Measurement Platform to Probe the Mechanism of Chiral-Induced Spin Selectivity through Direction-Dependent Magnetic Conductive Atomic Force Microscopy DOI Creative Commons

Joseph Albro,

Noah T. Garrett,

Keerthana Govindaraj

et al.

ACS Nano, Journal Year: 2025, Volume and Issue: unknown

Published: April 29, 2025

This work introduces a magnetic conductive atomic force microscopy (mc-AFM) measurement platform for determining spin polarizations, arising from the chiral-induced selectivity (CISS) effect along different directions in helical conducting fibers. By using principle that preference electron transport chiral material changes with momentum of electron, this method quantifies polarization materials, which straddle ferromagnetic electrode, i.e., by taking measurements regions to right and left electrode while it is magnetized in-plane. The working mechanism shown polyaniline (PANI) fibers, they reveal longitudinal, fiber's axis, transverse, perpendicular fiber magnetoresistance differ about factor 2. observations imply PANI fibers not consistent models attribute (or magnetoresistance) solely spinterface or spin-dependent charge injection barriers. In aggregate, new offers simplified approach extending mc-AFM resolving spin-filtered currents oriented samples.

Language: Английский

Tuning the Spin Polarization of Covalently Coupled CoFe2O4–Reduced Graphene Oxide through a Chiral Metal Support for Electrochemical Oxygen Reduction DOI

Anujit Balo,

Medina Yasmin,

Utkarsh Utkarsh

et al.

ACS Applied Energy Materials, Journal Year: 2025, Volume and Issue: unknown

Published: April 11, 2025

Language: Английский

Citations

0

Nanoarchitectonics for Pentagon Defects in Carbon: Properties and Catalytic Role in Oxygen Reduction Reaction DOI Creative Commons
Guoping Chen, Taro Koide, Junji Nakamura

et al.

Small Methods, Journal Year: 2025, Volume and Issue: unknown

Published: April 22, 2025

Abstract The oxygen reduction reaction (ORR) is a crucial process in electrochemical energy technologies, featuring fuel cells and metal‐air batteries the coming carbon‐neutral society. Carbon materials have garnered significant attention as economical, sustainable alternatives to precious metal catalysts. In particular, there been increasing reports recently that pentagons introduced into graphitic carbons promote catalytic activity for ORR. addition, interesting studies are reported on carbon materials’ synthesis, characterization, spin polarization properties with pentagonal defects. This review comprehensively summarizes formation mechanism, spin, (O 2 ) adsorption, ORR of catalysts By connecting dots between theoretical insights experimental results, this elucidates fundamental principles governing pentagon‐related offers perspectives future directions designing efficient based materials.

Language: Английский

Citations

0

Measurement Platform to Probe the Mechanism of Chiral-Induced Spin Selectivity through Direction-Dependent Magnetic Conductive Atomic Force Microscopy DOI Creative Commons

Joseph Albro,

Noah T. Garrett,

Keerthana Govindaraj

et al.

ACS Nano, Journal Year: 2025, Volume and Issue: unknown

Published: April 29, 2025

This work introduces a magnetic conductive atomic force microscopy (mc-AFM) measurement platform for determining spin polarizations, arising from the chiral-induced selectivity (CISS) effect along different directions in helical conducting fibers. By using principle that preference electron transport chiral material changes with momentum of electron, this method quantifies polarization materials, which straddle ferromagnetic electrode, i.e., by taking measurements regions to right and left electrode while it is magnetized in-plane. The working mechanism shown polyaniline (PANI) fibers, they reveal longitudinal, fiber's axis, transverse, perpendicular fiber magnetoresistance differ about factor 2. observations imply PANI fibers not consistent models attribute (or magnetoresistance) solely spinterface or spin-dependent charge injection barriers. In aggregate, new offers simplified approach extending mc-AFM resolving spin-filtered currents oriented samples.

Language: Английский

Citations

0