Published: Jan. 1, 2025
Language: Английский
Frontiers of Environmental Science & Engineering, Journal Year: 2024, Volume and Issue: 18(6)
Published: April 10, 2024
Abstract Carbon capture, utilization and storage (CCUS) technologies play an essential role in achieving Net Zero Emissions targets. Considering the lack of timely reviews on recent advancements promising CCUS technologies, it is crucial to provide a prompt review advances understand current research gaps pertained its industrial application. To that end, this first summarized developmental history large-scale demonstrations. Then, based visually bibliometric analysis, carbon capture remains hotspot development. Noting materials applied process determines performance. As result, state-of-the-art emerging were comprehensively discussed. Gaps between state-of-art ideal counterpart are analyzed, insights into needs such as material design, optimization, environmental impact, technical economic assessments provided.
Language: Английский
Citations
51
Talanta, Journal Year: 2024, Volume and Issue: 274, P. 125949 - 125949
Published: March 19, 2024
Language: Английский
Citations
37
Chemical Science, Journal Year: 2024, Volume and Issue: 15(29), P. 11229 - 11266
Published: Jan. 1, 2024
This paper reviews advancements in flexible carbon-based and polymer gel materials for various types of energy storage systems, providing guidance future development next-generation wearable electronics.
Language: Английский
Citations
30
Carbon Energy, Journal Year: 2024, Volume and Issue: 6(4)
Published: Feb. 5, 2024
Abstract Graphitic carbon nitride (g‐C 3 N 4 ) is a highly recognized two‐dimensional semiconductor material known for its exceptional chemical and physical stability, environmental friendliness, pollution‐free advantages. These remarkable properties have sparked extensive research in the field of energy storage. This review paper presents latest advances utilization g‐C various storage technologies, including lithium‐ion batteries, lithium‐sulfur sodium‐ion potassium‐ion supercapacitors. One key strengths lies simple preparation process along with ease optimizing structure. It possesses abundant amino Lewis basic groups, as well high density nitrogen, enabling efficient charge transfer electrolyte solution penetration. Moreover, graphite‐like layered structure presence large π bonds contribute to versatility preparing multifunctional materials different dimensions, element group doping, conjugated systems. characteristics open up possibilities expanding application devices. article comprehensively reviews progress on highlights potential future applications this field. By exploring advantages unique features , provides valuable insights into harnessing full applications.
Language: Английский
Citations
19
Journal of Materials Informatics, Journal Year: 2025, Volume and Issue: 5(1)
Published: Feb. 12, 2025
Single-atom catalysts (SACs) have emerged as a research frontier in catalytic materials, distinguished by their unique atom-level dispersion, which significantly enhances activity, selectivity, and stability. SACs demonstrate substantial promise electrocatalysis applications, such fuel cells, CO2 reduction, hydrogen production, due to ability maximize utilization of active sites. However, the development efficient stable involves intricate design screening processes. In this work, artificial intelligence (AI), particularly machine learning (ML) neural networks (NNs), offers powerful tools for accelerating discovery optimization SACs. This review systematically discusses application AI technologies through four key stages: (1) Density functional theory (DFT) ab initio molecular dynamics (AIMD) simulations: DFT AIMD are used investigate mechanisms, with high-throughput applications expanding accessible datasets; (2) Regression models: ML regression models identify features that influence performance, streamlining selection promising materials; (3) NNs: NNs expedite known structural models, facilitating rapid assessment potential; (4) Generative adversarial (GANs): GANs enable prediction novel high-performance tailored specific requirements. work provides comprehensive overview current status insights recommendations future advancements field.
Language: Английский
Citations
3
Energy and AI, Journal Year: 2024, Volume and Issue: 16, P. 100361 - 100361
Published: March 30, 2024
Coupled electrochemical systems for the direct capture and conversion of CO2 have garnered significant attention owing to their potential enhance energy- cost-efficiency by circumventing amine regeneration step. However, optimizing coupled system is more challenging than handling separated because its complexity, caused incorporation solvent heterogeneous catalysts. Nevertheless, deployment machine learning can be immensely beneficial, reducing both time cost ability simulate describe complex with numerous parameters involved. In this review, we summarized techniques employed in development solvents such as ionic liquids, well To optimize a system, these two separately developed will need combined via future.
Language: Английский
Citations
17
Journal of Cleaner Production, Journal Year: 2024, Volume and Issue: 470, P. 143263 - 143263
Published: July 27, 2024
Language: Английский
Citations
12
Journal of CO2 Utilization, Journal Year: 2024, Volume and Issue: 83, P. 102809 - 102809
Published: May 1, 2024
MIL-101(Cr), a class of metal-organic framework, is potential candidate for CO2 capture applications because its high capacity adsorption and separation capability. However, the intrinsic microporous structure this nanomaterial poses limitations on kinetics. Techniques employed to enhance kinetics often adversely impact at equilibrium. Herein, as new approach, we prepared amine-functionalized FAC@MIL-101(Cr) composites with adjustable micro-mesoporous tunable nitrogen content by embedding different ratios activated carbon throughout framework MIL-101(Cr). This led simultaneous improvement in both CO2. The best adsorbent, FAC-6@MIL-101(Cr), has excellent textural properties surface area (1763.1 m2.g−1), great pore volume (1.29 cm3.g−1), suitable (4.7 wt%). analysis revealed that modification MIL-101(Cr) improved from 3.21 5.27 mmol/g under standard conditions 1 bar 25 °C. Furthermore, FAC-6@MIL-101(Cr) adsorbent demonstrated fast (three times more relative pure MIL-101(Cr)), CO2/N2 selectivity, remarkable cyclic stability. results confirmed hybridization enhanced polarizability samples, causing robust CO2-adsorbent interactions. Simultaneously, existence mesopores facilitated transport into interior pores, resulting efficient contact molecules all amine sites faster rate well regeneration. According density functional theory (DFT) calculations, process induces significant changes composites' electronic structure, enhancing their interact effectively. On other hand, DFT calculations confirm N2 molecule less evidenced calculated small energy charge-transfer values.
Language: Английский
Citations
11
Inorganic Chemistry Frontiers, Journal Year: 2024, Volume and Issue: 11(19), P. 6275 - 6306
Published: Jan. 1, 2024
We summarize the different synthetic strategies of MOF-derived micro-/nano-materials to date, including but not limited calcining, phosphating, sulfurization, selenylation method, ion exchange, and etching strategies.
Language: Английский
Citations
11
Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 130981 - 130981
Published: Dec. 1, 2024
Language: Английский
Citations
11