Advanced Materials,
Journal Year:
2022,
Volume and Issue:
34(30)
Published: May 25, 2022
Coupling
charge
impurity
scattering
effects
and
charge-carrier
modulation
by
doping
can
offer
intriguing
opportunities
for
atomic-level
control
of
resistive
switching
(RS).
Nonetheless,
such
have
remained
unexplored
memristive
applications
based
on
2D
materials.
Here
a
facile
approach
is
reported
to
transform
an
RS-inactive
rhenium
disulfide
(ReS2
)
into
effective
material
through
interfacial
induced
molybdenum-irradiation
(Mo-i)
doping.
Using
ReS2
as
model
system,
this
study
unveils
unique
RS
mechanism
the
formation/dissolution
metallic
β-ReO2
filament
across
defective
interface
during
set/reset
process.
Through
simple
modulation,
various
thicknesses
are
switchable
modulating
Mo-irradiation
period.
Besides,
Mo-irradiated
(Mo-ReS2
memristor
further
exhibits
bipolar
non-volatile
ratio
nearly
two
orders
magnitude,
programmable
multilevel
resistance
states,
long-term
synaptic
plasticity.
Additionally,
fabricated
device
achieve
high
MNIST
learning
accuracy
91%
under
non-identical
pulse
train.
The
study's
findings
demonstrate
potential
in
materials
via
doping-induced
charged
property.
Advanced Materials,
Journal Year:
2021,
Volume and Issue:
34(25)
Published: Sept. 12, 2021
Memristor
crossbar
with
programmable
conductance
could
overcome
the
energy
consumption
and
speed
limitations
of
neural
networks
when
executing
core
computing
tasks
in
image
processing.
However,
implementation
array
(CBA)
based
on
ultrathin
2D
materials
is
hindered
by
challenges
associated
large-scale
material
synthesis
device
integration.
Here,
a
memristor
CBA
demonstrated
using
wafer-scale
(2-inch)
polycrystalline
hafnium
diselenide
(HfSe2
)
grown
molecular
beam
epitaxy,
metal-assisted
van
der
Waals
transfer
technique.
The
exhibits
small
switching
voltage
(0.6
V),
low
(0.82
pJ),
simultaneously
achieves
emulation
synaptic
weight
plasticity.
Furthermore,
enables
artificial
network
high
recognition
accuracy
93.34%.
Hardware
multiply-and-accumulate
(MAC)
operation
narrow
error
distribution
0.29%
also
demonstrated,
power
efficiency
greater
than
8-trillion
operations
per
second
Watt
achieved.
Based
MAC
results,
hardware
convolution
processing
can
be
performed
kernels
(i.e.,
soft,
horizontal,
vertical
edge
enhancement),
which
constitutes
vital
function
for
hardware.
Nature Communications,
Journal Year:
2022,
Volume and Issue:
13(1)
Published: Dec. 2, 2022
Neuromorphic
computing
memristors
are
attractive
to
construct
low-power-
consumption
electronic
textiles
due
the
intrinsic
interwoven
architecture
and
promising
applications
in
wearable
electronics.
Developing
reconfigurable
fiber-based
is
an
efficient
method
realize
that
capable
of
neuromorphic
function.
However,
previously
reported
artificial
synapse
neuron
need
different
materials
configurations,
making
it
difficult
multiple
functions
a
single
device.
Herein,
textile
memristor
network
Ag/MoS
Advanced Functional Materials,
Journal Year:
2022,
Volume and Issue:
32(25)
Published: April 3, 2022
Abstract
Artificial
optoelectronic
synapses
with
both
electrical
and
light‐induced
synaptic
behaviors
have
recently
been
studied
for
applications
in
neuromorphic
computing
artificial
vision
systems.
However,
the
combination
of
visual
perception
high‐performance
information
processing
capabilities
still
faces
challenges.
In
this
work,
authors
demonstrate
a
memristor
based
on
2D
bismuth
oxyiodide
(BiOI)
nanosheets
that
can
exhibit
bipolar
resistive
switching
(RS)
performance
as
well
plasticity
eminently
suitable
low‐power
synapses.
The
fabricated
exhibits
RS
high
ON/OFF
ratio
up
to
10
5
,
an
ultralow
SET
voltage
≈0.05
V
which
is
one
order
magnitude
lower
than
most
reported
memristors
materials,
low
power
consumption.
Furthermore,
demonstrates
not
only
voltage‐driven
long‐term
potentiation,
depression
plasticity,
paired‐pulse
facilitation,
but
also
short‐
plasticity.
Moreover,
photonic
synapse
be
used
simulate
“learning
experience”
human
brain.
Consequently,
BiOI
shows
ultra‐low
consumption,
provides
new
material
strategy
construct
retina‐like
sensors
functions
perceiving
information.
Chemical Society Reviews,
Journal Year:
2023,
Volume and Issue:
52(20), P. 7071 - 7136
Published: Jan. 1, 2023
This
review
highlights
the
film
preparation
methods
and
application
advances
in
memory
neuromorphic
electronics
of
porous
crystalline
materials,
involving
MOFs,
COFs,
HOFs,
zeolites.
Nature Communications,
Journal Year:
2022,
Volume and Issue:
13(1)
Published: May 19, 2022
Neuromorphic
computing
targets
the
hardware
embodiment
of
neural
network,
and
device
implementation
individual
neuron
synapse
has
attracted
considerable
attention.
The
emulation
synaptic
plasticity
shown
promising
results
after
advent
memristors.
However,
neuronal
intrinsic
plasticity,
which
involves
in
learning
process
through
interactions
with
been
rarely
demonstrated.
Synaptic
occur
concomitantly
process,
suggesting
need
simultaneous
implementation.
Here,
we
report
a
neurosynaptic
that
mimics
single
cell.
Threshold
switch
phase
change
memory
are
merged
threshold
switch-phase
device.
Neuronal
is
demonstrated
based
on
bottom
layer,
resembles
modulation
firing
frequency
biological
neuron.
also
introduced
nonvolatile
switching
top
layer.
Intrinsic
simultaneously
emulated
cell
to
establish
positive
feedback
between
them.
A
loop
retraining
system
implemented
array
for
accelerated
training.
The Journal of Physical Chemistry Letters,
Journal Year:
2022,
Volume and Issue:
13(31), P. 7130 - 7138
Published: July 28, 2022
The
memristor
is
an
excellent
candidate
for
nonvolatile
memory
and
neuromorphic
computing.
Recently,
two-dimensional
(2D)
materials
have
been
developed
use
in
memristors
with
high-performance
resistive
switching
characteristics,
such
as
high
on/off
ratios,
low
SET/RESET
voltages,
good
retention
endurance,
fast
speed,
power
energy
consumption.
Low-power
are
highly
desired
recent
fast-speed
energy-efficient
artificial
networks.
This
Perspective
focuses
on
the
progress
of
low-power
based
2D
materials,
providing
a
condensed
overview
relevant
developments
memristive
performance,
physical
mechanism,
material
modification,
device
assembly
well
potential
applications.
detailed
research
status
has
reviewed
different
from
insulating
hexagonal
boron
nitride,
semiconducting
transition
metal
dichalcogenides,
to
some
newly
materials.
Furthermore,
brief
summary
introducing
perspectives
challenges
included,
aim
insightful
guide
this
field.
Advanced Materials,
Journal Year:
2022,
Volume and Issue:
34(26)
Published: April 8, 2022
In-memory
computing
based
on
memristor
arrays
holds
promise
to
address
the
speed
and
energy
issues
of
classical
von
Neumann
system.
However,
stochasticity
ions'
transport
in
conventional
oxide-based
memristors
imposes
severe
intrinsic
variability,
which
compromises
learning
accuracy
hinders
implementation
neural
network
hardware
accelerators.
Here,
these
challenges
are
addressed
using
a
low-voltage
array
an
ultrathin
PdSeOx
/PdSe2
heterostructure
switching
medium
realized
by
controllable
ultraviolet
(UV)-ozone
treatment.
A
distinctively
different
mechanism
is
revealed
that
can
confine
formation
conductive
filaments,
leading
remarkable
uniform
with
low
set
reset
voltage
variability
values
4.8%
-3.6%,
respectively.
Moreover,
convolutional
image
processing
further
implemented
various
crossbar
kernels
achieve
high
recognition
≈93.4%
due
highly
linear
symmetric
analog
weight
update
as
well
multiple
conductance
states,
manifesting
its
potential
beyond
computing.
Advanced Materials,
Journal Year:
2022,
Volume and Issue:
34(9)
Published: Jan. 6, 2022
Copper
chalcogenides
represent
a
class
of
materials
with
unique
crystal
structures,
high
electrical
conductivity,
and
earth
abundance,
are
recognized
as
promising
candidates
for
next-generation
green
electronics.
However,
their
2D
structures
the
corresponding
electronic
properties
have
rarely
been
touched.
Herein,
series
ultrathin
copper
chalcogenide
nanosheets
thicknesses
down
to
two
unit
cells
successfully
synthesized,
including
layered
Cu2
Te,
well
nonlayered
CuSe
Cu9
S5
,
via
van
der
Waals
epitaxy,
nonvolatile
memristive
behavior
is
investigated
first
time.
Benefiting
from
highly
active
Cu
ions
low
migration
barriers,
memristors
based
on
crystals
exhibit
relatively
small
switching
voltage
(≈0.4
V),
fast
speed,
uniformity,
wide
operating
temperature
range
(from
80
420
K),
stable
retention
good
cyclic
endurance.
These
results
demonstrate
tangible
applications
in
future
low-power,
cryogenic,
harsh
Nature Communications,
Journal Year:
2022,
Volume and Issue:
13(1)
Published: Nov. 17, 2022
Abstract
Neuromorphic
machines
are
intriguing
for
building
energy-efficient
intelligent
systems,
where
spiking
neurons
pivotal
components.
Recently,
memristive
with
promising
bio-plausibility
have
been
developed,
but
limited
reliability,
bulky
capacitors
or
additional
reset
circuits.
Here,
we
propose
an
anti-ferroelectric
field-effect
transistor
neuron
based
on
the
inherent
polarization
and
depolarization
of
Hf
0.2
Zr
0.8
O
2
film
to
meet
these
challenges.
The
intrinsic
accumulated
polarization/spontaneous
films
implements
integration/leaky
behavior
neurons,
avoiding
external
Moreover,
exhibits
low
energy
consumption
(37
fJ/spike),
high
endurance
(>10
12
),
uniformity
stability.
We
further
construct
a
two-layer
fully
ferroelectric
neural
networks
that
combines
synapses,
achieving
96.8%
recognition
accuracy
Modified
National
Institute
Standards
Technology
dataset.
This
work
opens
way
emulate
materials
provides
approach
high-efficient
neuromorphic
hardware.