Hydrogen Bonds Reinforced Ionogels with High Sensitivity and Stable Autonomous Adhesion as Versatile Ionic Skins DOI

Shuquan Zheng,

Xuelian Chen, Kaixiang Shen

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(3), P. 4035 - 4044

Published: Jan. 10, 2024

Flexible wearable sensors have demonstrated enormous potential in various fields such as human health monitoring, soft robotics, and motion detection. Among them, based on ionogels garnered significant attention due to their wide range of applications. However, the fabrication with high sensitivity stable autonomous adhesion remains a challenge, thereby limiting Herein, we present an advanced ionogel (PACG-MBAA) exceptional performances multiple hydrogen bonds, which is fabricated through one-step radical polymerization N-acryloylglycine (ACG) 1-ethyl-3-methylimidazolium ethyl sulfate (EMIES) presence N,N′-methylenebis(acrylamide) (MBAA). Compared (PAA-MBAA) formed by acrylic acid (AA) EMIES, resulting exhibits tunable mechanical strength (35–130 kPa) Young's modulus comparable skin (60–70 owing bonds formation. Importantly, they demonstrate substrates good self-healing capabilities. Furthermore, ionogel-based sensor shows (with gauge factor up 6.16 tensile 300–700%), enabling detection both gross subtle movements daily activities. By integration International Morse code, enables encryption, decryption, transmission information, thus expanding its application prospects.

Language: Английский

Conductive polymer based hydrogels and their application in wearable sensors: a review DOI Creative Commons
Dong Liu,

Chenxi Huyan,

Zibi Wang

et al.

Materials Horizons, Journal Year: 2023, Volume and Issue: 10(8), P. 2800 - 2823

Published: Jan. 1, 2023

Hydrogels have been attracting increasing attention for application in wearable electronics, due to their intrinsic biomimetic features, highly tunable chemical-physical properties (mechanical, electrical, etc.), and excellent biocompatibility. Among many proposed varieties of hydrogels, conductive polymer-based hydrogels (CPHs) emerged as a promising candidate future sensor designs, with capability realizing desired features using different tuning strategies ranging from molecular design (with low length scale 10-10 m) micro-structural configuration (up 10-2 m). However, considerable challenges remain be overcome, such the limited strain sensing range mechanical strength, signal loss/instability caused by swelling/deswelling, significant hysteresis signals, de-hydration induced malfunctions, surface/interfacial failure during manufacturing/processing. This review aims offer targeted scan recent advancements CPH based technology, establishment dedicated structure-property relationships lab advanced manufacturing routes potential scale-up production. The CPHs sensors is also explored, suggested new research avenues prospects included.

Language: Английский

Citations

126

3D printing of polymer composites to fabricate wearable sensors: A comprehensive review DOI Creative Commons
Amr Osman, Jian Lü

Materials Science and Engineering R Reports, Journal Year: 2023, Volume and Issue: 154, P. 100734 - 100734

Published: May 15, 2023

The application of wearable sensors in domains related to healthcare systems, human motion detection, robotics, and human–machine interactions has attracted significant attention. Because these applications require stretchable, flexible, non-invasive materials, polymer composites are now at the forefront research aimed preparing innovative sensors. Three-dimensional (3D) printing techniques can be used obtain highly customised scalable fabricate sensors, which is a challenging task for conventional fabrication techniques. This review provides insights into prospects commonly conductive nanomaterials 3D prepare devices. Subsequently, progress, sensing mechanisms, performance 3D-printed such as strain, pressure, temperature, humidity discussed. In addition, novel multifunctional multi-directional, multi-modal, self-healable, self-powered, situ printed, ultrasonic highlighted. challenges future trends further development clarified.

Language: Английский

Citations

79

Reversible Wet‐Adhesive and Self‐Healing Conductive Composite Elastomer of Liquid Metal DOI

Danfeng Pei,

Shanyu Yu,

Ping Liu

et al.

Advanced Functional Materials, Journal Year: 2022, Volume and Issue: 32(35)

Published: June 22, 2022

Abstract Stretchable conductors with the combination of high elasticity and electric conductivity have long been pursued in soft electronics. Liquid metals (LMs), whose mechanical properties match well elastomeric matrix, successfully applied robotics, electronic skins wearable devices. But it remains challenging to develop conductive composite elastomers LMs reversible adhesion self‐healing. Herein, EGaIn droplets are uniformly dispersed into elastomer, which contain dynamic disulfide endow elastomer thermal processability, recyclability, wet adhesion, With content ≥40 vol.%, resultant shows 1.3 × 104 S m −1 , self‐healing 8.0 h, strength up 670 kPa after curing for 2.0 h. When serving as adhesive, can easily adhere metal electrode light LED even when stretched 50%. self‐adhesive bioelectrode, also detect human electromyography signals. Thus, not only may this study provide a new platform designing self‐adhesive, self‐healing, liquid metals, but their promise facileness building damage‐endurable electronics applying human–machine interfaces.

Language: Английский

Citations

77

Recent progress in conductive electrospun materials for flexible electronics: Energy, sensing, and electromagnetic shielding applications DOI
Luiza A. Mercante, Rafaela S. André, Murilo H.M. Facure

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 465, P. 142847 - 142847

Published: April 10, 2023

Language: Английский

Citations

70

Electrochemical and Electrical Biosensors for Wearable and Implantable Electronics Based on Conducting Polymers and Carbon-Based Materials DOI
Peikai Zhang, Bicheng Zhu, Peng Du

et al.

Chemical Reviews, Journal Year: 2023, Volume and Issue: 124(3), P. 722 - 767

Published: Dec. 29, 2023

Bioelectronic devices are designed to translate biological information into electrical signals and vice versa, thereby bridging the gap between living world electronic systems. Among different types of bioelectronics devices, wearable implantable biosensors particularly important as they offer access physiological biochemical activities tissues organs, which is significant in diagnosing researching various medical conditions. Organic conducting semiconducting materials, including polymers (CPs) graphene carbon nanotubes (CNTs), some most promising candidates for biosensors. Their unique electrical, electrochemical, mechanical properties bring new possibilities that could not be realized by utilizing metals- or silicon-based analogues. The use organic- carbon-based conductors development has emerged a rapidly growing research field, with remarkable progress being made recent years. such materials addresses issue mismatched well improvement accuracy fidelity transferred information. In this review, we highlight advances field provide insights organic (semi)conducting materials' relate these their applications wearable/implantable We also perspective on potential exciting future developments

Language: Английский

Citations

53

An overview of flexible sensors from ionic liquid-based gels DOI
Xihua Cui,

Yangbin Xi,

Shiwen Tu

et al.

TrAC Trends in Analytical Chemistry, Journal Year: 2024, Volume and Issue: 174, P. 117662 - 117662

Published: March 23, 2024

Language: Английский

Citations

29

Projection Stereolithography 3D Printing High‐Conductive Hydrogel for Flexible Passive Wireless Sensing DOI

Yongding Sun,

Jin Cui, Shiwei Feng

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(25)

Published: April 4, 2024

Hydrogel-based electronics have inherent similarities to biological tissues and hold potential for wearable applications. However, low conductivity, poor stretchability, nonpersonalizability, uncontrollable dehydration during use limit their further development. In this study, projection stereolithography 3D printing high-conductive hydrogel flexible passive wireless sensing is reported. The prepared photocurable silver-based rapidly planarized into antenna shapes on substrates using surface stereolithography. After partial dehydration, silver flakes within the circuits form sufficient conductive pathways achieve high conductivity (387 S cm

Language: Английский

Citations

23

Biodegradable based TENGs for self-sustaining implantable medical devices DOI Creative Commons

Aiswarya Baburaj,

Swagata Banerjee,

Akshaya Kumar Aliyana

et al.

Nano Energy, Journal Year: 2024, Volume and Issue: 127, P. 109785 - 109785

Published: May 23, 2024

Biodegradable Triboelectric Nanogenerators (B-TENGs) have emerged as a groundbreaking technology with the potential to revolutionize healthcare, particularly in field of self-powered implanted medical devices. This review explains fundamental role B-TENGs addressing critical need for sustainable energy sources power implantable Beginning an exploration significance devices emphasizes necessity biodegradable and solutions. Through in-depth examination principles TENGs their integration both traditional materials, highlights design considerations essential development. The discusses diverse array materials employed various layers B-TENGs, including active layers, electrodes, associated signal conditioning circuits. evaluation performance enabling self-sustaining devices, promising outlook healthcare advancement through these innovative technologies. Moreover, critically assesses lifespan B-TENG addresses concerns regarding device durability. By identifying challenges practical implementation commercialization offers insights into overcoming barriers widespread adoption, thereby facilitating mainstream practices. Despite significant progress, acknowledges current facing provides perspectives on Finally, this paper underscores transformative advancing predicting future where could greatly impact patient care while reducing reliance conventional sources.

Language: Английский

Citations

22

Highly sensitive stretchable fiber-based temperature sensor enhanced by surface-chemically modified silver nanowires DOI

Jingling Ban,

Ying Lu, Jing Lü

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 482, P. 148772 - 148772

Published: Jan. 20, 2024

Language: Английский

Citations

19

3D printing of self-healing and degradable conductive ionoelastomers for customized flexible sensors DOI
Xin Luo,

Han Wu,

Chengyun Wang

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 483, P. 149330 - 149330

Published: Feb. 6, 2024

Language: Английский

Citations

19