From Ab Initio to Instrumentation: A Field Guide to Characterizing Multivalent Liquid Electrolytes DOI
Glenn Pastel, Travis P. Pollard,

Oleg Borodin

et al.

Chemical Reviews, Journal Year: 2025, Volume and Issue: unknown

Published: March 10, 2025

In this field guide, we outline empirical and theory-based approaches to characterize the fundamental properties of liquid multivalent-ion battery electrolytes, including (i) structure chemistry, (ii) transport, (iii) electrochemical properties. When detailed molecular-scale understanding multivalent electrolyte behavior is insufficient use examples from well-studied lithium-ion electrolytes. recognition that coupling techniques highly effective, but often nontrivial, also highlight recent characterization efforts uncover a more comprehensive nuanced underlying structures, processes, reactions drive performance system-level behavior. We hope insights these discussions will guide design future studies, accelerate development next-generation batteries through modeling with experiments, help avoid pitfalls ensure reproducibility results.

Language: Английский

From Ab Initio to Instrumentation: A Field Guide to Characterizing Multivalent Liquid Electrolytes DOI
Glenn Pastel, Travis P. Pollard,

Oleg Borodin

et al.

Chemical Reviews, Journal Year: 2025, Volume and Issue: unknown

Published: March 10, 2025

In this field guide, we outline empirical and theory-based approaches to characterize the fundamental properties of liquid multivalent-ion battery electrolytes, including (i) structure chemistry, (ii) transport, (iii) electrochemical properties. When detailed molecular-scale understanding multivalent electrolyte behavior is insufficient use examples from well-studied lithium-ion electrolytes. recognition that coupling techniques highly effective, but often nontrivial, also highlight recent characterization efforts uncover a more comprehensive nuanced underlying structures, processes, reactions drive performance system-level behavior. We hope insights these discussions will guide design future studies, accelerate development next-generation batteries through modeling with experiments, help avoid pitfalls ensure reproducibility results.

Language: Английский

Citations

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