Expanding Chemical Space in the Synthesis of Gold Bipyramids DOI Creative Commons
Ana Sánchez‐Iglesias, Marek Grzelczak

Published: July 26, 2024

Gold bipyramids (AuBPs), despite having superior properties compared to their spectroscopically similar counterparts, gold nanorods, have found comparatively limited applications. This discrepancy is primarily due the lack of protocols tailor dimensions. Typically, concentration Au seeds virtually sole factor that determines aspect ratio and thus, optical AuBPs. As a result, varying volumes AuBPs while incurring minimal changes spectra remains synthetically non-trivial task. Here, we expand chemical space in seeded growth AuBPs, by exploiting interplay between bromide, silver ions, seed for tuning final dimensions Specifically, achieved 6-fold change maintaining fixed plasmon band position. Further overgrowth as-prepared broadens realizable without compromising quality initial morphology. Overall, our results toolbox wet-chemistry synthesis anisotropic nanoparticles, which relevant health, colorimetric sensors, energy

Language: Английский

DYNAMICS OF ABSORPTION PEAKS IN PLASMONIC NANOSTRUCTURES DOI
Imtiaz Ahmad, Sajjad Ahmad Khan, Rahim Jan

et al.

Colloids and Surfaces A Physicochemical and Engineering Aspects, Journal Year: 2025, Volume and Issue: 709, P. 136115 - 136115

Published: Jan. 5, 2025

Language: Английский

Citations

0

Bacterial synthesis of anisotropic gold nanoparticles DOI Creative Commons
Islam M. Ahmady, Javad B. M. Parambath, Elsiddig A. E. Elsheikh

et al.

Applied Microbiology and Biotechnology, Journal Year: 2025, Volume and Issue: 109(1)

Published: March 10, 2025

Abstract Pseudomonas aeruginosa was used to synthesize anisotropic gold nanoparticles from the unusually reducible aryldiazonium (III) salt of chemical formula [HOOC-4-C 6 H 4 N≡N]AuCl (abbreviated as DS-AuCl ). We investigated effect bacterial cell density, temperature, and pH on AuNP synthesis. The density 6.0 × 10 8 CFU/mL successfully reduced 0.5 mM AuNPs after incubation at 37 °C (24 h), 42 25 (48 h). Transmission electron microscopy (TEM) images revealed formation spherical, triangle, star, hexagon, truncated triangular morphologies for synthesized using P. bacteria. average size h) 39.0 ± 9.1 nm, 26.0 8.1 36.7 7.7 respectively. 3.7, 7.0, 12.7 14.7 3.8 7.3 2.5 respectively, with decreasing a 12.7. reduction confirmed X-ray photoelectron spectroscopy (XPS). significant peaks C1s, Au4f doublet, N1s, O1s are centered 285, 84–88, 400, 532 eV. ability inactivated bacteria (autoclave-dead mechanically lysed bacteria), peptidoglycan, lipopolysaccharides reduce also investigated. Anisotropic were peptidoglycan but not lipopolysaccharides. demonstrated biocompatibility human RBCs safe, no antibacterial activities against Escherichia coli Staphylococcus aureus . This is first report demonstrating synthesis gold(III) salts These promising candidates exploring potential applications in nanomedicine drug delivery. Key points • Dead residues AuNPs. hemocompatible. Graphical

Language: Английский

Citations

0

Growth of NIR-II-Responsive Gold Nanobipyramids with Improved Yield and a Study of Their Application in Cancer Therapy DOI
Yujie Ma, Liang‐Bin Xiong, Wenbin Qiu

et al.

Langmuir, Journal Year: 2025, Volume and Issue: unknown

Published: April 23, 2025

Gold nanobipyramids (Au NBPs), as a novel and emerging plasmonic nanomaterial, have shown larger local electric field enhancements, optical cross-sections, higher refractive index sensitivity compared to other nanoparticles. Besides, their localized surface plasmon resonance (LSPR) absorption can be tailored cover the entire NIR-II light region, which is crucial for clinical cancer treatment. However, strategies synthesize Au NBPs with an response still several disadvantages, such tedious procedures use of hazardous chemical substances. In this work, we used seed-mediated growth method explored new high-yield response, especially in region above 1030 nm, by regulating conditions during seed growth. The yield at 1060 nm has been improved 5-fold 6-fold previous methods when 230 μL sodium citrate or controlled temperature 45 °C were solution containing 125 NaBH4. influence mechanism these factors on detail. Furthermore, photodynamic photothermal behaviors LSPR investigated, results indicate that great potential therapy. proven induce immunogenic cell death (ICD), indicating immunotherapy. This work may provide idea synthesis biomedical applications response.

Language: Английский

Citations

0

Isomerization of inorganic nanomaterials DOI
Reilly P. Lynch, Richard D. Robinson

MRS Communications, Journal Year: 2025, Volume and Issue: unknown

Published: May 15, 2025

Language: Английский

Citations

0

Expanding Chemical Space in the Synthesis of Gold Bipyramids DOI Creative Commons
Ana Sánchez‐Iglesias, Marek Grzelczak

Small, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 9, 2024

Gold bipyramids (AuBPs), despite having superior properties compared to their spectroscopically similar counterparts, gold nanorods, have found comparatively limited applications. This discrepancy is primarily due the lack of protocols tailor dimensions. Typically, concentration Au seeds virtually sole factor that determines aspect ratio and thus, optical AuBPs. As a result, varying volumes AuBPs while incurring minimal changes spectra remains synthetically non-trivial task. Here, chemical space in seeded growth AuBPs, expanded by exploiting interplay between bromide, silver ions, seed for tuning final dimensions Specifically, 6 fold change achieved maintaining fixed plasmon band position. Further overgrowth as-prepared broadens realizable without compromising quality initial morphology. Overall, results expand toolbox wet-chemistry synthesis anisotropic nanoparticles, which relevant health, colorimetric sensors, energy

Language: Английский

Citations

2

Expanding Chemical Space in the Synthesis of Gold Bipyramids DOI Creative Commons
Ana Sánchez‐Iglesias, Marek Grzelczak

Published: July 26, 2024

Gold bipyramids (AuBPs), despite having superior properties compared to their spectroscopically similar counterparts, gold nanorods, have found comparatively limited applications. This discrepancy is primarily due the lack of protocols tailor dimensions. Typically, concentration Au seeds virtually sole factor that determines aspect ratio and thus, optical AuBPs. As a result, varying volumes AuBPs while incurring minimal changes spectra remains synthetically non-trivial task. Here, we expand chemical space in seeded growth AuBPs, by exploiting interplay between bromide, silver ions, seed for tuning final dimensions Specifically, achieved 6-fold change maintaining fixed plasmon band position. Further overgrowth as-prepared broadens realizable without compromising quality initial morphology. Overall, our results toolbox wet-chemistry synthesis anisotropic nanoparticles, which relevant health, colorimetric sensors, energy

Language: Английский

Citations

1