Intermarrying MOF Glass and Lead Halide Perovskites for Artificial Photosynthesis

Journal of the American Chemical Society, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 29, 2024

The development of efficient artificial photosynthesis systems is crucial for sustainable chemical production, as they mimic natural processes to convert solar energy into products, thereby addressing both and environmental challenges. main bottlenecks in current research include fabricating highly selective, stable, scalable catalysts, well effectively harnessing the full spectrum light, particularly low-energy, long-wavelength portion. Herein, we report a novel composite photocatalyst system based on lead halide perovskites embedded functionalized MOF glass. construction well-defined interface between light-harvesting perovskite stable Rh single-atom-containing glass mimics functions photosystem I (PS I). This facilitates photoinduced electron generation under visible light subsequent transfer coenzyme (NADH) regeneration with high selectivity. regenerated NADH can then be consumed by immobilized enzymes CO

Language: Английский

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Molecular dipole-modulated visible light photoredox reaction over conjugated polymers

Journal of Catalysis, Journal Year: 2023, Volume and Issue: 429, P. 115281 - 115281

Published: Dec. 27, 2023

Language: Английский

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Smart therapeutics: Evolution from small biomolecules to synthetic cells

Elsevier eBooks, Journal Year: 2024, Volume and Issue: unknown, P. 271 - 290

Published: Oct. 1, 2024

Language: Английский

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