Springer proceedings in physics, Journal Year: 2024, Volume and Issue: unknown, P. 138 - 142
Published: Jan. 1, 2024
Language: Английский
The Innovation, Journal Year: 2025, Volume and Issue: 6(1), P. 100754 - 100754
Published: Jan. 1, 2025
Heterogeneous catalysis at the metal surface generally involves transport of molecules through interfacial water layer to access surface, which is a rate-determining step nanoscale. In this study, taking oxygen reduction reaction on electrode in aqueous solution as an example, using accurate molecular dynamic simulations, we propose novel long-range regulation strategy midinfrared stimulation (MIRS) with frequency approximately 1,000 cm-1 applied nonthermally induce structural transition from ordered disordered state, facilitating surfaces room temperature and increasing activity 50-fold. Impressively, theoretical prediction confirmed by experimental observation significant discharge voltage increase zinc-air batteries under MIRS. This MIRS approach can be seamlessly integrated into existing strategies, offering new for accelerating heterogeneous reactions gas sensing within system.
Language: Английский
Citations
2
Carbon, Journal Year: 2024, Volume and Issue: 228, P. 119402 - 119402
Published: June 28, 2024
Language: Английский
Citations
5
Chemical Society Reviews, Journal Year: 2024, Volume and Issue: unknown
Published: Dec. 19, 2024
This review outlines recent advances in field-regulated catalysis and reveals the key role of dipole manipulation by electric/magnetic/electromagnetic fields.
Language: Английский
Citations
5
The Journal of Physical Chemistry Letters, Journal Year: 2024, Volume and Issue: 15(36), P. 9136 - 9143
Published: Aug. 29, 2024
Spatial orderliness, which is the orderly structure of molecules, differs significantly between interfacial water and bulk water. Understanding this property essential for various applications in both natural engineered environments. However, subnanometer thickness presents challenges direct rapid characterization its structural orderliness. Herein, through molecular dynamics simulations infrared spectral analysis a graphene slit pore, we reveal hyperbolic tangent relationship ordering O–H stretching information spectrum. Specifically, symmetric dominated highly ordered structure, while transition to asymmetric corresponded an increase degree disorder. Thus, behavior could serve as useful quick assessment orderliness This work provided insights into water's unique network identified vibrations' key role order, providing insight fields such nanotechnology, biology, material science.
Language: Английский
Citations
4
Research, Journal Year: 2025, Volume and Issue: 8
Published: Jan. 1, 2025
The study of many phenomena in the terahertz (THz) frequency spectral range has emerged as a promising playground modern science and technology, with extensive applications high-speed communication, imaging, sensing, biosensing. Many THz metamaterial designs explore quantum physics embedded into classical framework exhibiting various unexpected behaviors. For spatial waves, effects inspired by include electromagnetically induced transparency (EIT), Fano resonance, bound states continuum (BICs), exceptional points (EPs) non-Hermitian systems. They facilitate realization functional metadevices applications. on-chip physics-inspired topological metamaterials, photonic analogs insulators, can ensure robust, low-loss propagation suppressed backscattering. These trends open new pathways for data transmission integrated circuits, being crucial upcoming 6G 7G wireless communication technologies. Here, we summarize underlying principles metamaterials highlight latest advances their application band, encompassing both metadevice realizations.
Language: Английский
Citations
0
Journal of Applied Physics, Journal Year: 2025, Volume and Issue: 137(10)
Published: March 10, 2025
The heating effect of infrared pulses with varying frequencies on heavy water solutions different concentrations was investigated using non-equilibrium molecular dynamics simulations. Numerical calculations indicate that when the pulse are 39 and 72 THz, excite molecules, while temperature light molecules remains unchanged. At 53 99 molecules. Additionally, in far region (1–20 THz), both simultaneously, albeit a significantly reduced energy absorption efficiency. We also conducted comparative analysis efficiency under three distinct modes: Vibrational excitation, rotational microwave heating. results reveal vibrational excitation is seven times This conclusion holds great potential for practical applications.
Language: Английский
Citations
0
Spectrochimica Acta Part A Molecular and Biomolecular Spectroscopy, Journal Year: 2025, Volume and Issue: unknown, P. 126039 - 126039
Published: March 1, 2025
Language: Английский
Citations
0
ACS Nano, Journal Year: 2025, Volume and Issue: unknown
Published: April 3, 2025
Regulation of liquid adhesion on functional surfaces has attracted increasing attention due to its significant implications for fundamental research in manipulation and a wide array applications. Inspired by the slippery peristomes Nepenthes pitcher plants, concept with regulatable under external stimuli was proposed demonstrated. This review concentrates advancements regulation these bioinspired surfaces. Initially, we provide concise introduction basic theory design criteria stable Following this, summarize characterization methods influence factors We then categorize smart modes into four key aspects: modulating lubricant's phase, thickness, structure, interactions between lubricant repellent liquid. Additionally, systematically emphasize multibehavioral strategies, such as movement, merging, splitting, bouncing, rotating, along emerging applications surfaces, including pipetting devices, fog collection, microreactors, biochips, nanogenerators. Finally, discuss remaining challenges future perspectives regulating potential
Language: Английский
Citations
0
Communications Chemistry, Journal Year: 2025, Volume and Issue: 8(1)
Published: April 3, 2025
Ion channels are essential for various physiological processes, and their defects associated with many diseases. Previous research has revealed that a Terahertz electromagnetic field can alter the channel conductance by affecting motion of chemical groups ion channels, hence regulate electric signals neurons. In this study, we conducted molecular dynamics simulations to systematically investigate effects terahertz fields on permeation voltage-gated potassium sodium particularly focusing bound ions in selectivity filters have not been extensively studied previously. Our results identified multiple new characteristic frequencies showed 1.4, 2.2, or 2.9 THz increases permeability Kv1.2, 2.5 48.6 Nav1.5. Such specific directions field, which determined intrinsic oscillation motions permeating filter certain channels. The amplitude positively correlates change permeation. This study demonstrates specifically conductances mechanisms, may carry great potential biomedical applications.
Language: Английский
Citations
0
Journal of Applied Polymer Science, Journal Year: 2025, Volume and Issue: unknown
Published: April 28, 2025
ABSTRACT Polymer tribopair materials (such as UHMWPE) are widely used in complex environments like dry friction and pure water lubrication. However, with the rapid development of electromagnetic technology, how electric fields influence tribological performance UHMWPE underlying mechanisms remain unclear. Understanding this mechanism is crucial for enhancing application potential polymer specialized working conditions. This study uses DFT MD to investigate effects field parameters (intensity direction) on Fe/UHMWPE tribopairs under lubrication The results show that, conditions, field's effect minimal due lack polar groups. Under parallel range −0.5 −0.2 V/Å significantly increase average forces, while vertical have little effect. calculations that X‐ Y‐axis reduce LUMO energy molecules, Z‐axis Δ E gap dipole moment. provides guidance optimizing recommends using fluctuations extend service life materials.
Language: Английский
Citations
0