Defect Engineering of Metal‐Based Atomically Thin Materials for Catalyzing Small‐Molecule Conversion Reactions DOI Open Access

Juanjuan Huo,

Yuhai Dou, Chao Wu

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 20, 2024

Abstract Recently, metal‐based atomically thin materials (M‐ATMs) have experienced rapid development due to their large specific surface areas, abundant electrochemically accessible sites, attractive chemistry, and strong in‐plane chemical bonds. These characteristics make them highly desirable for energy‐related conversion reactions. However, the insufficient active sites slow reaction kinetics leading unsatisfactory electrocatalytic performance limited commercial application. To address these issues, defect engineering of M‐ATMs has emerged increase modify electronic structure, enhance catalytic reactivity stability. This review provides a comprehensive summary strategies M‐ATM nanostructures, including vacancy creation, heteroatom doping, amorphous phase/grain boundary generation, heterointerface construction. Introducing recent advancements in application electrochemical small molecule reactions (e.g., hydrogen, oxygen, carbon dioxide, nitrogen, sulfur), which can contribute circular economy by recycling molecules like H 2 , O CO N S. Furthermore, crucial link between reconstruction atomic‐level structure activity via analyzing dynamic evolution during process is established. The also outlines challenges prospects associated with M‐ATM‐based catalysts inspire further research efforts developing high‐performance M‐ATMs.

Language: Английский

Materials and System Design in Solar-Driven Hydrogen Production DOI Creative Commons
Jingxiang Low, Yujie Xiong

ACS Materials Letters, Journal Year: 2024, Volume and Issue: 6(8), P. 3713 - 3715

Published: Aug. 5, 2024

Language: Английский

Citations

5
Advanced bipolar membranes with earth-abundant water dissociation catalysts for durable ampere-level water electrolysis DOI Creative Commons

Fanglin Duan,

Xiaojiang Li,

Fen Luo

et al.

Advanced Membranes, Journal Year: 2025, Volume and Issue: unknown, P. 100152 - 100152

Published: May 1, 2025

Language: Английский

Citations

0
Design and Application of Electrocatalyst Based on Machine Learning DOI Creative Commons

Yulan Gu,

Hailong Zhang, Zhen Xu

et al.

Interdisciplinary materials, Journal Year: 2025, Volume and Issue: unknown

Published: May 15, 2025

ABSTRACT Data‐driven artificial intelligence provides strong technical support for addressing global energy and environmental issues. The powerful data processing analysis capabilities of machine learning (ML) can quickly predict electrocatalytic performance, improving the efficiency catalyst design time‐consuming inefficient nature traditional design. By integrating ML with theoretical calculations experiments, catalytic reaction processes be precisely regulated. This not only accelerates discovery new catalysts but also drives development more efficient environmentally friendly sustainable technologies. In this article, we discuss approaches to discovering novel driven by ML, focusing on activity prediction, barrier optimization, innovative materials. We systematically application in field electrocatalysis explore future prospects domain. provide a comprehensive in‐depth its potential development.

Language: Английский

Citations

0
Defect Engineering of Metal‐Based Atomically Thin Materials for Catalyzing Small‐Molecule Conversion Reactions DOI Open Access

Juanjuan Huo,

Yuhai Dou, Chao Wu

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 20, 2024

Abstract Recently, metal‐based atomically thin materials (M‐ATMs) have experienced rapid development due to their large specific surface areas, abundant electrochemically accessible sites, attractive chemistry, and strong in‐plane chemical bonds. These characteristics make them highly desirable for energy‐related conversion reactions. However, the insufficient active sites slow reaction kinetics leading unsatisfactory electrocatalytic performance limited commercial application. To address these issues, defect engineering of M‐ATMs has emerged increase modify electronic structure, enhance catalytic reactivity stability. This review provides a comprehensive summary strategies M‐ATM nanostructures, including vacancy creation, heteroatom doping, amorphous phase/grain boundary generation, heterointerface construction. Introducing recent advancements in application electrochemical small molecule reactions (e.g., hydrogen, oxygen, carbon dioxide, nitrogen, sulfur), which can contribute circular economy by recycling molecules like H 2 , O CO N S. Furthermore, crucial link between reconstruction atomic‐level structure activity via analyzing dynamic evolution during process is established. The also outlines challenges prospects associated with M‐ATM‐based catalysts inspire further research efforts developing high‐performance M‐ATMs.

Language: Английский

Citations

2