
Atmospheric measurement techniques, Journal Year: 2024, Volume and Issue: 17(16), P. 4843 - 4861
Published: Aug. 23, 2024
Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties clouds. In this work, we develop a novel method that differentiates between various phases clouds, such as dominated by pure liquid or segments, compared with those having crystals surrounded supercooled water droplets vice versa. Using method, examine relationship macrophysical Southern Ocean at −40 to 0 °C (e.g. stratiform cumuliform clouds) based on situ aircraft-based observations during US National Science Foundation Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. results show exchange from perspective, represented increasing spatial ratio regions containing relative total in-cloud region (defined ratio), is positively correlated phase content (IWC), decreasing (LWC), mass fraction, particle number fraction (IPNF). becomes more significant 3 when cloud (ICRs) start appear. Occurrence frequencies thermodynamic change similar temperature (i.e. −17.5 °C) among three types definitions ratio, IPNF. indirect effects are quantified for different using concentrations aerosols greater than 100 500 nm (N>100 N>500, respectively). N>500 shows stronger positive correlations ratios N>100. This result indicates larger potentially contain ice-nucleating particles (INPs), which facilitate formation impact also 2 just appear mixed ICRs have formed, possibly due competing aerosol primary secondary production 3. dynamic conditions each phase. turbulence higher updraughts coexist (phases 1 4, highest seen crystals. These indicate both support maintenance amongst Overall, these illustrate varying aerosols, thermodynamics, dynamics through stages evolution new categorizes phases.
Language: Английский