Nanomaterials for spin-based quantum information DOI
Pengbo Ding, Dezhang Chen, Pui Kei Ko

et al.

Nanoscale, Journal Year: 2024, Volume and Issue: 17(3), P. 1148 - 1170

Published: Nov. 15, 2024

Quantum information science has garnered significant attention due to its potential in solving problems that are beyond the capabilities of classical computations based on integrated circuits. At heart quantum is bit or qubit, which used carry information. Achieving large-scale and high-fidelity bits requires optimization materials with trap-free characteristics long coherence times. Nanomaterials have emerged as promising candidates for building qubits their inherent confinement effect, enabling manipulation addressing individual spins within nanostructures. In this comprehensive review, we focus nanomaterials, including 0D dots, 1D nanotubes nanowires, 2D nanoplatelets nanolayers. Our review aims bridge gap between nanotechnology science, a particular emphasis material aspects such selection, properties, synthesis. By providing insights into these areas, contribute understanding advancement nanomaterial-based science.

Language: Английский

Intense Circular Dichroism and Spin Selectivity in AgBiS2 Nanocrystals by Chiral Ligand Exchange DOI Creative Commons
Pengbo Ding, Dezhang Chen, Mohsen Tamtaji

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 11, 2024

Abstract Chiral semiconducting nanomaterials offer many potential applications in photodetection, light emission, quantum information, and so on. However, it is difficult to achieve a strong circular dichroism (CD) signal nanocrystals (NCs) due the complexity of chiral ligand surface engineering multiple, uncertain mechanisms chiroptical behavior. Here, exchange strategy with cysteine on ternary metal chalcogenide AgBiS 2 NCs developed, strong, long‐lasting CD near‐UV region achieved. By carefully optimizing concentration, peaks are observed at 260 320 nm, respectively, giving insight into different binding influencing NCs. Using density‐functional theory, large degree crystal distortion by bidentate mode chelation, efficient ligand‐NC electron transfer, synergistically resulting strongest (g‐factor over 10 −2 ) ligand‐exchanged semiconductor date, demonstrated. To demonstrate effective properties these NCs, spin‐filter device 86% efficiency fabricated. This work represents considerable leap field points toward their future applications.

Language: Английский

Citations

3
Assessment of Interface Passivation in AgBiS2 Q-dot Sensitized Solar Cell on the carrier transport and recombination DOI

Dimuthumal Rajakaruna,

Hongyi Tan, Chang-Feng Yan

et al.

Electrochimica Acta, Journal Year: 2025, Volume and Issue: unknown, P. 146173 - 146173

Published: April 1, 2025

Language: Английский

Citations

0
Nanomaterials for spin-based quantum information DOI
Pengbo Ding, Dezhang Chen, Pui Kei Ko

et al.

Nanoscale, Journal Year: 2024, Volume and Issue: 17(3), P. 1148 - 1170

Published: Nov. 15, 2024

Quantum information science has garnered significant attention due to its potential in solving problems that are beyond the capabilities of classical computations based on integrated circuits. At heart quantum is bit or qubit, which used carry information. Achieving large-scale and high-fidelity bits requires optimization materials with trap-free characteristics long coherence times. Nanomaterials have emerged as promising candidates for building qubits their inherent confinement effect, enabling manipulation addressing individual spins within nanostructures. In this comprehensive review, we focus nanomaterials, including 0D dots, 1D nanotubes nanowires, 2D nanoplatelets nanolayers. Our review aims bridge gap between nanotechnology science, a particular emphasis material aspects such selection, properties, synthesis. By providing insights into these areas, contribute understanding advancement nanomaterial-based science.

Language: Английский

Citations

1