Decoupling of mechanical properties and ionic conductivity in supramolecular lithium ion conductors DOI Creative Commons
David G. Mackanic, Xuzhou Yan, Qiuhong Zhang

et al.

Nature Communications, Journal Year: 2019, Volume and Issue: 10(1)

Published: Nov. 26, 2019

The emergence of wearable electronics puts batteries closer to the human skin, exacerbating need for battery materials that are robust, highly ionically conductive, and stretchable. Herein, we introduce a supramolecular design as an effective strategy overcome canonical tradeoff between mechanical robustness ionic conductivity in polymer electrolytes. lithium ion conductor utilizes orthogonally functional H-bonding domains ion-conducting create electrolyte with unprecedented toughness (29.3 MJ m-3) high (1.2 × 10-4 S cm-1 at 25 °C). Implementation binder material allows creation stretchable lithium-ion electrodes strain capability over 900% via conventional slurry process. nature these components enables intimate bonding electrode-electrolyte interface. Combination leads capacity 1.1 mAh cm-2 functions even when stretched 70% strain. method reported here decoupling from properties opens promising route high-toughness transport energy storage applications.

Language: Английский

Neural recording and modulation technologies DOI
Ritchie Chen,

Andrés Canales,

Polina Anikeeva

et al.

Nature Reviews Materials, Journal Year: 2017, Volume and Issue: 2(2)

Published: Jan. 4, 2017

Language: Английский

Citations

549

Self‐Healing Hydrogels: The Next Paradigm Shift in Tissue Engineering? DOI Creative Commons
Sepehr Talebian, Mehdi Mehrali, Nayere Taebnia

et al.

Advanced Science, Journal Year: 2019, Volume and Issue: 6(16)

Published: June 14, 2019

Abstract Given their durability and long‐term stability, self‐healable hydrogels have, in the past few years, emerged as promising replacements for many brittle currently being used preclinical or clinical trials. To this end, incompatibility between hydrogel toughness rapid self‐healing remains unaddressed, therefore most of still face serious challenges within dynamic mechanically demanding environment human organs/tissues. Furthermore, depending on target tissue, must comply with a wide range properties including electrical, biological, mechanical. Notably, incorporation nanomaterials into double‐network is showing great promise feasible way to generate above‐mentioned attributes. Here, recent progress development multifunctional various tissue engineering applications discussed detail. Their potential rapidly expanding areas bioelectronic hydrogels, cyborganics, soft robotics are further highlighted.

Language: Английский

Citations

529

Glial responses to implanted electrodes in the brain DOI
Joseph W. Salatino, Kip A. Ludwig, Takashi D.Y. Kozai

et al.

Nature Biomedical Engineering, Journal Year: 2017, Volume and Issue: 1(11), P. 862 - 877

Published: Nov. 3, 2017

Language: Английский

Citations

516

Ultraflexible nanoelectronic probes form reliable, glial scar–free neural integration DOI Creative Commons
Lan Luan, Xiaoling Wei, Zhengtuo Zhao

et al.

Science Advances, Journal Year: 2017, Volume and Issue: 3(2)

Published: Feb. 3, 2017

Implanted brain electrodes construct the only means to electrically interface with individual neurons in vivo, but their recording efficacy and biocompatibility pose limitations on scientific clinical applications. We showed that nanoelectronic thread (NET) subcellular dimensions, ultraflexibility, cellular surgical footprints form reliable, glial scar-free neural integration. demonstrated NET reliably detected tracked units for months; impedance, noise level, single-unit yield, signal amplitude remained stable during long-term implantation. In vivo two-photon imaging postmortem histological analysis revealed seamless, integration of probes local vasculature networks, featuring fully recovered capillaries an intact blood-brain barrier complete absence chronic neuronal degradation scar.

Language: Английский

Citations

515

High-performance stretchable conductive nanocomposites: materials, processes, and device applications DOI
Suji Choi, Sang Ihn Han,

Dokyoon Kim

et al.

Chemical Society Reviews, Journal Year: 2018, Volume and Issue: 48(6), P. 1566 - 1595

Published: Dec. 6, 2018

Highly conductive and intrinsically stretchable electrodes are vital components of soft electronics such as transistors circuits, sensors actuators, light-emitting diode arrays, energy harvesting devices. Many kinds conducting nanomaterials with outstanding electrical mechanical properties have been integrated elastomers to produce nanocomposites. Understanding the characteristics these nanocomposites assessing feasibility their fabrication therefore critical for development high-performance conductors electronic We herein summarise recent advances in based on percolation networks nanoscale fillers elastomeric media. After discussing material-, dimension-, size-dependent implications, we highlight various techniques that used reduce contact resistance between filler materials. Furthermore, categorize elastomer matrices different stretchabilities polymeric chain structures. Then, discuss toward use electronics. Finally, provide representative examples device applications conclude review a brief outlook future research.

Language: Английский

Citations

513

Stretchable Electronics Based on PDMS Substrates DOI
Dianpeng Qi, Kuiyuan Zhang, Gongwei Tian

et al.

Advanced Materials, Journal Year: 2020, Volume and Issue: 33(6)

Published: Aug. 23, 2020

Abstract Stretchable electronics, which can retain their functions under stretching, have attracted great interest in recent decades. Elastic substrates, bear the applied strain and regulate distribution circuits, are indispensable components stretchable electronics. Moreover, self‐healing property of substrate is a premise to endow electronics with same characteristics, so device may recover from failure resulting large frequent deformations. Therefore, properties elastic crucial overall performance devices. Poly(dimethylsiloxane) (PDMS) widely used as material for not only because its advantages, include stable chemical properties, good thermal stability, transparency, biological compatibility, but also capability attaining designer functionalities via surface modification bulk tailoring. Herein, strategies fabricating on PDMS substrates summarized, influence physical PDMS, including status, modulus, geometric structures, discussed. Finally, challenges future opportunities based considered.

Language: Английский

Citations

513

Nanobiotechnology approaches for engineering smart plant sensors DOI
Juan Pablo Giraldo, Honghong Wu, Gregory M. Newkirk

et al.

Nature Nanotechnology, Journal Year: 2019, Volume and Issue: 14(6), P. 541 - 553

Published: June 1, 2019

Language: Английский

Citations

467

Tissue–electronics interfaces: from implantable devices to engineered tissues DOI
Ron Feiner, Tal Dvir

Nature Reviews Materials, Journal Year: 2017, Volume and Issue: 3(1)

Published: Nov. 28, 2017

Language: Английский

Citations

460

Human eye-inspired soft optoelectronic device using high-density MoS2-graphene curved image sensor array DOI Creative Commons
Changsoon Choi, Moon Kee Choi, Siyi Liu

et al.

Nature Communications, Journal Year: 2017, Volume and Issue: 8(1)

Published: Nov. 15, 2017

Soft bioelectronic devices provide new opportunities for next-generation implantable owing to their soft mechanical nature that leads minimal tissue damages and immune responses. However, a form of the optoelectronic device optical sensing retinal stimulation has not been developed yet because bulkiness rigidity conventional imaging modules composing materials. Here, we describe high-density hemispherically curved image sensor array leverages atomically thin MoS2-graphene heterostructure strain-releasing designs. The exhibits infrared blindness successfully acquires pixelated signals. We corroborate validity proposed materials ultrathin designs through theoretical modeling finite element analysis. Then, propose as promising in implant. CurvIS is applied human eye-inspired can detect signals apply programmed electrical optic nerves with minimum side effects retina.

Language: Английский

Citations

456

Next-generation probes, particles, and proteins for neural interfacing DOI Creative Commons
Jonathan Rivnay,

Huiliang Wang,

Lief E. Fenno

et al.

Science Advances, Journal Year: 2017, Volume and Issue: 3(6)

Published: June 2, 2017

Multimodal and multidisciplinary approaches lead to next-generation technologies for reading modulating neural function.

Language: Английский

Citations

445