Innovative Approach to Sustainable Fertilizer Production: Leveraging Electrically Assisted Conversion of Sewage Sludge for Nutrient Recovery DOI Creative Commons
Gerardine G. Botte, Dayana Donneys-Victoria, Christian E. Alvarez‐Pugliese

et al.

ACS Omega, Journal Year: 2024, Volume and Issue: 9(50), P. 49692 - 49706

Published: Dec. 7, 2024

Efforts addressing sludge management, food security, and resource recovery have led to novel approaches in these areas. Electrically assisted conversion of stands out as a promising technology for sewage valorization, producing nitrogen phosphorus-based fertilizers. The adoption this technology, which could lead fertilizer circular economy, holds the potential catalyze transformative change wastewater treatment facilities toward process intensification, innovation, sustainability. This paper provides insights into economic aspects policy considerations, challenges involved realizing electrified processes valorization. To demonstrate impact case study its implementation United States assuming municipal plants market is discussed. It was found that electrically enable phosphorus from waste, representing up 9% 32% consumption U.S. use. also enables full electrification modularization process, thereby presenting significant environmental opportunities.

Language: Английский

Exploring CO2 reduction and crossover in membrane electrode assemblies DOI Creative Commons
Eric W. Lees, Justin C. Bui, Oyinkansola Romiluyi

et al.

Nature Chemical Engineering, Journal Year: 2024, Volume and Issue: 1(5), P. 340 - 353

Published: May 6, 2024

Language: Английский

Citations

19

Accelerating CO2 electrochemical conversion towards industrial implementation DOI Creative Commons
Doris Segets, Corina Andronescu, Ulf‐Peter Apfel

et al.

Nature Communications, Journal Year: 2023, Volume and Issue: 14(1)

Published: Dec. 1, 2023

The electrochemical conversion of carbon dioxide by means renewable electricity holds great promise. However, despite significant progress in current literature, there remains a gap between fundamental research and the industrial demands to establish new disruptive technologies real world applications. This primarily arises from mismatch performance parameters requirements both areas, leading challenges technology transfer. We herein suggest pathways bridge this outline limitations field, proposing key procedures towards accelerated streamlined development. Despite CO2 demands. Comment discusses for applications outlines field.

Language: Английский

Citations

31

Electrochemical CO2 Reduction: Advances, Insights, Challenges, and Future Directions DOI Creative Commons
Asghar Ali, Muhammad Qasim, S. Sakhi

et al.

Materials Today Sustainability, Journal Year: 2025, Volume and Issue: unknown, P. 101089 - 101089

Published: Feb. 1, 2025

Language: Английский

Citations

1

Carbon utilization in natural gas-based hydrogen production via carbon dioxide electrolysis: Towards cost-competitive clean hydrogen DOI
Wonjun Noh,

Seoyeon Cho,

Inkyu Lee

et al.

Energy Conversion and Management, Journal Year: 2024, Volume and Issue: 314, P. 118719 - 118719

Published: June 22, 2024

Language: Английский

Citations

8

Deriving an Efficient and Stable Microenvironment for a CO2 MEA Electrolyzer by Reverse Osmosis DOI
Jae‐Yong Park,

Eung‐Dab Kim,

Sang-Kuk Kim

et al.

ACS Energy Letters, Journal Year: 2024, Volume and Issue: 9(7), P. 3342 - 3350

Published: June 14, 2024

In a membrane electrode assembly (MEA) electrolyzer based on cation-exchange membrane, achieving an efficient and stable CO2 reduction reaction (CO2RR) is challenging because the transport of protons, cations, electro-osmotic water from anode changes balance ions. Herein, we derived microenvironment for CO2RR performance by using two strategies. First, mixture carbon anion-exchange ionomer buffer layers used to hold cations while managing in local alkaline media. The second strategy involves pressurizing only cathode side, resulting high concentration enhancing reverse osmosis phenomenon. synergistic effects these strategies create leading operation. Our approach viable industrial applications pressurized MEA systems are processes that can be commercialized.

Language: Английский

Citations

7

Benchmarking microwave-induced CO2 plasma splitting against electrochemical CO2 reduction for a comparison of promising technologies DOI Creative Commons
Ante Hećimović, Matthew T. Mayer, L.G.J. de Haart

et al.

Journal of CO2 Utilization, Journal Year: 2024, Volume and Issue: 83, P. 102825 - 102825

Published: May 1, 2024

Plasma conversion technology is an emerging technique under development to activate, convert or valorize gas molecules such as CO2, N2, CH4, NH3 and others. A large-scale application beyond the lab-scale demonstrator unit requires assessment of efficiency this new technology. The straightforward approach for benchmarking with other well-established technologies similar readiness level (TRL). In paper we present a atmospheric pressure microwave-induced CO2 plasma splitting electrochemical conversion, via both low-temperature high-temperature electrolysis. An additional step oxygen removal in case reactor implemented due difference output stream (gas mixture containing CO, O2) (typical on cathode CO). For benchmarking, comprehensive set comparison parameters that are applicable route identified grouped three categories: performance, interfaces, economics. these demonstrates terms electric power consumption (EPC; required production one Nm3CO) (∼20 kWh/Nm3CO) ballpark two (∼4–20 kWh/Nm3CO). key features relatively large (up 56%) moderate energy efficiencies 27%). Also, reduced purity only 98% can be used without decrease CO values currently at 3.5 slm (standard litre per minute). Fast on/off response time order minutes, no need hot standby indicate particularly suitable use intermittent renewable sources. aspects require further include optimization process towards lower EPCtotal values, improved separation, reliable ignition plasma.

Language: Английский

Citations

6

Salt Precipitation and Water Flooding Intrinsic to Electrocatalytic CO2 Reduction in Acidic Membrane Electrode Assemblies: Fundamentals and Remedies DOI Creative Commons
Qianqian Bai,

Likun Xiong,

Yongjia Zhang

et al.

EES Catalysis, Journal Year: 2024, Volume and Issue: unknown

Published: Jan. 1, 2024

The fundamentals of salt precipitation and water flooding in membrane electrode assemblies for acidic electrocatalytic CO 2 reduction are discussed potential remedies via engineering electrodes, electrolytes, membranes proposed.

Language: Английский

Citations

6

Heterogeneous catalysis for the environment DOI
Jun Liu,

Rihana Burciaga,

S. Q. Tang

et al.

The Innovation Materials, Journal Year: 2024, Volume and Issue: unknown, P. 100090 - 100090

Published: Jan. 1, 2024

<p>Anthropogenic climate and environmental changes increasingly threaten the sustainability of life on Earth, hindering sustainable development human societies. These detrimental ecological are driven by activities that have elevated atmospheric levels greenhouse gases toxic substances, increased inorganic organic pollutants in water bodies, led to accumulation solid waste soils. Over next two three decades, impacts change, pollution, soil contamination expected intensify, posing increasing risks health global stability. Considering these trends, it is essential implement robust mitigation adaptation strategies. This paper analyzes pollution problems from perspectives atmospheric, water, contamination. It summarizes current research heterogeneous catalysis for treating gaseous, liquid, phases, with an emphasis key challenges applying catalytic conversion technologies cost-effective industrial settings. Finally, strategies mitigating via discussed material flow, energy data flow. aims offer scientific insights enhance future practice remediation.</p>

Language: Английский

Citations

5

Trilayer Polymer Electrolytes Enable Carbon‐Efficient CO2 to Multicarbon Product Conversion in Alkaline Electrolyzers DOI
Jundong Wang, Yuesheng Zhang,

H Y Bai

et al.

Angewandte Chemie International Edition, Journal Year: 2024, Volume and Issue: 63(37)

Published: June 21, 2024

The electrochemical CO

Language: Английский

Citations

4

CO residence time modulates multi-carbon formation rates in a zero-gap Cu based CO2 electrolyzer DOI Creative Commons
Siddhartha Subramanian,

Jesse Kok,

Pratik Gholkar

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: 17(18), P. 6728 - 6738

Published: Jan. 1, 2024

This study shows how flow field designs can be used to modulate CO concentrations and hydrocarbon production rates in a zero gap copper based carbon dioxide electrolyzer.

Language: Английский

Citations

4