Applied Physics Letters,
Journal Year:
2024,
Volume and Issue:
124(26)
Published: June 24, 2024
Compact
and
broadband
mid-infrared
(MIR)
sources
are
in
high
demand
because
of
a
wide
range
potential
applications
such
as
molecular
sensing
the
fingerprint
region.
The
generation
coherent
MIR
radiation
at
arbitrary
frequencies
typically
requires
nonlinear
mixing
between
least
two
input
waves,
which
is
often
cumbersome
to
implement.
We
present
an
integrated
and,
therefore,
adjustment-free
solution
combining
few-femtosecond
pulse
compression
germanosilicate
optical
fiber
rectification.
To
this
end,
16-μm-thin
GaSe
crystal
directly
mounted
on
end
facet
highly
assembly
exploiting
focused
ion
beam.
With
pulses
minute
energy
5
nJ
duration
120
fs
telecom
wavelength
1.55
μm,
we
obtain
ultrabroadband
phase-stable
output
transients.
Electro-optic
sampling
free
space
reveals
single-cycle
with
spectral
components
covering
entire
from
10
THz.
APL Photonics,
Journal Year:
2024,
Volume and Issue:
9(3)
Published: March 1, 2024
Detecting
the
electric-field
waveform
of
an
optical
pulse
from
terahertz
to
visible
spectral
domain
provides
a
complete
characterization
average
field
and
holds
great
potential
for
quantum
optics,
time-domain
(including
frequency-comb)
spectroscopy,
high-harmonic
generation,
attosecond
science,
name
few.
The
field-resolved
measurements
can
be
performed
using
electro-optic
sampling,
where
laser
is
characterized
through
interaction
with
another
much
shorter
duration.
measured
train
must
consist
identical
pulses,
including
their
equal
carrier-envelope
phase
(CEP).
Due
limited
coverage
broadband
gain
media,
creating
CEP-stable
trains
in
mid-infrared
typically
requires
nonlinear
frequency
conversion,
such
as
difference
parametric
amplification,
or
rectification.
These
techniques
operate
single-pass
geometry,
often
limiting
efficiency.
In
this
work,
we
demonstrate
analysis
pulses
generated
resonant
system,
oscillator
(OPO).
inherent
feedback,
device
exhibits
relatively
high
conversion
efficiency
at
given
level
input
power.
By
prove
that
subharmonic
OPO
pumped
few-cycle
fiber-laser
generates
output.
full
amplitude
information
renders
dispersion
control
straightforward.
We
also
confirm
existence
exotic
“flipping”
state
directly
time
domain,
electric
consecutive
has
opposite
sign.
IEEE Journal of Quantum Electronics,
Journal Year:
2023,
Volume and Issue:
59(1), P. 1 - 7
Published: Jan. 12, 2023
Cr-doped
ZnS
and
ZnSe
are
excellent
gain
mediums
for
high
power
broadband
ultrashort
pulse
generation
in
the
2
–
$3~\mu
\text{m}$
wavelength
range.
SESAM
modelocked
Cr:ZnS
oscillators
have
advantage
of
reliable,
self-starting
passive
modelocking.
We
present
a
diode-pumped,
oscillator
delivering
pulses
189
fs
at
550
mW
average
output
with
repetition
rate
435
MHz
low
relative
intensity
noise
(RIN)
timing
jitter.
measured
an
integrated
RIN
0.05%
within
frequency
span
[10
Hz,
5
MHz]
dominated
by
1560-nm
pump
diode,
very
jitter
10.9
[2
kHz,
10
MHz].
This
type
laser
source
benefits
not
only
from
but
also
reduced
complexity
cost
due
to
direct
diode
pumping,
which
is
suitable
many
applications
such
as
spectroscopy,
ranging,
conversion.
Optics Letters,
Journal Year:
2023,
Volume and Issue:
48(17), P. 4468 - 4468
Published: July 31, 2023
The
influence
of
the
carrier-envelope
phase
(CEP)
a
pump
pulse
on
multioctave
supercontinuum
(SC)
generation
in
gas-filled
anti-resonant
hollow-core
fiber
(AR
HCF)
by
soliton
self-compression
(SSC)
has
been
explored.
We
have
shown
an
octave-wide
third
harmonic
(THG)
visible-to-near-infrared
range
during
compression
down
to
sub-cycle
duration.
CEP
multi-cycle
provides
control
interference
between
(TH)
and
SC
that
indicates
coherent
synthesis
with
duration
about
0.4
optical
cycles
peak
power
more
than
2
GW
at
output.
Optics Letters,
Journal Year:
2024,
Volume and Issue:
49(4), P. 1049 - 1049
Published: Jan. 23, 2024
Ultrashort
pulses
at
infrared
wavelengths
are
advantageous
when
studying
light–matter
interaction.
For
the
spectral
region
around
2
µm,
multi-stage
parametric
amplification
is
most
common
method
to
reach
higher
pulse
energies.
Yet
it
has
been
a
key
challenge
for
such
systems
deliver
waveform-stable
without
active
stabilization
and
synchronization
systems.
Here,
we
present
different
approach
generation
of
centered
1.8
µm
with
watt-level
average
power
utilizing
only
single
nonlinear
crystal.
Our
laser
system
relies
on
well-established
Yb:YAG
thin-disk
technology
1.03
wavelength
combined
hybrid
two-stage
broadening
scheme.
We
show
high-power
downconversion
process
via
intra-pulse
difference
frequency
generation,
which
leads
excellent
passive
stability
carrier
envelope
phase
below
20
mrad—comparable
modern
oscillators.
It
also
provides
simple
control
over
central
within
broad
range.
The
developed
source
employed
generate
multi-octave
continuum
from
500
nm
2.5
opening
path
toward
sub-cycle
synthesis
extreme
waveform
stability.
Optics Express,
Journal Year:
2024,
Volume and Issue:
32(20), P. 35462 - 35462
Published: Sept. 17, 2024
Soliton
molecules,
or
soliton
bound
states,
are
envisioned
to
make
far-reaching
changes
in
both
fundamental
research
and
applications.
Here,
we
report
on
the
generation
precision
manipulation
of
molecules
based
a
Kerr-lens
mode-locked
single-crystal
Cr:ZnS
laser
at
2.4
µm.
In
classical
regime,
self-starting
near-transform-limited
pulses
with
duration
37
fs,
less
than
5
optical
cycles,
have
been
obtained
repetition
frequency
173
MHz
an
average
output
power
572
mW.
By
fine-tuning
cavity
group-delay
dispersion
profile,
bi-soliton
states
pulse
durations
between
55
fs
98
temporal
separations
348
604
observed
characterized.
These
shortest
separation
reported
so
far
mid-infrared
region,
best
our
knowledge.
With
ability
generated
sub-100-fs
timescale,
tunable
molecule
source
paves
way
for
applications
fields
telecommunications
ultrafast
technologies.
Physical review. A/Physical review, A,
Journal Year:
2023,
Volume and Issue:
107(2)
Published: Feb. 22, 2023
Single-atom
high-order
harmonic
generation
(HHG)
induced
by
an
intense
linearly
polarized
infrared
(IR)
field
and
assisted
a
perturbative
extreme
ultraviolet
(XUV)
short
pulse
with
linear
polarization
is
analyzed
in
perpendicular
geometry.
It
shown
that
for
the
case
of
initial
$p$
state,
two
independent
projections
laser-induced
dipole
are
formed
physical
channels,
which
responsible
IR-induced
HHG
XUV-initiated
HHG.
This
property
utilized
control
generated
radiation.
An
alternative
scheme
studying
proposed.
Optics Express,
Journal Year:
2023,
Volume and Issue:
31(15), P. 24862 - 24862
Published: June 13, 2023
Parametric
downconversion
driven
by
modern,
high-power
sources
of
10-fs-scale
near-infrared
pulses,
in
particular
intrapulse
difference-frequency
generation
(IPDFG),
affords
combinations
properties
desirable
for
molecular
vibrational
spectroscopy
the
mid-infrared
range:
broad
spectral
coverage,
high
brilliance,
and
spatial
temporal
coherence.
Yet,
unifying
these
a
robust
compact
radiation
source
has
remained
key
challenge.
Here,
we
address
this
need
employing
IPDFG
multi-crystal
in-line
geometry,
100-W-level,
10.6-fs
pulses
10.6-MHz-repetition-rate,
nonlinearly
post-compressed
Yb:YAG
thin-disk
oscillator.
Polarization
tailoring
driving
using
bichromatic
waveplate
is
followed
sequence
two
crystals,
LiIO3
LiGaS2,
resulting
simultaneous
coverage
800-cm-1-to-3000-cm-1
range
(at
-30-dB
intensity)
with
130
mW
average
power.
We
demonstrate
that
optical-phase
coherence
maintained
theory
experiment,
latter
ultra-broadband
electro-optic
sampling.
These
results
pave
way
toward
coherent
schemes
like
field-resolved
frequency-comb
spectroscopy,
as
well
nonlinear,
ultrafast
optical-waveform
synthesis
across
entire
infrared
fingerprint
region.
Abstract
Intense
long‐wave
infrared
(LWIR)
femtosecond
pulses
within
the
8−14
µm
atmospheric
window
present
an
array
of
applications,
such
as
in
strong‐field
physics,
ultrafast
nonlinear
spectroscopy,
and
self‐guided
propagation.
However,
realization
LWIR
source
capable
delivering
millijoule‐class
energy,
few‐cycle
duration,
kHz
repetition
rate
concurrently
remains
challenging.
Here,
via
combination
different
parametric
processes
is
reported,
driven
by
a
1
Yb:YAG
thin‐disk
laser.
The
system
comprises
two
parallel
multi‐cycle
optical
chirped‐pulse
amplifiers
(OPCPAs)
operating
at
2.3
3.1
µm,
respectively,
alongside
stage
ZnGeP
2
‐crystal‐based
difference‐frequency
generation
(DFG).
resulting
9
DFG
have
record
energy
0.21
mJ,
3‐cycle
rate,
long‐term
stability.
simultaneous
output
three
synchronized
intense
lasers
short‐wave
(2.3
µm),
mid‐wave
(3.1
(9
µm)
renders
particularly
appealing
for
multicolor
applications.
Optics Letters,
Journal Year:
2022,
Volume and Issue:
47(23), P. 6217 - 6217
Published: Oct. 26, 2022
Diode-pumped
Cr:ZnS
oscillators
have
emerged
as
precursors
for
single-cycle
infrared
pulse
generation
with
excellent
noise
performance.
Here
we
demonstrate
a
amplifier
direct
diode-pumping
to
boost
the
output
of
an
ultrafast
oscillator
minimum
added
intensity
noise.
Seeded
0.66-W
train
at
50-MHz
repetition
rate
and
2.4
µm
center
wavelength,
provides
over
2.2
W
35-fs
pulses.
Due
low-noise
performance
laser
pump
diodes
in
relevant
frequency
range,
achieves
root
mean
square
(RMS)
level
only
0.03%
10
Hz-1
MHz
range
long-term
power
stability
0.13%
RMS
one
hour.
The
diode-pumped
reported
here
is
promising
driving
source
nonlinear
compression
single-
or
sub-cycle
regime,
well
bright,
multi-octave-spanning
mid-infrared
pulses
ultra-sensitive
vibrational
spectroscopy.