
Conclusions
increased
risks
children,
could
To
have
an
in-depth
understanding
impact
critical
intervention
strategies
aimed
mitigating
pollution
regarding
adverse
impacts
under
changing
climate.
Remote Sensing of Environment,
Journal Year:
2024,
Volume and Issue:
312, P. 114321 - 114321
Published: July 24, 2024
Satellite
observations
from
instruments
such
as
the
TROPOspheric
Monitoring
Instrument
(TROPOMI)
show
significant
potential
for
monitoring
spatiotemporal
variability
of
NO2,
however
they
typically
provide
vertically
integrated
measurements
over
tropospheric
column.
In
this
study,
we
introduce
a
machine
learning
approach
entitled
'S-MESH'
(Satellite
and
ML-based
Estimation
Surface
air
quality
at
High
resolution)
that
allows
estimating
daily
surface
NO2
concentrations
Europe
1
km
spatial
resolution
based
on
eXtreme
gradient
boost
(XGBoost)
model
using
primarily
observation-based
datasets
period
2019–2021.
Spatiotemporal
used
by
include
TROPOMI
vertical
column
density,
night
light
radiance
Visible
Infrared
Imaging
Radiometer
Suite
(VIIRS),
Normalized
Difference
Vegetation
Index
Moderate
Resolution
Spectroradiometer
(MODIS),
stations
European
Environment
Agency
database
modeled
meteorological
parameters
planetary
boundary
layer
height,
wind
velocity,
temperature.
The
overall
evaluation
shows
mean
absolute
error
7.77
μg/m3,
median
bias
0.6
μg/m3
Spearman
rank
correlation
0.66.
performance
is
found
to
be
influenced
concentration
levels,
with
most
reliable
predictions
levels
10–40
<40%.
temporal
analyses
indicate
robustness
across
study
area,
better
prediction
accuracy
during
winter
months
associated
higher
concentrations.
Despite
complexity
continental
scale
XGBoost-based
fast
execution
in
providing
estimates
Europe.
Shapley
Additive
exPlanations
(SHAP)
value
analysis
highlights
density
main
source
information
deriving
concentrations,
indicating
its
studies.
SHAP
values
also
importance
anthropogenic
emission
proxy
inputs
VIIRS
lights,
complementing
detailed
patterns
variations.
Atmospheric chemistry and physics,
Journal Year:
2024,
Volume and Issue:
24(7), P. 4177 - 4192
Published: April 8, 2024
Abstract.
Narrowing
surface
ozone
disparities
between
urban
and
nonurban
areas
escalate
health
risks
in
densely
populated
zones.
A
comprehensive
understanding
of
the
impact
photochemistry
on
this
transition
remains
constrained
by
current
knowledge
aerosol
effects
availability
monitoring.
Here
we
reconstructed
spatiotemporal
gapless
air
quality
concentrations
using
a
novel
transformer
deep
learning
(DL)
framework
capable
perceiving
dynamics
to
analyze
urban–nonurban
differences.
Subsequently,
photochemical
effect
these
discrepancies
was
analyzed
elucidating
shifts
regimes
inferred
from
an
interpretable
machine
method.
The
evaluations
model
exhibited
average
out-of-sample
cross-validation
coefficient
determination
0.96,
0.92,
0.95
for
ozone,
nitrogen
dioxide,
fine
particulate
matter
(PM2.5),
respectively.
sensitivity
areas,
dominated
nitrogen-oxide-limited
(NOx-limited)
regime,
observed
shift
towards
increased
volatile
organic
compounds
(VOCs)
when
extended
areas.
third
“aerosol-inhibited”
regime
identified
Jiaodong
Peninsula,
where
uptake
hydroperoxyl
radicals
onto
aerosols
suppressed
production
under
low
NOx
levels
during
summertime.
reduction
PM2.5
could
increase
VOCs,
necessitating
more
stringent
VOC
emission
abatement
mitigation.
In
2020,
Shandong
surpassed
those
primarily
due
pronounced
decrease
latter
resulting
stronger
suppression
less
PM2.5.
This
case
study
demonstrates
critical
need
advanced
spatially
resolved
models
analysis
tackling
pollution
challenges.
Geophysical Research Letters,
Journal Year:
2024,
Volume and Issue:
51(15)
Published: Aug. 6, 2024
Abstract
Quantifying
the
variable
impacts
of
wildfire
smoke
on
ozone
air
quality
is
challenging.
Here
we
use
airborne
measurements
from
2018
Western
Wildfire
Experiment
for
Cloud
Chemistry,
Aerosol
Absorption,
and
Nitrogen
(WE‐CAN)
to
parameterize
emissions
reactive
nitrogen
(NO
y
)
wildfires
into
peroxyacetyl
nitrate
(PAN;
37%),
NO
3
−
(27%),
(36%)
in
a
global
chemistry‐climate
model
with
13
km
spatial
resolution
over
contiguous
US.
The
partitioning,
compared
emitting
all
as
NO,
reduces
bias
near‐fire
plumes
sampled
by
aircraft
enhances
downwind
5–10
ppbv
when
Canadian
travel
Washington,
Utah,
Colorado,
Texas.
Using
multi‐platform
observations,
identify
smoke‐influenced
days
daily
maximum
8‐hr
average
(MDA8)
70–88
Kennewick,
Salt
Lake
City,
Denver
Dallas.
On
these
days,
enhanced
MDA8
5–25
ppbv,
through
produced
remotely
during
plume
transport
locally
via
interactions
urban
emissions.
npj Climate and Atmospheric Science,
Journal Year:
2025,
Volume and Issue:
8(1)
Published: Jan. 10, 2025
Climate
change
poses
direct
and
indirect
threats
to
public
health,
including
exacerbating
air
pollution.
However,
the
influence
of
rising
temperature
on
quality
remains
highly
uncertain
in
United
States,
particularly
under
rapid
reduction
anthropogenic
emissions.
Here,
we
examined
sensitivity
surface-level
fine
particulate
matter
(PM2.5)
ozone
(O3)
summer
anomalies
contiguous
US
as
well
their
decadal
changes
using
high-resolution
datasets
generated
by
machine
learning.
Our
findings
demonstrate
that
eastern
US,
stringent
emission
control
strategies
have
significantly
reduced
positive
responses
PM2.5
O3
temperature,
thereby
lowering
population
exposure
associated
with
warming-induced
deterioration.
In
contrast,
western
became
more
sensitive
highlighting
urgent
need
manage
mitigate
impact
worsening
wildfires.
results
important
implications
for
management
risk
assessments
future
climate
change.
Abstract.
The
TROPOspheric
Monitoring
Instrument
(TROPOMI),
onboard
the
Sentinel-5
Precursor
(S5P)
satellite
launched
in
October
2017,
is
dedicated
to
monitoring
atmospheric
composition
associated
with
air
quality
and
climate
change.
This
paper
presents
global
retrieval
of
TROPOMI
tropospheric
formaldehyde
(HCHO)
nitrogen
dioxide
(NO2)vertical
columns
using
an
updated
version
Peking
University
OMI
NO2
(POMINO)
algorithm,
which
focuses
on
improving
calculation
mass
factors
(AMFs).
algorithm
features
explicit
corrections
for
surface
reflectance
anisotropy
aerosol
optical
effects,
uses
daily
high-resolution
(0.25°×0.25°)
a
priori
HCHO
profiles
from
Global
Earth
Observing
System
Composition
Forecast
(GEOS-CF)
dataset.
For
cloud
correction,
consistent
approach
used
both
retrievals,
where
(1)
fraction
re-calculated
at
440
nm
same
ancillary
parameters
as
those
AMF
calculation,
(2)
top
pressure
taken
operational
FRESCO-S
product.
comparison
between
POMINO
reprocessed
(RPRO)
products
April,
July,
2021
January
2022
exhibits
high
spatial
agreement,
but
RPRO
NO2
columns
are
lower
by
10
%
20
over
polluted
regions.
Sensitivity
tests
show
that
differences
mainly
caused
different
correction
methods
(implicit
versus
explicit),
prior
information
vertical
profile
shapes
background
corrections;
while
discrepancies
result
corrections,
reflectances
well
their
non-linear
interactions.
With
structural
uncertainty
due
within
±
%,
height
differences.
Validation
against
ground-based
measurements
Multi-Axis
Differential
Optical
Absorption
Spectroscopy
(MAX-DOAS)
observations
Pandonia
Network
(PGN)
shows
2022,
retrievals
present
comparable
day-to-day
correlation
reduced
bias
compared
(HCHO:
R
=
0.62,
NMB
=
−30.8
0.68,
−35.0
%;
NO2:
0.84,
−9.5
0.85,
−19.4
%).
An
improved
agreement
HCHO/NO2
ratio
(FNR)
PGN
based
also
found
(R
0.83,
−18.4
0.82,
−24.1
Our
provides
useful
source
particularly
studies
combining
NO2.
Abstract.
The
TROPOspheric
Monitoring
Instrument
(TROPOMI),
onboard
the
Sentinel-5
Precursor
(S5P)
satellite
launched
in
October
2017,
is
dedicated
to
monitoring
atmospheric
composition
associated
with
air
quality
and
climate
change.
This
paper
presents
global
retrieval
of
TROPOMI
tropospheric
formaldehyde
(HCHO)
nitrogen
dioxide
(NO2)vertical
columns
using
an
updated
version
Peking
University
OMI
NO2
(POMINO)
algorithm,
which
focuses
on
improving
calculation
mass
factors
(AMFs).
algorithm
features
explicit
corrections
for
surface
reflectance
anisotropy
aerosol
optical
effects,
uses
daily
high-resolution
(0.25°×0.25°)
a
priori
HCHO
profiles
from
Global
Earth
Observing
System
Composition
Forecast
(GEOS-CF)
dataset.
For
cloud
correction,
consistent
approach
used
both
retrievals,
where
(1)
fraction
re-calculated
at
440
nm
same
ancillary
parameters
as
those
AMF
calculation,
(2)
top
pressure
taken
operational
FRESCO-S
product.
comparison
between
POMINO
reprocessed
(RPRO)
products
April,
July,
2021
January
2022
exhibits
high
spatial
agreement,
but
RPRO
NO2
columns
are
lower
by
10
%
20
over
polluted
regions.
Sensitivity
tests
show
that
differences
mainly
caused
different
correction
methods
(implicit
versus
explicit),
prior
information
vertical
profile
shapes
background
corrections;
while
discrepancies
result
corrections,
reflectances
well
their
non-linear
interactions.
With
structural
uncertainty
due
within
±
%,
height
differences.
Validation
against
ground-based
measurements
Multi-Axis
Differential
Optical
Absorption
Spectroscopy
(MAX-DOAS)
observations
Pandonia
Network
(PGN)
shows
2022,
retrievals
present
comparable
day-to-day
correlation
reduced
bias
compared
(HCHO:
R
=
0.62,
NMB
=
−30.8
0.68,
−35.0
%;
NO2:
0.84,
−9.5
0.85,
−19.4
%).
An
improved
agreement
HCHO/NO2
ratio
(FNR)
PGN
based
also
found
(R
0.83,
−18.4
0.82,
−24.1
Our
provides
useful
source
particularly
studies
combining
NO2.