Applied Catalysis A General, Journal Year: 2024, Volume and Issue: unknown, P. 120032 - 120032
Published: Nov. 1, 2024
Language: Английский
Applied Catalysis A General, Journal Year: 2024, Volume and Issue: unknown, P. 120032 - 120032
Published: Nov. 1, 2024
Language: Английский
International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: 299, P. 140230 - 140230
Published: Jan. 22, 2025
Language: Английский
Citations
1Proceedings of the National Academy of Sciences, Journal Year: 2025, Volume and Issue: 122(4)
Published: Jan. 24, 2025
Lignin degradation by biocatalysts is a key strategy to develop plant-based sustainable carbon economy and thus alleviate global climate change. This process involves synergy between ligninases auxiliary enzymes. However, enzymes within secretomes, which are composed of thousands enzymes, remain enigmatic, although several ligninolytic have been well characterized. Moreover, it challenge understand synergistic lignin via diverse array especially in bacterial systems. In this study, the coexpression network periplasmic proteome uncovers potential accessory for B-type dye-decolorizing peroxidases (DypBs) Pseudomonas putida A514. The catalytic DypBs-based multienzyme complex DypBs couple with quinone reductases nitroreductase participate redox cycling. They work superoxide dismutase induce Fenton reaction oxidation. A synthetic enzyme cocktail (SEC), recruiting 15 was consequently designed four functions. It overcomes limitation repolymerization, exhibiting capacity comparable that native secretome. Importantly, we reveal mechanism SEC-A514 cell system, incorporates advantages vitro catalysis vivo microbial catabolism. Chemical analysis shows system significantly reduces molecular weight lignin, substantially extends spectra functional groups, efficiently metabolizes derivatives. As result, 25% utilized, its average reduced 27%. Our study advances knowledge lignin-degrading multienzymes provides viable strategy.
Language: Английский
Citations
1Applied Microbiology and Biotechnology, Journal Year: 2025, Volume and Issue: 109(1)
Published: Jan. 27, 2025
Language: Английский
Citations
0Bioresource Technology, Journal Year: 2025, Volume and Issue: unknown, P. 132402 - 132402
Published: March 1, 2025
Language: Английский
Citations
0Green Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 1, 2025
We developed an efficient conversion technology for the production of 4-vinylphenol through deep eutectic solvent pretreatment and fast pyrolysis.
Language: Английский
Citations
0Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 162375 - 162375
Published: April 1, 2025
Language: Английский
Citations
0Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 162977 - 162977
Published: April 1, 2025
Language: Английский
Citations
0Green Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 1, 2025
Physical, chemical, and biological methods can prepare core-shell structured LMNPs. The cube in the figure symbolizes their diverse biomedical applications, with its height indicating breadth of these applications.
Language: Английский
Citations
0Industrial & Engineering Chemistry Research, Journal Year: 2024, Volume and Issue: 63(46), P. 19916 - 19935
Published: Nov. 7, 2024
Given the global greenhouse effect caused by excessive CO2 emissions and fossil energy exploitation, cleaner sources are crucial for modern developments. Lignin present in biomass is being considered to replace petroleum due its abundance reproducibility. Although depolymerization of lignin produce high-value chemicals has gained attention, it encounters significant challenges. possesses a high molecular weight, structural changes during separation often diminish potential producing value-added chemicals. This study reviews recent research on using three traditional methods, including hydrolysis, pyrolysis, hydrogenolysis. First, hydrolysis presented, where properties mechanisms under various conditions detailed. Subsequently, pyrolysis mechanism, products, methods (catalytic microwave molten salt pyrolysis) discussed detail. In addition, this provides comprehensive summary hydrogenolysis terms both solvent selection catalytic system. Finally, addresses challenges proposes solutions future research.
Language: Английский
Citations
2Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 156286 - 156286
Published: Sept. 1, 2024
Language: Английский
Citations
1