CuI Coordination Polymer‐Catalyzed Azide–Alkyne Cycloaddition Click Reaction at Room Temperature DOI
Subham Sahoo, Rajesh Patra, Tanmay Rom

et al.

European Journal of Inorganic Chemistry, Journal Year: 2023, Volume and Issue: 27(2)

Published: Nov. 2, 2023

Abstract Framework based compounds for eco‐friendly catalysis is of utmost industrial interest. Cu I ‐catalyzed “click” reactions are a class highly efficient and widely used chemical in organic synthesis potential applications biotechnology, medicine, polymer, material sciences. The importance click chemistry also acknowledge by 2022 Noble Prize chemistry. One the most well‐known copper‐catalyzed azide‐alkyne cycloaddition (CuAAC), which type Huisgen 1,3‐dipolar reaction. Herein, three stable copper(I)‐coordination polymers (CPs), [Cu(4‐ABPT)Cl], CP‐1 ; [Cu(4‐ABPT)Br], CP‐2 [Cu 2 (4‐ABPT) 0.5 ], CP‐3 (4‐ABPT=3,5‐di(pyridine‐4‐yl)‐4H‐1,2,4‐triazol‐4‐amine) have been chosen CuAAC reaction, due to presence both Lewis acidic (copper ion), basic (pyridyl amine) sites. counter anion plays crucial role their structural motif as well catalytic efficiency. These easily synthesizable scalable catalysts exhibit trend > selective conversion phenylacetylene, benzyl bromide, sodium azide into 1,4‐cycloaddition product within h at ambient temperature solvent free reaction conditions. using catalyst exhibits near quantitative room we demonstrated bulk‐scale CPs under mild

Language: Английский

A review on zirconium-based metal–organic frameworks: synthetic approaches and biomedical applications DOI Creative Commons
Krishna Chattopadhyay, Manas Mandal, Dilip K. Maiti

et al.

Materials Advances, Journal Year: 2023, Volume and Issue: 5(1), P. 51 - 67

Published: Nov. 21, 2023

Zr-MOFs, known for stability, low cytotoxicity and high drug-loading capacity; have been thoroughly investigated biomedical uses. This article reviews the various synthetic methods recent applications of important Zr-based MOFs.

Language: Английский

Citations

19

Advancements in porous framework materials for chemiresistive hydrogen sensing: Exploring MOFs and COFs DOI
Nany Thokala, Marilyn Esclance DMello,

Krishnaveni Valle

et al.

Dalton Transactions, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

Semiconductor metal oxides detect H 2 even at the ppm level but need high temperatures and oxygen. MOFs/COFs higher concentrations, work lower temperatures, perform very well under inert conditions.

Language: Английский

Citations

0

Preparation and Characterization of Muscone Oil-Based Cyclodextrin Metal–Organic Frameworks: Molecular Dynamics Simulations and Stability Evaluation DOI Creative Commons
Z.Y. Qiao, Lihua Chen, Mubarak G. Bello

et al.

Pharmaceutics, Journal Year: 2025, Volume and Issue: 17(4), P. 497 - 497

Published: April 9, 2025

Objective: Muscone (MUS), a primary active component of musk, is known for its significant pharmacological properties. However, clinical application limited due to poor water solubility and moderate stability. This study aims address these limitations by encapsulating MUS within biodegradable γ-cyclodextrin metal–organic frameworks (γ-CD-MOFs) using solvent-free method enable oral delivery improving stability, pending in vivo validation. Methods: was encapsulated into γ-CD-MOFs method, achieving an optimal loading rate 10.6 ± 0.7%. Comprehensive characterization performed scanning electron microscopy (SEM), X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FTIR), thermogravimetric analysis (TGA). Biocompatibility assessed RAW264.7 cells, molecular dynamics simulations were conducted the interactions between γ-CD-MOFs. Results: Characterization techniques confirmed successful encapsulation studies revealed no cytotoxicity, indicating that system safe drug delivery. Molecular showed preferentially occupies large spherical cages γ-CD-MOFs, driven non-covalent interactions. Solubility tests vitro release demonstrated improved after Stability assessments indicated significantly enhanced thermal photostability MUS, with high residual amounts remaining under various storage conditions. Conclusions: demonstrates potential solidify enhance solubility, improve providing foundation future use pharmaceutical applications.

Language: Английский

Citations

0

CoCorrole‐Functionalized PCN‐222 for Carbon Monoxide Selective Adsorption DOI Creative Commons

Margerie Loze,

Stéphane Brandès, Paul Fleurat‐Lessard

et al.

Chemistry - A European Journal, Journal Year: 2024, Volume and Issue: unknown

Published: Aug. 22, 2024

The high risk of CO poisoning justifies the need for indoor air quality control and warning systems based on detection low concentrations (ppm-ppb) CO. Cobalt corrole complexes selectively bind vs. O

Language: Английский

Citations

2

CuI Coordination Polymer‐Catalyzed Azide–Alkyne Cycloaddition Click Reaction at Room Temperature DOI
Subham Sahoo, Rajesh Patra, Tanmay Rom

et al.

European Journal of Inorganic Chemistry, Journal Year: 2023, Volume and Issue: 27(2)

Published: Nov. 2, 2023

Abstract Framework based compounds for eco‐friendly catalysis is of utmost industrial interest. Cu I ‐catalyzed “click” reactions are a class highly efficient and widely used chemical in organic synthesis potential applications biotechnology, medicine, polymer, material sciences. The importance click chemistry also acknowledge by 2022 Noble Prize chemistry. One the most well‐known copper‐catalyzed azide‐alkyne cycloaddition (CuAAC), which type Huisgen 1,3‐dipolar reaction. Herein, three stable copper(I)‐coordination polymers (CPs), [Cu(4‐ABPT)Cl], CP‐1 ; [Cu(4‐ABPT)Br], CP‐2 [Cu 2 (4‐ABPT) 0.5 ], CP‐3 (4‐ABPT=3,5‐di(pyridine‐4‐yl)‐4H‐1,2,4‐triazol‐4‐amine) have been chosen CuAAC reaction, due to presence both Lewis acidic (copper ion), basic (pyridyl amine) sites. counter anion plays crucial role their structural motif as well catalytic efficiency. These easily synthesizable scalable catalysts exhibit trend > selective conversion phenylacetylene, benzyl bromide, sodium azide into 1,4‐cycloaddition product within h at ambient temperature solvent free reaction conditions. using catalyst exhibits near quantitative room we demonstrated bulk‐scale CPs under mild

Language: Английский

Citations

6