Oxy-vacancy Mo-acetylacetone catalyzes N-acetylglucosamine to co-produce furan and pyrrole compounds DOI

Changqu Lin,

Lulu Xu,

Yue Zhuang

et al.

Chemical Engineering Science, Journal Year: 2024, Volume and Issue: unknown, P. 121099 - 121099

Published: Dec. 1, 2024

Language: Английский

Photon and phonon powered photothermal catalysis DOI
Chang Xu, Qijun Tang, Wenguang Tu

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: 17(13), P. 4461 - 4480

Published: Jan. 1, 2024

Synergistic coupling of photons and phonons make the photothermal catalytic conversion various important processes possible.

Language: Английский

Citations

26
Sustainable ammonia synthesis: An in-depth review of non-thermal plasma technologies DOI Creative Commons

Vahid Shahed Gharahshiran,

Ying Zheng

Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: 96, P. 1 - 38

Published: April 24, 2024

Language: Английский

Citations

20
Recent Advances in Ammonia Synthesis: From Haber‐Bosch Process to External Field Driven Strategies DOI
Jiayang Li,

Qingchuan Xiong,

Xiaowei Mu

et al.

ChemSusChem, Journal Year: 2024, Volume and Issue: 17(15)

Published: March 12, 2024

Ammonia, a pivotal chemical feedstock and potential hydrogen energy carrier, demands efficient synthesis as key step in its utilization. The traditional Haber-Bosch process, known for high consumption, has spurred researchers to seek ammonia under milder conditions. Advances surface science characterization technologies have deepened our understanding of the microscopic reaction mechanisms synthesis. This article concentrates on gas-solid phase synthesis, initially exploring latest breakthroughs improvements thermal catalytic Building this, it especially focuses emerging external field-driven alternatives, such photocatalysis, photothermal catalysis, low-temperature plasma catalysis strategies. paper concludes by discussing future prospects objectives nitrogen fixation technologies. comprehensive review is intended provide profound insights overcoming inherent thermodynamic kinetic constraints thereby fostering shift towards "green ammonia" production significantly reducing footprint.

Language: Английский

Citations

15
Unlocking Low‐Temperature Ammonia Decomposition via an Iron Metal–Organic Framework‐Derived Catalyst Under Photo‐Thermal Conditions DOI Open Access
Angel Sousa, D. Mateo, Luis Garzón‐Tovar

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 6, 2025

Photo-thermal catalysis, leveraging both thermal and non-thermal solar contributions, emerges as a sustainable approach for fuel chemical synthesis. In this study, an Fe-based catalyst derived from metal-organic framework is presented efficient photo-thermal ammonia (NH3) decomposition. Optimal conditions, under light irradiation without external heating, result in notable 55% NH3 conversion. Mechanistic investigations reveal that the enhanced catalytic activity arises synergistic interplay between light-induced hot carriers elevated temperatures during irradiation. Supported by density functional theory calculations, findings elucidate dual role of catalyst. At lower temperatures, photo-generated electrons Fe3O4 phase serve to raise energies reaction intermediates, preventing formation thermodynamic sink. Conversely, at higher metallic Fe predominant active phase, with contributions prevailing. Overall, work advances understanding cooperative effects heat systems, paving way innovative applications energy

Language: Английский

Citations

1
Bi2MO6 (M=Mo, W) Aurivillius Oxides for Efficient Photocatalytic N2-to-NH3 Conversion: A perspective review DOI
Xin Huang, Razium Ali Soomro, Huidong Shen

et al.

Inorganic Chemistry Frontiers, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

This summary describes and elucidates an enhanced strategy for photocatalytic nitrogen fixation over Bi 2 MO 6 (M = Mo, W)-based catalysts points out the development prospects of fixation.

Language: Английский

Citations

1
Carbon nitride with grafted benzothiadiazole as electron acceptor and active site to promote exciton dissociation for metal-free photocatalytic N2 fixation DOI

Donghui Cui,

Xue Yang,

Yu Liu

et al.

Journal of Colloid and Interface Science, Journal Year: 2025, Volume and Issue: 686, P. 795 - 806

Published: Feb. 3, 2025

Language: Английский

Citations

1
Interface reconstruction of MXene-Ti3C2 doped CeO2 nanorods for remarked photocatalytic ammonia synthesis DOI
Huaiwei Zhang, Liang Bao, Ying Pan

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 675, P. 130 - 138

Published: July 3, 2024

Language: Английский

Citations

6
Strategy of constructing D-A structure and accurate active sites over graphitic carbon nitride nanowires for high efficient photocatalytic nitrogen fixation DOI

Donghui Cui,

Xue Yang,

Yu Liu

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 678, P. 955 - 969

Published: Sept. 7, 2024

Language: Английский

Citations

6
Structural regulation of three-dimensional bismuth vanadate nanochannels for excellent visible light photocatalytic nitrogen fixation DOI
Xiaoyi Wang, Junhua You,

Yanjun Xue

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: 363, P. 124817 - 124817

Published: Nov. 12, 2024

Language: Английский

Citations

5
A recyclable Cu@C2N nano-catalyst applied in the transformation of alkynes: pH switchable access to ketones and 1,3-diynes DOI
Yuanjin Li, Tianyu Yang, Shuhui Wang

et al.

Green Chemistry, Journal Year: 2024, Volume and Issue: 26(5), P. 2540 - 2545

Published: Jan. 1, 2024

We synthesized a reusable heterogeneous Cu@C 2 N catalyst for pH switchable conversion of alkynes to ketones and 1,3-diynes with 92% 95% yield. The has broad substrate scope, the reaction conditions are environmentally-friendly.

Language: Английский

Citations

4