Thgraphene with High Polysulfide Anchoring Ability and Catalytic Performance for Advanced Na–S Batteries: A First-Principles Study DOI
Jiajun Wang, Xintao Chai,

Chen Sun

et al.

Langmuir, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 11, 2024

The sodium-sulfur (Na-S) batteries, with advantages such as high energy density, specific capacity, and low cost, have attracted significant attention in the field of rechargeable batteries recent years. However, their practical application still faces many challenges. In this study, we employ first-principles calculations to investigate performance a 2D carbon allotrope, thgraphene, an anchoring material Na-S batteries. Our studies reveal that thgraphene possesses modest adsorption strength (0.70-1.75 eV) toward S

Language: Английский

Transition Metal-Doped 2D GaN as Single-Atom Electrocatalysts for Lithium–Sulfur Batteries: Insights from First-Principles Calculations DOI
Keat Hoe Yeoh, Yee Hui Robin Chang, Khian‐Hooi Chew

et al.

ACS Applied Electronic Materials, Journal Year: 2025, Volume and Issue: unknown

Published: April 11, 2025

Language: Английский

Citations

0
Design Strategies Based on Electronic Interactions for Effective Catalysts in Lithium‐Sulfur Batteries DOI Creative Commons
Donghyeok Son, Cheol‐Young Park, Jinuk Kim

et al.

Angewandte Chemie International Edition, Journal Year: 2025, Volume and Issue: unknown

Published: April 30, 2025

Abstract Lithium–sulfur batteries (LSBs) are considered promising next‐generation due to their high energy density (>500 W h kg −1 ). However, LSBs exhibit an unsatisfactory (<400 ) and cycle life (<300 cycles) because of the shuttle effect caused by soluble lithium polysulfide (LiPS) intermediates sluggish conversion reaction kinetics insulating sulfur (S 8 sulfide (Li 2 S). Although various types catalysts, including metal‐based compounds single‐atom have been reported address these issues, most catalysts exhibited limited catalytic activity under practical lean electrolyte conditions (<5 µL mg A comprehensive understanding synthetic strategy mechanism is essential for design, but electronic effects LiPS more important. Furthermore, design not well understood. In this review, we introduce mechanisms in discuss catalyst strategies terms on interactions between reactants with a primary focus heterogeneous systems. We additionally consider how property homogeneous systems, particularly redox mediators, affects behavior propose future research directions development LSBs.

Language: Английский

Citations

0
The synergistic effect of heteronuclear diatom enhances the catalytic and adsorption ability of lithium-sulfur batteries DOI
Yue Zhao, Yan Xi, Yifan Zhu

et al.

Applied Surface Science, Journal Year: 2025, Volume and Issue: unknown, P. 163600 - 163600

Published: May 1, 2025

Language: Английский

Citations

0
Theoretical evaluation of monolayer MA2Z4 (M = Ti, Zr, or Hf; A = Si or Ge; and Z = P or As) family as promising candidates for lithium–sulfur batteries DOI
Jiguang Du,

Xuying Zhou,

Xiujuan Cheng

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: unknown

Published: Sept. 1, 2024

Language: Английский

Citations

3
Thgraphene with High Polysulfide Anchoring Ability and Catalytic Performance for Advanced Na–S Batteries: A First-Principles Study DOI
Jiajun Wang, Xintao Chai,

Chen Sun

et al.

Langmuir, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 11, 2024

The sodium-sulfur (Na-S) batteries, with advantages such as high energy density, specific capacity, and low cost, have attracted significant attention in the field of rechargeable batteries recent years. However, their practical application still faces many challenges. In this study, we employ first-principles calculations to investigate performance a 2D carbon allotrope, thgraphene, an anchoring material Na-S batteries. Our studies reveal that thgraphene possesses modest adsorption strength (0.70-1.75 eV) toward S

Language: Английский

Citations

0