Advanced Energy and Sustainability Research,
Journal Year:
2024,
Volume and Issue:
unknown
Published: Dec. 30, 2024
Metal‐organic
frameworks
(MOFs)
have
emerged
as
key
materials
for
carbon
capture
and
conversion,
particularly
in
photocatalytic
CO
2
reduction.
However,
inconsistent
reporting
of
essential
parameters
the
literature
hinders
informed
decisions
about
material
selection
optimization.
This
perspective
highlights
need
a
user‐friendly,
centralized
database
supported
by
automated
data
extraction
using
natural
language
processing
tools
to
streamline
comparisons
MOF
materials.
By
consolidating
crucial
from
scientific
literature,
such
promotes
efficient
decision‐making
utilization.
Emphasizing
significance
open‐source
initiatives
principles
FAIR
data—ensuring
are
Findable,
Accessible,
Interoperable,
Reusable—a
collaborative
approach
management
sharing
is
advocated
for.
Making
database‐accessible
worldwide
enhances
quality
reliability,
fostering
innovation
progress
conversion
Additionally,
databases
valuable
creating
artificial
intelligence
assist
researchers
discovery
synthesis
conversion.
Nano Letters,
Journal Year:
2025,
Volume and Issue:
unknown
Published: May 2, 2025
Trace
residual
solvents
in
solid
polymer
electrolytes
(SPEs)
significantly
affect
electrolyte
and
interface
properties,
where
optimal
selection
enhances
the
ionic
conductivity
transference
numbers.
However,
solvent
complexity
hinders
general
screening
methods.
We
establish
a
universal
criterion
linking
electronic
(highest
occupied
molecular
orbital
(HOMO),
lowest
unoccupied
(LUMO))
macroscopic
properties
(dielectric
constant,
dipole
moment,
polarizability)
via
machine
learning
on
an
∼10
000-solvent
dataset
from
high-throughput
density
functional
theory
(DFT).
Two
solvents,
N-methoxy-N-methyl-2,2,2-trifluoroacetamide
2,2,2-trifluoro-N,N-dimethylacetamide
were
identified.
Experimental
incorporation
of
trace
into
poly(vinylidene
fluoride-co-hexafluoropropylene)
matrix
achieves
4.5
V
window,
5.5
×
10-4
S
cm-1
(30
°C),
Li+
number
0.78.
The
cell
retains
86.7%
capacity
over
500
cycles
(LiFePO4)
98.7%
after
200
at
2C
(LiNi0.9Co0.05Mn0.05O2),
outperforming
2,2,2-trifluoro-N,N-dimethylacetamide,
dimethylformamide,
N-methyl-2-pyrrolidone,
dimethyl
sulfoxide.
This
synergy
enables
balanced
ion
transport,
wide
stability,
cycling
durability,
advancing
safer
high-energy
lithium
metal
batteries.
Our
integrated
approach
establishes
paradigm
for
rational
SPE
design,
accelerating
next-generation
battery
development.
Advanced Energy and Sustainability Research,
Journal Year:
2024,
Volume and Issue:
unknown
Published: Dec. 30, 2024
Metal‐organic
frameworks
(MOFs)
have
emerged
as
key
materials
for
carbon
capture
and
conversion,
particularly
in
photocatalytic
CO
2
reduction.
However,
inconsistent
reporting
of
essential
parameters
the
literature
hinders
informed
decisions
about
material
selection
optimization.
This
perspective
highlights
need
a
user‐friendly,
centralized
database
supported
by
automated
data
extraction
using
natural
language
processing
tools
to
streamline
comparisons
MOF
materials.
By
consolidating
crucial
from
scientific
literature,
such
promotes
efficient
decision‐making
utilization.
Emphasizing
significance
open‐source
initiatives
principles
FAIR
data—ensuring
are
Findable,
Accessible,
Interoperable,
Reusable—a
collaborative
approach
management
sharing
is
advocated
for.
Making
database‐accessible
worldwide
enhances
quality
reliability,
fostering
innovation
progress
conversion
Additionally,
databases
valuable
creating
artificial
intelligence
assist
researchers
discovery
synthesis
conversion.
