Multifunctional Phase Change Films with High Mechanical Strength, Thermally Induced Switchable Adhesion, and Shape Recoverability for Infrared Stealth DOI
Guangyu Zhu, Wenjing Chen, Xiaowu Hu

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 17(1), P. 2293 - 2303

Published: Dec. 20, 2024

The application of organic solid–liquid phase change materials (PCMs) is limited for the leakage problem after and high rigidity. In this work, a novel flexible solid–solid PCM (DXPCM) was synthesized using block copolymerization process with polyethylene glycol (PEG) as energy storage segment. transition temperature (from 36.2 to 49.4 °C) enthalpy 83.27 123.35 J/g) DXPCM could be changed through adjusting molecular weight PEG. introduction hard chain segments endowed excellent flexibility, foldability, mechanical properties at room temperature. large number internal hydrogen bonds π–π stacking provided interesting thermally induced switchable adhesion recyclability. release elastic potential ensured that recover its original shape being deformed by external forces. It worth mentioning exhibits infrared stealth capability it can absorb latent heat long period time. conclusion, work developed film strength, adhesion, recovery capability, which has great in stealth.

Language: Английский

One‐Step Formed Janus Hydrogel with Time‐Space Regulating Properties for Suture‐Free and High‐Quality Tendon Healing DOI Creative Commons

Chenguang Ouyang,

Tian Tu, Haojie Yu

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 8, 2025

Janus hydrogels have promising applications in tendon healing and anti-peritendinous adhesions. However, their complicated preparation methods, weak mechanical properties, unstable adhesion interfaces severely limited application suture-free high-quality healing. In this work, by controlling the interfacial distribution of free -COOH groups cationic-π structures on both sides hydrogels, a series PZBA-EGCG-ALC with varying degrees asymmetric properties are successfully prepared using simple efficient one-step synthesis method. The tensile strength elongation at break hydrogel as high 0.51 ± 0.04 MPa 922.89 28.59%. addition, can achieve difference (nearly 20-fold) while maintaining strong bottom (up to 524.8 33.1 J m-2). spatial dimension, its excellent compliance one-sided behavior provide effective support physical barriers for injured Achilles tendons. More importantly, also minimize early inflammation generation time dimension via ROS-responsive PZBA-EGCG prodrug macromolecules. This study provided more convenient strategy constructing promote

Language: Английский

Citations

1

Multifunctional polyurethane materials in regenerative medicine and tissue engineering DOI Creative Commons
Gao‐peng Dang,

Jun‐ting Gu,

Jing‐han Song

et al.

Cell Reports Physical Science, Journal Year: 2024, Volume and Issue: 5(7), P. 102053 - 102053

Published: June 17, 2024

Facing the problems encountered in contemporary hard and soft tissue repair, need for better solutions has never been so pressing. Traditional repair methods often fall short, leading to disappointing therapeutic outcomes complications. To address associated with engineering, polyurethane stands out because of its remarkable adaptability healing potential. This review embarks on a journey through essential properties diverse classifications polyurethane, unveiling modification strategies that amplify efficacy. Beyond process mending gaps, capability as sophisticated drug delivery system is explored offer glimpse into versatile applications. Most notably, cutting-edge advancements clinical trials bridging voids both are discussed. The present explores future bio-interface providing wave inventive poised redefine landscape regenerative medicine.

Language: Английский

Citations

5

A bioinspired injectable antioxidant hydrogel for prevention of postoperative adhesion DOI

Lei Yuan,

Hongxiu Wei,

Zhongjing Pan

et al.

Journal of Materials Chemistry B, Journal Year: 2024, Volume and Issue: 12(28), P. 6968 - 6980

Published: Jan. 1, 2024

Postoperative adhesions, a prevalent complication following abdominal surgery, affect 90% of patients undergoing surgical procedures. Currently, the primary approach to prevent postoperative adhesions involves physical isolation site and surrounding tissues using hydrogel; however, this method represents rudimentary strategy. Herein, considering impact oxidative stress free radicals on adhesion during wound healing, an injectable antioxidant hydrogel, named PU-OHA-D, was successfully synthesized, which is formed by crosslinking dopamine-modified oxidized hyaluronic acid (OHA-D) dihydrazide-terminated polyurethane (PU-ADH) through hydrazone bonding. PU-OHA-D hydrogel possesses versatile characteristics such as rapid gel formation, injectability, self-repair capability biodegradability. Additionally, they exhibit excellent ability clear superior tissue adhesion. can be injected

Language: Английский

Citations

4

Amino acid-crosslinked 4arm-PLGA Janus Patch with Anti-Adhesive and Anti-bacterial Properties for Hernia Repair DOI
Yinghua Tao,

Guanhua Jiao,

Xiaocong Zhao

et al.

Colloids and Surfaces B Biointerfaces, Journal Year: 2024, Volume and Issue: 243, P. 114126 - 114126

Published: Aug. 3, 2024

Language: Английский

Citations

4

Self-healing physiological monitoring epidermal sensors of dual conductivity pathway with self-adaptive transformation DOI

Ziming Liao,

Zhu Ximing,

Shuquan Zhang

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 160169 - 160169

Published: Feb. 1, 2025

Language: Английский

Citations

0

A linearly programmable strategy for polymer elastomer mechanics DOI
Xue Dong, Xing Su, Jin Xu

et al.

Materials Horizons, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

The mechanical properties of polymer elastomer materials, such as strength and ductility, play important roles in a wide range applications, including the carrying major equipment construction infrastructure.

Language: Английский

Citations

0

Janus Textile: Advancing Wearable Technology for Autonomous Sweat Management and Beyond DOI Open Access
Dan Li, Weiyi Liu, Tao Peng

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: March 5, 2025

To alleviate the discomfort caused by excessive sweating, there is a growing emphasis on developing wearable textiles that can evacuate sweat autonomously. These advanced fabrics, unlike their absorbent and retention-prone predecessors, harness Janus structure-distinguished its asymmetric wettability-to facilitate one-way transport of liquid. This unique characteristic has significant potential in addressing issues related to bodily moisture propelling realm smart wearables. review offers comprehensive overview advancements Janus-structured within field, delving into mechanisms behind unidirectional liquid transport, which rely chemical gradient curvature strategies, alongside methodologies for achieving wettability. It further spotlights multifaceted applications Janus-based wearables, including thermal management, wound care, analysis. In addition examining existing hurdles, also explores avenues future innovation, envisioning new era tailored personalized comfort health monitoring capabilities.

Language: Английский

Citations

0

Facile preparation of lac terpene acid based heat setting adhesive with improved performances DOI
Sheng Yang, Lanxiang Liu, Qi Chen

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: unknown, P. 141947 - 141947

Published: March 1, 2025

Language: Английский

Citations

0

Recent Progress on Bio-based Polyurethanes: Synthesis, Structure and Cutting-Edge Applications DOI

Yunran Zhang,

Hui Dong,

Wenjie Yang

et al.

Materials Today Communications, Journal Year: 2025, Volume and Issue: unknown, P. 112279 - 112279

Published: March 1, 2025

Language: Английский

Citations

0

Tough and UV-resistant biodegradable polyurethane elastomers based on extracted lignin and treated wood flour DOI

Zi Feng He,

Li Chang, Fang Tian

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: unknown, P. 142259 - 142259

Published: March 1, 2025

Language: Английский

Citations

0