Developing Heterogeneous Catalysts for Reverse Water–Gas Shift Reaction in CO2 Valorization DOI Creative Commons

Gunjoo Kim,

Hyunjoo Lee

Korean Journal of Chemical Engineering, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 5, 2024

Abstract Carbon dioxide capture and utilization (CCU) in chemical processes is vital for achieving sustainable economically viable solutions the context of climate change mitigation. This review focuses on reverse water–gas shift (RWGS) reaction as a promising pathway converting CO₂ into carbon monoxide (CO), which can subsequently be used precursor synthesis various hydrocarbon compounds. The discussion centers catalyst design strategies aimed at enhancing low-temperature activity RWGS reaction, emphasizing roles supports active sites. Key approaches include increasing surface area, introducing defect sites, improving redox properties catalysts. Methods controlling adsorption strength gas reactants products to enhance CO selectivity are explored, with particular attention use ligands, promoters, doping, advanced structures such single-atom or core–shell configurations. Considerations regarding durability reducing environments development feasible catalysts also addressed. Well-designed offer significant advantages valorization, conversion hydrocarbons more readily achieved starting from CO.

Language: Английский

Overconfidence in climate overshoot DOI Creative Commons
Carl-Friedrich Schleußner, Gaurav Ganti, Quentin Lejeune

et al.

Nature, Journal Year: 2024, Volume and Issue: 634(8033), P. 366 - 373

Published: Oct. 9, 2024

Global emission reduction efforts continue to be insufficient meet the temperature goal of Paris Agreement

Language: Английский

Citations

23

The green hydrogen ambition and implementation gap DOI Creative Commons
Adrian Odenweller, Falko Ueckerdt

Nature Energy, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 14, 2025

Language: Английский

Citations

19

Feasible deployment of carbon capture and storage and the requirements of climate targets DOI Creative Commons
Tsimafei Kazlou, Aleh Cherp, Jessica Jewell

et al.

Nature Climate Change, Journal Year: 2024, Volume and Issue: 14(10), P. 1047 - 1055

Published: Sept. 25, 2024

Climate change mitigation requires the large-scale deployment of carbon capture and storage (CCS). Recent plans indicate an eight-fold increase in CCS capacity by 2030, yet feasibility expansion is debated. Using historical growth other policy-driven technologies, we show that if double between 2023 2025 their failure rates decrease half, could reach 0.37 GtCO

Language: Английский

Citations

18

Uncertainties around net‐zero climate targets have major impact on greenhouse gas emissions projections DOI Creative Commons
Michel den Elzen, Ioannis Dafnomilis, Leonardo Nascimento

et al.

Annals of the New York Academy of Sciences, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 12, 2025

Abstract Globally, more than 100 countries have adopted net‐zero targets. Most studies agree on how this increases the chance of keeping end‐of‐century global warming below 2°C. However, they typically make assumptions about targets that do not capture uncertainties related to gas coverage, sector sinks, and removals. This study aims analyze impact many uncertainty factors projected greenhouse (GHG) emissions by 2050 for major emitting following their pathways, aggregate GHG emissions. Global emission projections range from 23 40 gigatons CO 2 equivalent (GtCO eq), with a median 31 GtCO eq. Our full corresponds 40–75% 2015 levels, which is much wider 30–45% reported various integrated assessment models. The main contributing divergence are in coverage socioeconomic baseline. Countries small emissions, while beyond unclear such as China, India, Indonesia, large 2050.

Language: Английский

Citations

1

Navigating stakeholder heterogeneity in carbon dioxide removal governance DOI Creative Commons
Yuwan Malakar, Kerryn Brent,

A.A. Bester

et al.

Published: Jan. 15, 2025

Citations

1

Polyimide-based thermal rearranged (TR) membrane for highly efficient natural gas separation: A review DOI

Mingwei Cai,

Jiongcai Chen,

Huaixu Wang

et al.

Separation and Purification Technology, Journal Year: 2024, Volume and Issue: 355, P. 129624 - 129624

Published: Sept. 13, 2024

Language: Английский

Citations

5

Over-reliance on land for carbon dioxide removal in net-zero climate pledges DOI Creative Commons
Kate Dooley, Kirstine Lund Christiansen, Jens Friis Lund

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: Oct. 23, 2024

Abstract Achieving net-zero climate targets requires some level of carbon dioxide removal. Current assessments focus on tonnes CO 2 removed, without specifying what form these removals will take. Here, we show that countries’ pledges require approximately 1 (0.9–1.1) billion ha land for removals. For over 40% this area, the envisage conversion existing uses to forests, while remaining area restores ecosystems and uses. We analyse how demand is distributed geographically time. The results are concerning, both in terms aggregate land, but also rate extent use change. Our findings demonstrate a gap between governments’ expected reliance role can realistically play mitigation. This adds another layer observed shortcomings national indicates need more transparency around mitigation plans.

Language: Английский

Citations

4

Marine Forests Forever—A Necessary Multilateral Program for a Fair Future DOI
Paulo Antunes Horta, Marina Nasri Sissini, Alessandra Fonseca

et al.

Aquatic Conservation Marine and Freshwater Ecosystems, Journal Year: 2025, Volume and Issue: 35(1)

Published: Jan. 1, 2025

Language: Английский

Citations

0

Imputation of missing land carbon sequestration data in the AR6 Scenarios Database DOI Creative Commons
Ruben Prütz, Sabine Fuss, Joeri Rogelj

et al.

Earth system science data, Journal Year: 2025, Volume and Issue: 17(1), P. 221 - 231

Published: Jan. 27, 2025

Abstract. The AR6 Scenarios Database is a vital repository of climate change mitigation pathways used in the latest Intergovernmental Panel on Climate Change (IPCC) assessment cycle. In its current version, many scenarios database lack information about level anthropogenic carbon dioxide (CO2) removal via land sinks, as net-negative CO2 emissions and gross removals are not always separated consistently reported across models. This makes scenario analyses focusing challenging. We test compare performance different regression models to impute missing data sequestration for global several sub-global macro-regions from available net agriculture, forestry, other uses. find that k-nearest neighbors performs best among tested use it provide two publicly imputation datasets (https://doi.org/10.5281/zenodo.13373539, Prütz et al., 2024) sinks incomplete (n=404) regional R10 variants (n=2358) Database. discuss limitations our approach, secondary assessments ensembles, how this approach compares recent reanalyses.

Language: Английский

Citations

0

Increasing Carbon Sequestration, Land-Use Efficiency, and Building Decarbonization with Short Rotation Eucalyptus DOI Open Access

Kate Chilton,

Otávio Camargo Campoe, Neil L. Allan

et al.

Sustainability, Journal Year: 2025, Volume and Issue: 17(3), P. 1281 - 1281

Published: Feb. 5, 2025

Global construction activity remains the least responsive large economic sector to exigencies of global climate change. The focus has centered on operating emissions buildings, while upfront embodied in building materials remain unabated. Softwood timber, a commonly used material, can remove and store atmospheric carbon buildings for decades. However, benefits using softwoods frames are limited due multi-decadal growth harvest cycles forest plantations. objective this study was demonstrate that fast-growing Eucalyptus is superior sequestration feedstock compared slow-growing softwoods. We quantified relative group North American an all-carbon-pools, risk-adjusted model compares net present value flows over 100-year period. Using novel benefit multiple metric, analysis shows short-rotation, high-yield plantations 2.7× 4.6× better at sequestering than softwoods, depending various risk perception scenarios. results indicate decarbonization be enhanced by high-yielding species

Language: Английский

Citations

0