A large-sized cell for solar-driven CO2 conversion with a solar-to-formate conversion efficiency of 7.2% DOI Creative Commons
Naohiko Kato, Shintaro Mizuno, Masahito Shiozawa

et al.

Joule, Journal Year: 2021, Volume and Issue: 5(3), P. 687 - 705

Published: Feb. 6, 2021

Language: Английский

In situ Irradiated XPS Investigation on S‐Scheme TiO2@ZnIn2S4 Photocatalyst for Efficient Photocatalytic CO2 Reduction DOI
Libo Wang, Bei Cheng, Liuyang Zhang

et al.

Small, Journal Year: 2021, Volume and Issue: 17(41)

Published: Sept. 12, 2021

Reasonable design of efficient hierarchical photocatalysts has gained significant attention. Herein, a step-scheme (S-scheme) core-shell TiO2 @ZnIn2 S4 heterojunction is designed for photocatalytic CO2 reduction. The optimized sample exhibits much higher photoreduction conversion rates (the sum yield CO, CH3 OH, and CH4 ) than the blank control, i.e., ZnIn2 . improved performance can be attributed to inhibited recombination photogenerated charge carriers induced by S-scheme heterojunction. improvement also large specific surface areas abundant active sites. Meanwhile, transfer mechanism testified in situ irradiated X-ray photoelectron spectroscopy, work function calculation, electron paramagnetic resonance measurements. This provides an effective strategy designing highly solar fuels.

Language: Английский

Citations

655
Solar fuels: research and development strategies to accelerate photocatalytic CO2 conversion into hydrocarbon fuels DOI Creative Commons
Eunhee Gong, Shahzad Ali, Chaitanya B. Hiragond

et al.

Energy & Environmental Science, Journal Year: 2021, Volume and Issue: 15(3), P. 880 - 937

Published: Nov. 16, 2021

Photocatalytic CO 2 conversion is vital technology to realize global carbon neutrality and generate future energy supplies. This review proposes fundamentals, challenges, strategies, prospects for photocatalytic research.

Language: Английский

Citations

554
Technological Innovations in Photochemistry for Organic Synthesis: Flow Chemistry, High-Throughput Experimentation, Scale-up, and Photoelectrochemistry DOI
Laura Buglioni, Fabian Raymenants, Aidan Slattery

et al.

Chemical Reviews, Journal Year: 2021, Volume and Issue: 122(2), P. 2752 - 2906

Published: Aug. 10, 2021

Photoinduced chemical transformations have received in recent years a tremendous amount of attention, providing plethora opportunities to synthetic organic chemists. However, performing photochemical transformation can be quite challenge because various issues related the delivery photons. These challenges barred widespread adoption steps industry. past decade, several technological innovations led more reproducible, selective, and scalable photoinduced reactions. Herein, we provide comprehensive overview these exciting advances, including flow chemistry, high-throughput experimentation, reactor design scale-up, combination photo- electro-chemistry.

Language: Английский

Citations

544
Next-generation applications for integrated perovskite solar cells DOI Creative Commons
Abdulaziz S. R. Bati, Yu Lin Zhong, Paul L. Burn

et al.

Communications Materials, Journal Year: 2023, Volume and Issue: 4(1)

Published: Jan. 5, 2023

Abstract Organic/inorganic metal halide perovskites attract substantial attention as key materials for next-generation photovoltaic technologies due to their potential low cost, high performance, and solution processability. The unique properties of the rapid advances that have been made in solar cell performance facilitated integration into a broad range practical applications, including tandem cells, building-integrated photovoltaics, space with batteries supercapacitors energy storage systems, photovoltaic-driven catalysis. In this Review, we outline notable achievements these photovoltaic-integrated technologies. Outstanding challenges future perspectives development fields applications are discussed.

Language: Английский

Citations

312
Operando cathode activation with alkali metal cations for high current density operation of water-fed zero-gap carbon dioxide electrolysers DOI
Balázs Endrődi, Angelika Anita Samu, Egon Kecsenovity

et al.

Nature Energy, Journal Year: 2021, Volume and Issue: 6(4), P. 439 - 448

Published: April 19, 2021

Language: Английский

Citations

270
Mott–Schottky Analysis of Photoelectrodes: Sanity Checks Are Needed DOI Creative Commons
Kevin Sivula

ACS Energy Letters, Journal Year: 2021, Volume and Issue: 6(7), P. 2549 - 2551

Published: July 9, 2021

ADVERTISEMENT RETURN TO ISSUEEditorialNEXTMott–Schottky Analysis of Photoelectrodes: Sanity Checks Are NeededKevin SivulaKevin SivulaÉcole Polytechnique Fédérale de Lausanne, Station 6, 1015 SwitzerlandMore by Kevin Sivulahttps://orcid.org/0000-0002-8458-0270Cite this: ACS Energy Lett. 2021, 7, 2549–2551Publication Date (Web):July 9, 2021Publication History Published online9 July 2021Published inissue 9 2021https://pubs.acs.org/doi/10.1021/acsenergylett.1c01245https://doi.org/10.1021/acsenergylett.1c01245editorialACS PublicationsCopyright © 2021 American Chemical Society. This publication is available under these Terms Use. Request reuse permissions free to access through this site. Learn MoreArticle Views21093Altmetric-Citations84LEARN ABOUT THESE METRICSArticle Views are the COUNTER-compliant sum full text article downloads since November 2008 (both PDF and HTML) across all institutions individuals. These metrics regularly updated reflect usage leading up last few days.Citations number other articles citing article, calculated Crossref daily. Find more information about citation counts.The Altmetric Attention Score a quantitative measure attention that research has received online. Clicking on donut icon will load page at altmetric.com with additional details score social media presence for given article. how calculated. Share Add toView InAdd Full Text ReferenceAdd Description ExportRISCitationCitation abstractCitation referencesMore Options onFacebookTwitterWechatLinked InRedditEmail (984 KB) Get e-AlertscloseSUBJECTS:Electrical properties,Electrodes,Nanorods,Photonics,Semiconductors e-Alerts

Language: Английский

Citations

218
Toward solar-driven carbon recycling DOI Creative Commons
Huiwen Lin, Shunqin Luo, Huabin Zhang

et al.

Joule, Journal Year: 2022, Volume and Issue: 6(2), P. 294 - 314

Published: Jan. 31, 2022

Carbon recycling will become a dominant trend toward alleviating extreme climate change and coping with the increasing energy demand in coming years. Solar-driven strategies have potential to convert CO2 solar fuels chemicals. In this forward-looking perspective, framework is outlined achieve "net-zero emission" blueprint by sorting out raw sources, products, feasible pathways, practical implementation through photocatalysis, photothermal catalysis, photoelectrochemical catalysis techniques. We comprehensively inspect compare state-of-art works framework, including solar-driven C1 fuel production from CO2, as well direct stepwise C2+ involving conversion. This analysis aspires provide most pathway forward finds that converting renewable H2 into can currently obtain best solar-to-fuel conversion efficiency target products high selectivity. Future visions on scientific, technological, economic issues are put determine what should be focus following decades.

Language: Английский

Citations

217
Photocatalytic CO2 conversion over single-atom MoN2 sites of covalent organic framework DOI

Mingpu Kou,

Wei Liu,

Yongye Wang

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2021, Volume and Issue: 291, P. 120146 - 120146

Published: March 18, 2021

Language: Английский

Citations

196
Toward efficient single-atom catalysts for renewable fuels and chemicals production from biomass and CO2 DOI Creative Commons
Yubing Lu, Zihao Zhang, Huamin Wang

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2021, Volume and Issue: 292, P. 120162 - 120162

Published: March 20, 2021

Language: Английский

Citations

168
Systematic Assessment of Solvent Selection in Photocatalytic CO2 Reduction DOI Open Access
Risov Das, Subhajit Chakraborty, Sebastian C. Peter

et al.

ACS Energy Letters, Journal Year: 2021, Volume and Issue: 6(9), P. 3270 - 3274

Published: Aug. 24, 2021

ADVERTISEMENT RETURN TO ISSUEPREVViewpointNEXTSystematic Assessment of Solvent Selection in Photocatalytic CO2 ReductionRisov DasRisov DasNew Chemistry Unit and School Advanced Materials, Jawaharlal Nehru Centre for Scientific Research, Jakkur, Bangalore 560064, IndiaMore by Risov Das, Subhajit ChakrabortySubhajit ChakrabortyNew Chakraborty, Sebastian C. Peter*Sebastian PeterNew India*Phone: 080-22082998. Email: [email protected], protected]More Peterhttps://orcid.org/0000-0002-5211-446XCite this: ACS Energy Lett. 2021, 6, 9, 3270–3274Publication Date (Web):August 24, 2021Publication History Received21 July 2021Accepted12 August 2021Published online24 inissue 10 September 2021https://pubs.acs.org/doi/10.1021/acsenergylett.1c01522https://doi.org/10.1021/acsenergylett.1c01522article-commentaryACS PublicationsCopyright © 2021 American Chemical Society. This publication is available under these Terms Use. Request reuse permissions free to access through this site. Learn MoreArticle Views12133Altmetric-Citations62LEARN ABOUT THESE METRICSArticle Views are the COUNTER-compliant sum full text article downloads since November 2008 (both PDF HTML) across all institutions individuals. These metrics regularly updated reflect usage leading up last few days.Citations number other articles citing article, calculated Crossref daily. Find more information about citation counts.The Altmetric Attention Score a quantitative measure attention that research has received online. Clicking on donut icon will load page at altmetric.com with additional details score social media presence given article. how calculated. Share Add toView InAdd Full Text ReferenceAdd Description ExportRISCitationCitation abstractCitation referencesMore Options onFacebookTwitterWechatLinked InRedditEmail (1 MB) Get e-AlertscloseSupporting Info (1)»Supporting Information Supporting SUBJECTS:Beverages,Catalysts,Composites,Electromagnetic radiation,Solvents e-Alerts

Language: Английский

Citations

141