Exploring reaction dynamics involving post-transition state bifurcations based on quantum mechanical ambimodal transition states DOI
Ching Ching Lam, K. N. Houk

Pure and Applied Chemistry, Journal Year: 2025, Volume and Issue: unknown

Published: April 24, 2025

Abstract Computational methods for predicting product ratios in dynamically controlled reactions with shallow intermediates or bifurcating pathways after an ambimodal transition state are reviewed and benchmarked. The range of includes molecular dynamics simulations, machine learning-based models recent advancements correlational methods, all which rely on quantum mechanical computations. Together, these approaches form a computational toolbox that enhances the efficiency effectiveness exploring reaction selectivity influenced by dynamic effects.

Language: Английский

Exploring reaction dynamics involving post-transition state bifurcations based on quantum mechanical ambimodal transition states DOI
Ching Ching Lam, K. N. Houk

Pure and Applied Chemistry, Journal Year: 2025, Volume and Issue: unknown

Published: April 24, 2025

Abstract Computational methods for predicting product ratios in dynamically controlled reactions with shallow intermediates or bifurcating pathways after an ambimodal transition state are reviewed and benchmarked. The range of includes molecular dynamics simulations, machine learning-based models recent advancements correlational methods, all which rely on quantum mechanical computations. Together, these approaches form a computational toolbox that enhances the efficiency effectiveness exploring reaction selectivity influenced by dynamic effects.

Language: Английский

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