Flexible biomimetic olfactory neurons based on organic heterojunction DOI

Tianyang Feng,

Jialin Meng, Hang Xu

et al.

Journal of Semiconductors, Journal Year: 2024, Volume and Issue: 45(12), P. 122302 - 122302

Published: Dec. 1, 2024

Abstract Simulating the human olfactory nervous system is one of key issues in field neuromorphic computing. Olfactory neurons interact with gas molecules, transmitting and storing odor information to center brain. In order emulate complex functionalities neurons, this study presents a flexible synapse transistor (OST) based on pentacene/C8-BTBT organic heterojunction. By modulating interface between energy bands semiconductor layers, device demonstrates high sensitivity (ppb level) memory function for NH 3 sensing. Typical synaptic behaviors triggered by pulses have been successfully demonstrated, such as inhibitory postsynaptic currents (IPSC), paired-pulse depression (PPD), long-term potentiation/depression (LTP/LTD), transition from short-term (STD) (LTD). Furthermore, maintains stable functions even under different bending conditions, which can present new insights possibilities systems bio-inspired electronic products.

Language: Английский

Nanomaterials for Flexible Neuromorphics DOI

Guanglong Ding,

Hang Li,

Jiyu Zhao

et al.

Chemical Reviews, Journal Year: 2024, Volume and Issue: 124(22), P. 12738 - 12843

Published: Nov. 5, 2024

The quest to imbue machines with intelligence akin that of humans, through the development adaptable neuromorphic devices and creation artificial neural systems, has long stood as a pivotal goal in both scientific inquiry industrial advancement. Recent advancements flexible electronics primarily rely on nanomaterials polymers owing their inherent uniformity, superior mechanical electrical capabilities, versatile functionalities. However, this field is still its nascent stage, necessitating continuous efforts materials innovation device/system design. Therefore, it imperative conduct an extensive comprehensive analysis summarize current progress. This review highlights applications neuromorphics, involving inorganic (zero-/one-/two-dimensional, heterostructure), carbon-based such carbon nanotubes (CNTs) graphene, polymers. Additionally, comparison summary structural compositions, design strategies, key performance, significant these are provided. Furthermore, challenges future directions pertaining materials/devices/systems associated neuromorphics also addressed. aim shed light rapidly growing attract experts from diverse disciplines (e.g., electronics, science, neurobiology), foster further for accelerated development.

Language: Английский

Citations

18

An organic electrochemical neuron for a neuromorphic perception system DOI Creative Commons
Yao Yao, Robert M. Pankow, Wei Huang

et al.

Proceedings of the National Academy of Sciences, Journal Year: 2025, Volume and Issue: 122(2)

Published: Jan. 8, 2025

Human perception systems are highly refined, relying on an adaptive, plastic, and event-driven network of sensory neurons. Drawing inspiration from Nature, neuromorphic hold tremendous potential for efficient multisensory signal processing in the physical world; however, development artificial neuron with a widely calibratable spiking range reduced footprint remains challenging. Here, we report organic electrochemical (OECN) (<37 mm 2 ) based high-performance vertical OECT (vOECT) complementary circuitry enabled by advanced n-type polymer balanced p-/n-type vOECT performance. The OECN exhibits outstanding neuronal characteristics, capable producing spikes state-of-the art firing frequency 0.130 to 147.1 Hz. Leveraging this capability, develop system that integrates mechanical sensors them synapse tactile perception. successfully encodes stimulations into frequency-dependent spikes, which further converted postsynaptic responses. This bioinspired design demonstrates significant advance cyborg systems, providing perceptual capabilities.

Language: Английский

Citations

3

Artificial intelligence-assisted wearable electronics for human-machine interfaces DOI
Lingji Kong,

Juhuang Song,

Zheng Fang

et al.

Device, Journal Year: 2025, Volume and Issue: unknown, P. 100707 - 100707

Published: Feb. 1, 2025

Language: Английский

Citations

1

Backbone Engineering of Bithiophene Imide Dimer‐Based Polymeric Mixed Ionic‐Electronic Conductors for High‐Performance n‐Type Organic Electrochemical Transistors DOI
Xiage Zhang,

Rongjin Zhu,

Wanli Yang

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 22, 2025

Abstract Polymeric mixed ionic‐electronic conductors (PMIECs) are gaining significant attention due to their potential applications in organic electrochemical transistors (OECTs). However, the performance of n‐type OECTs still lags behind that p‐type counterparts. Here, structure‐performance correlation fused bithiophene imide dimer (BTI2)‐based PMIECs is systematically investigated with backbone evaluation from acceptor‐strong donor (A‐SD) acceptor‐donor (A‐D), acceptor‐weak (A‐WD), acceptor (A‐WA), and finally A‐A structures. Compared other PMIECs, backbone‐based PMIEC PBTI2g‐BTI features most suppressed lowest unoccupied molecular orbital energy level, a highly planar backbone, superior dopability. Consequently, polymer delivers an exceptional unipolar OECT high electron mobility 0.25 cm 2 V⁻¹ s⁻¹ remarkable µC * value 63.79 F cm⁻¹ s⁻¹, both which significantly higher than those types PMIECs. This study demonstrates strategy effective approach developing high‐performance for OECTs.

Language: Английский

Citations

0

A flexible multi-gate organic electrochemical synaptic transistor for image processing DOI
Jingwen Wang, Yunchao Xu,

Chenxing Jin

et al.

Applied Physics Letters, Journal Year: 2025, Volume and Issue: 126(5)

Published: Feb. 3, 2025

In this study, a P3HT-based multi-gate frequency-dependent synaptic transistor is fabricated, which demonstrates significant advantages in mimicking the transmission characteristics of biological activities. The proposed device simulates outputs related to frequency and gate voltage modulation. This can respond differently inputs ranging from 0.75 11.11 Hz, at same input frequency, it exhibits different responses by varying control 0 −0.8 V. innovative design dynamically adjust cutoff enhancing edge feature processing images, thereby significantly improving recognition accuracy information blurry images that be difficult for humans distinguish. Our results provide hardware edge-computing image method, overcoming limitations traditional single-gate transistors typically have fixed parameters. preprocessed improved 80% 100%. Combined with design, excels not only enhancement but also offers robust support future neuromorphic electronics.

Language: Английский

Citations

0

Organic Synaptic Transistors Based on C8-BTBT/PMMA/PbS QDs for UV to NIR Face Recognition Systems DOI

Tianyang Feng,

Hang Xu, Yafen Yang

et al.

Nano Letters, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 20, 2025

Developing optoelectronic synaptic devices with low power consumption, broadband response, and biological compatibility is crucial to simulate the functions of optic nerve. Here, an organic synapse transistor based on C8-BTBT/PMMA/PbS quantum dots (PbS QDs) fabricated, which has good stability, consumption (as as 0.49 fJ per event under 800 nm near-infrared optical pulse), response from ultraviolet wavelengths. Based trap release photogenerated carriers by PbS QDs, a series behaviors are simulated device. Furthermore, we use artificial neural network model realize recognition facial feature image in broad spectral range; rate reached 96.25% (350 ultraviolet), 92.14% (580 visible), 90.03% (800 near-infrared). This work beneficial for advancing development future intelligence vision sensing.

Language: Английский

Citations

0

A Solution‐Based Deposition Method Enabling Pigment Blue Edible Electrochemical Transistors DOI Creative Commons
Alessandro Luzio,

Fabrizio Mario Ferrarese,

Matteo Butti

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 27, 2025

Abstract Copper(II) phthalocyanine (CuPc), also known as Pigment Blue 15, is a widely utilized pigment renowned for its exceptional semiconducting properties when refined to electronic‐grade purity. Recent studies have confirmed safety if ingested at doses required essential active components in edible electronics advanced gastrointestinal tract monitoring. Since in‐body operations impose stringent constraints on operational biases, the development of transistors with high transconductance low voltages ensure adequate amplification gain. This study presents simple and cost‐effective method producing solution‐processed CuPc films characterized by unique porous microstructure that facilitates efficient volumetric ion uptake mixed ionic‐electronic conductivity electrolyte‐gated devices. These exhibit capacitance 30 times greater than compact produced through conventional physical vapor deposition methods. The resulting demonstrate On/Off ratios exceeding 10 3 channel width‐normalized up 50 µS mm −1 0.8 V, establishing their potential critical future Moreover, proposed results limited impact impurities charge transport efficiency, thus affecting purification costs and, crucially, enabling sourcing pigments recycling upcycling.

Language: Английский

Citations

0

Ultra‐Flexible Pixelated Perovskite Photodetectors Enabled by Honeycomb Polymer Grids for High‐Resolution Imaging DOI Creative Commons
Ding Zheng, Zhaoqian Xie, Wei Huang

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: March 17, 2025

Abstract A nature‐inspired fabrication method based on a photolithography‐free flexible polymer grid is reported for high‐resolution pixelation of perovskite photodiode arrays with exceptional mechanical ductility and morphology resembling that natural compound eyes. The resulting pixelated photosensitive layer has ≈1 µm pixel size 2000 Pixels per inch (PPI) resolution when fully assembled as photodetector array, delivering detectivity >10 13 Jones while providing cross‐talk free imaging. Using effectively releases stress the platform, greatly increasing agility otherwise brittle film. This novel methodology device design offer new possibilities applications in robotics, biomedical imaging, virtual augmented reality.

Language: Английский

Citations

0

Organic Photoelectrochemical Multisensory Integration DOI
Yu‐Ting Huang, Zheng Li, Yuan Cheng

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: March 18, 2025

Abstract Neuromorphic perception capable of multisensory integration (MSI) in electrolytes is important but remains challenging. Here, the aqueous implementation artificial MSI reported based on newly emerged organic photoelectrochemical transistor (OPECT) by representative visual (light)‐gustatory (sour) perception. Under co‐modulation light and H + /OH − , synaptic plasticity several typical characteristics are mimicked, including “super‐additive response,” “inverse effectiveness effect” “temporal congruency.” To demonstrate its potential usage, different types associative learning corresponding reflex activities further emulated. The chemical system also utilized to control salivation a closed loop real‐time perception, processing, integration, actuation emulate biological responses toward external stimuli. In contrast previous solid‐state operations, this work offers new strategy for developing neuromorphic environments that analogous those biology.

Language: Английский

Citations

0

Organic electrochemical transistors based on a conjugated diketopyrrolopyrrole-dialkoxybithiazole copolymer DOI Creative Commons

Zilan Chen,

Xiaowei Zhao, Chengdong Wang

et al.

Nanoscale, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

The performance of the donor–acceptor polymer PDPP-TEG-2Tz in organic electrochemical transistors was investigated using various anions.

Language: Английский

Citations

0