Surface Reaction Mechanism of ZSM-5(3T)@NH2-MIL-53(Al) Core-Shell Catalyst for Dimethyldichlorosilane Synthesis DOI
Wenyuan Xu,

Kehan Wu,

Y. Wang

et al.

Journal of Solid State Chemistry, Journal Year: 2024, Volume and Issue: unknown, P. 125127 - 125127

Published: Dec. 1, 2024

Language: Английский

Strategies for Stabilizing Metal Halide Perovskite Light-Emitting Diodes: Bulk and Surface Reconstruction of Perovskite Nanocrystals DOI
Ye Wu, Desui Chen, Guangruixing Zou

et al.

ACS Nano, Journal Year: 2025, Volume and Issue: unknown

Published: March 7, 2025

Light-emitting colloidal lead halide perovskite nanocrystals (PeNCs) are considered promising candidates for next-generation vivid displays. However, the operational stability of light-emitting diodes (LEDs) based on PeNCs is still lower than those polycrystalline films, which requires an understanding defect formation in PeNCs, both inside crystal lattice ("bulk") and at surface. Meanwhile, uncontrollable ion redistribution electrochemical reactions under LED operation can be severe, also related to bulk surface quality a well-designed device architecture boost carrier injection balance radiative recombination. In this review, we consider reconstruction by enhancing rigidity rationally selecting ligands. Degradation pathways applied voltage discussed, strategies avoid undesirable migration PeNC films. Subsequently, other critical issues hindering commercial application LEDs including toxicity Pb perovskites, scale-up deposition design active-matrix prototypes high-resolution modules.

Language: Английский

Citations

1

Effect of precursors on the structure and photocatalytic performance of g-C3N4 for NO oxidation and CO2 reduction DOI
Liang Ma, Zhou Li, Zhiqiang Jiang

et al.

Chinese Journal of Structural Chemistry, Journal Year: 2024, Volume and Issue: 43(11), P. 100416 - 100416

Published: Aug. 14, 2024

Language: Английский

Citations

7

Boosting Photocatalytic CO2 Methanation through Interface Fusion over CdS Quantum Dot Aerogels DOI

Shishun Xu,

Guocan Jiang, Hangkai Zhang

et al.

Small, Journal Year: 2024, Volume and Issue: unknown

Published: May 15, 2024

Abstract In the field of photocatalytic CO 2 reduction, quantum dot (QD) assemblies have emerged as promising candidate photocatalysts due to their superior light absorption and better substrate adsorption. However, poor contacts within QD lead low interfacial charge transfer efficiency, making suffer from unsatisfactory performance. Herein, a novel approach is presented involving construction strongly fused CdS (CdS gel) for reduction. The gel demonstrates outstanding performance methanation, achieving CH 4 generation rate ≈296 µmol g −1 h , with selectivity surpassing 76% an apparent yield (AQY) 1.4%. Further investigations reveal that robust fusion in these QDs not only boosts ability absorb visible but also significantly promotes separation. present work paves way utilizing realizing efficient reduction highlights critical role engineering photocatalysts.

Language: Английский

Citations

6

Micro/Nano Engineering Advances Next-Generation Flexible X-ray Detectors DOI
Xiangyu Ou,

Zhongzhu Hong,

Qinxia Wu

et al.

ACS Nano, Journal Year: 2024, Volume and Issue: unknown

Published: Sept. 23, 2024

The growing demands for X-ray imaging applications impose diverse and stringent requirements on advanced detectors. Among these, flexibility stands out as the most expected characteristic next-generation Flexible detectors can spatially conform to nonflat surfaces, substantially improving resolution, reducing exposure dosage, enabling extended application opportunities that are hardly achievable by conventional rigid flat-panel Over past years, indirect- direct-conversion flexible have made marvelous achievements. In particular, microscale nanoscale engineering technologies play a pivotal role in defining optical, electrical, mechanical properties of this Perspective, we spotlight recent landmark advancements from aspects micro/nano strategies, which broadly categorized into two prevailing modalities: materials-in-substrate materials-on-substrate. We also discuss existing challenges hindering development detectors, well prospective research mitigate these issues.

Language: Английский

Citations

5

Preparation and properties of multiphase composite enhanced functional organosilicon nano-coatings DOI
Peipei Lu,

Yiyao Wang,

Hongfeng Wang

et al.

Journal of the Taiwan Institute of Chemical Engineers, Journal Year: 2024, Volume and Issue: 165, P. 105717 - 105717

Published: Aug. 20, 2024

Language: Английский

Citations

4

Locking in Color: Stable RGB Perovskite Nanocrystal Films via UV Cross‐Linking DOI Creative Commons
Patrick Ganswindt,

Isabella Tepfenhart,

Andreas Singldinger

et al.

Advanced Optical Materials, Journal Year: 2025, Volume and Issue: unknown

Published: April 7, 2025

Abstract Perovskite nanocrystals have positioned themselves at the forefront of next‐generation emitter applications due to their extraordinary optoelectronic properties, which include widely tunable narrow emission spectra and low‐cost syntheses. However, stability issues halide ion exchange inhibit realization heterostructures, severely limiting applicability decelerating commercialization. Here, a block copolymer templated perovskite nanocrystal synthesis with post‐synthetic treatment is combined UV‐C light obtain ultra‐stable thin film emitters. The UV induces cross‐linking between polymer strands, thereby rendering them insoluble organic solvent nearly impervious diffusion while retaining nanocrystals’ optical properties. This method enabled fabrication an all‐perovskite white light‐emitting film. resulting films feature linewidths ( < 95 meV) for each RGB peak. Additionally, color temperature ’white’ can be tuned gamut approximating Rec. 2020 standard. These RGB‐emissive phosphor commercial or blue LED backlights create high‐efficiency, high‐quality phosphor‐converted LEDs displays.

Language: Английский

Citations

0

Achieving High Loading Capacity of Perovskite Nanocrystals in Pore-Reamed Metal–Organic Frameworks for Bright Scintillators DOI

Linyuan Gu,

Zhi Yang,

Jiangtao Cui

et al.

ACS Nano, Journal Year: 2025, Volume and Issue: unknown

Published: April 14, 2025

Lead halide perovskite nanocrystal (PNC) scintillators featuring a fast decay and high radiation hardness have garnered significant attention. A PNC loading is essential to ensure strong X-ray absorption for scintillator applications, but concentrated PNCs tend aggregate in the solid state, resulting emission quenching. Employing dispersion medium offers promising strategy produce high-loading solids without agglomeration. Herein, we synthesize CsPbBr3 PNC/metal-organic framework (MOF) nanostructures achieve within MOF hosts. The macroporous cavities of hierarchically porous (HP) MOFs can host more than confined nanometer-scale spaces microporous MOFs. Additionally, surface-rich structure aids dispersing PNCs, effectively reducing aggregation-induced We find that HP-MOFs ratio 75%, as well less-aggregated PNCs. As result, PNC/HP-MOF exhibits 2.3 times higher light yield scintillator, primarily from enhanced luminance efficiency well-dispersed bright features nanostructure enable static dynamic imaging industrial inspection applications. These findings highlight constructing crucial advancing applications scintillators.

Language: Английский

Citations

0

Multidentate Chelation Defect Passivation via Hyperbranched Polysiloxane for Efficient and Stable Inverted Perovskite Solar Cells DOI

Guangpeng Feng,

Tong Wang,

Xilai He

et al.

Nano Energy, Journal Year: 2025, Volume and Issue: unknown, P. 111084 - 111084

Published: April 1, 2025

Language: Английский

Citations

0

Metal Halide Perovskite as Down‐Conversion Materials for Advanced Display DOI
Xiang Zhang, Nian Liu,

Hainan Du

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: May 9, 2025

Abstract Metal halide perovskites have gained worldwide attention as excellent optoelectronic materials. Over the past decade, perovskite‐based color conversion technology has shown significant promise for commercialization, particularly in display applications. Prototypes of displays utilizing this made remarkable achievements. As slightly more than a decade elapsed since discovery metal perovskite light‐emitting diodes, comprehensive review, and outlook is crucial to advance explore its full potential next‐generation displays. To end, paper systematically outlined strategies enhancing material performance patterning fabrication techniques converters. Building on current technological advancements, review also summarizes new chances emerging morphologies. Furthermore, key challenges hindering commercialization converters are pointed out guide future research development. This aims offer valuable insights into advanced

Language: Английский

Citations

0

Dual-Shell Protection Enables Highly Efficient and Stable All-Inorganic Perovskite Composites for Light-Emitting-Diodes DOI
Yanqiao Xu, Wentao Li, Qing Hu

et al.

Journal of Alloys and Compounds, Journal Year: 2024, Volume and Issue: unknown, P. 177135 - 177135

Published: Oct. 1, 2024

Language: Английский

Citations

2