Photocatalytic Self-Fenton System of g-C3N4-Based for Degradation of Emerging Contaminants: A Review of Advances and Prospects DOI Creative Commons

Zhouze Chen,

Yujie Yan, Changyu Lu

et al.

Molecules, Journal Year: 2023, Volume and Issue: 28(15), P. 5916 - 5916

Published: Aug. 6, 2023

The discharge of emerging pollutants in the industrial process poses a severe threat to ecological environment and human health. Photocatalytic self-Fenton technology combines advantages photocatalysis Fenton oxidation through situ generation hydrogen peroxide (H2O2) interaction with iron (Fe) ions generate large number strong reactive oxygen species (ROS) effectively degrade environment. Graphite carbon nitride (g-C3N4) is considered as most potential photocatalytic reduction reaction (ORR) photocatalyst for H2O2 production due its excellent chemical/thermal stability, unique electronic structure, easy manufacturing, moderate band gap (2.70 eV). Hence, this review, we briefly introduce degradation mechanisms. In addition, modification strategy g-C3N4-based system related applications environmental remediation are fully discussed summarized detail. Finally, prospects challenges discussed. We believe that review can promote construction novel efficient systems well further application other research fields.

Language: Английский

Controllable surface carrier type of metal oxide nanocrystals for multifunctional photocatalysis DOI Creative Commons
Han Li, Yingchun Ding, Kaiyi Luo

et al.

iScience, Journal Year: 2025, Volume and Issue: 28(2), P. 111750 - 111750

Published: Jan. 5, 2025

Language: Английский

Citations

7
Degradation of micropollutants in secondary wastewater effluent using nonthermal plasma-based AOPs: The roles of free radicals and molecular oxidants DOI
Changtao Chen, Chuanlong Ma, Yongyuan Yang

et al.

Water Research, Journal Year: 2023, Volume and Issue: 235, P. 119881 - 119881

Published: March 20, 2023

Language: Английский

Citations

41
Preparation of Structure Vacancy Defect Modified Diatomic‐Layered g‐C3N4 Nanosheet with Enhanced Photocatalytic Performance DOI Creative Commons

Tian Liu,

Wei Zhu, Ning Wang

et al.

Advanced Science, Journal Year: 2023, Volume and Issue: 10(24)

Published: June 21, 2023

Structure self-modification of graphitic carbon nitride (g-C

Language: Английский

Citations

40
Integration of Single‐Atom Catalyst with Z‐Scheme Heterojunction for Cascade Charge Transfer Enabling Highly Efficient Piezo‐Photocatalysis DOI Creative Commons
Wenbin Jiang, Hui Zhu, Jing Yang

et al.

Advanced Science, Journal Year: 2023, Volume and Issue: 10(28)

Published: Aug. 6, 2023

Piezo-assisted photocatalysis (namely, piezo-photocatalysis), which utilizes mechanical energy to modulate spatial and distribution of photogenerated charge carriers, presents a promising strategy for molecule activation reactive oxygen species (ROS) generation toward applications such as environmental remediation. However, similarly photocatalysis, piezo-photocatalysis also suffers from inferior separation utilization efficiency. Herein, Z-scheme heterojunction composed single Ag atoms-anchored polymeric carbon nitride (Ag-PCN) SnO2-x is developed efficient carrier transfer/separation both within the catalyst between surface molecules (O2 ). As revealed by dynamics analysis theoretical simulations, synergy atoms initiates cascade electron transfer Ag-PCN then O2 adsorbed on Ag. With ultrasound irradiation, polarization field generated piezoelectric hybrid further accelerates regulates pathway. result, Ag-PCN/SnO2-x efficiently activates into ·O2- , ·OH, H2 under co-excitation visible light ultrasound, are consequently utilized trigger aerobic degradation refractory antibiotic pollutants. This work provides maneuver integrating single-atom catalysts (SACs) with heterojunction.

Language: Английский

Citations

38
Photocatalytic Self-Fenton System of g-C3N4-Based for Degradation of Emerging Contaminants: A Review of Advances and Prospects DOI Creative Commons

Zhouze Chen,

Yujie Yan, Changyu Lu

et al.

Molecules, Journal Year: 2023, Volume and Issue: 28(15), P. 5916 - 5916

Published: Aug. 6, 2023

The discharge of emerging pollutants in the industrial process poses a severe threat to ecological environment and human health. Photocatalytic self-Fenton technology combines advantages photocatalysis Fenton oxidation through situ generation hydrogen peroxide (H2O2) interaction with iron (Fe) ions generate large number strong reactive oxygen species (ROS) effectively degrade environment. Graphite carbon nitride (g-C3N4) is considered as most potential photocatalytic reduction reaction (ORR) photocatalyst for H2O2 production due its excellent chemical/thermal stability, unique electronic structure, easy manufacturing, moderate band gap (2.70 eV). Hence, this review, we briefly introduce degradation mechanisms. In addition, modification strategy g-C3N4-based system related applications environmental remediation are fully discussed summarized detail. Finally, prospects challenges discussed. We believe that review can promote construction novel efficient systems well further application other research fields.

Language: Английский

Citations

37