Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 129871 - 129871
Published: Sept. 1, 2024
Language: Английский
Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 129871 - 129871
Published: Sept. 1, 2024
Language: Английский
Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 674, P. 972 - 981
Published: June 28, 2024
Piezo-photocatalysis combines photocatalysis and piezoelectric effects to enhance catalytic efficiency by creating an internal electric field in the photocatalyst, improving carrier separation overall performance. This study presents a high-performance piezo-photocatalyst for efficient dye degradation using synergistic barium titanate (BTO)-MXene composite. The composite was synthesized via facile method, combining unique properties of BTO nanoparticles with high conductivity MXene. structural morphological analysis confirmed successful formation composite, well-dispersed on MXene surface. piezo-photocatalytic activity evaluated typical solution (Rhodamine B: RhB) under ultraviolet irradiation mechanical agitation. results revealed remarkable enhancement (90 % 15 min piezo-photocatalysis) compared individual stimuli (58.2 95.8 90 piezocatalysis), highlighting between enhanced performance attributed charge transfer facilitated composite's structure, leading increased reactive species generation molecule degradation. Furthermore, exhibited excellent stability reusability, showcasing its potential practical applications wastewater treatment. Overall, this work represents promising strategy designing catalysts, addressing pressing need sustainable solutions environmental remediation.
Language: Английский
Citations
9Advanced Functional Materials, Journal Year: 2024, Volume and Issue: 34(48)
Published: July 2, 2024
Abstract Piezocatalysis is capable of harnessing mechanical energy for environmental remediation, which regarded as a green and promising technology to be exploited. Piezoceramics are struggling used highly efficient piezocatalysts due their grain size reaching tens micrometers usually. Herein, feasible straightforward method proposed turn piezoceramic powders into by integrating optimization oxygen vacancy modulation. This strategy validated treating lead‐free Sr 0.5 Ba Nb 2 O 6 (SBN) with high‐energy ball‐milling (hBM). The rate constant k value 46.95 × 10 −3 min −1 rhodamine B (RhB) piezocatalytic degradation SBN‐hBM‐12h almost 18 times higher than that pristine SBN. Besides, the SBN‐hBM‐12 h catalyst performed superior antibacterial properties against Escherichia coli. enhanced efficiency attributed introduced abundant vacancies absorbing activating reactive species. Well‐modulated concentration can effectively accelerate generation separation free carriers. However, excess in SBN render weakened piezoresponse thus suppressing activity. study elucidates critical role piezocatalysis provides insights development piezocatalysts.
Language: Английский
Citations
6Journal of Alloys and Compounds, Journal Year: 2024, Volume and Issue: 1009, P. 177015 - 177015
Published: Oct. 14, 2024
Language: Английский
Citations
5Journal of Materials Chemistry A, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 1, 2025
2D MXenes and silver enhance the piezo sensor sensitivity for sound-induced vibration. These flexible, self-powered sensors enable damage detection in carbon fiber composites structural health monitoring automotive aerospace sectors.
Language: Английский
Citations
0ChemCatChem, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 24, 2025
Abstract Piezoelectric materials offer great promise due to their ability generate electric fields under mechanical stress, producing surface charges that drive otherwise kinetically sluggish redox reactions. The strained surfaces of these provide a unique advantage in controlling product selectivity and enabling reaction pathways are unattainable with conventional methods. This perspective highlights advancements, challenges, the future potential piezoelectric synthetic organic chemistry, focus on designing optimized for piezocatalyzed synthesis. Piezocatalysis is industrially relevant because its operational simplicity, mild, gram scale synthesis reusable catalysts, minimal solvent use, air tolerant conditions. It involves cycles facilitate one electron events without requiring light exposure or electrical bias. Despite significant progress, many fundamental aspects yet be fully understood. One example correlation between piezoelectricity catalytic activity, which not always linear, as demonstrated by comparison tetragonal cubic BaTiO₃. While BaTiO₃ piezoelectric, it shows excellent activity certain reactions such arylation, dicarbonylation, cyclization mechanochemical conditions comparable Considering all aspects, this aims stimulate discussion advance promising field right direction.
Language: Английский
Citations
0Journal of environmental chemical engineering, Journal Year: 2025, Volume and Issue: unknown, P. 116058 - 116058
Published: March 1, 2025
Language: Английский
Citations
0Small, Journal Year: 2025, Volume and Issue: unknown
Published: March 11, 2025
Abstract Amid the global energy crisis and rising emphasis on sustainability, efficient harvesting has become a research priority. Nanogenerators excel in converting abundant mechanical thermal into electricity, offering promising path for sustainable solutions. Among various nanogenerator's materials, Polyvinylidene fluoride (PVDF), with its distinctive molecular structure, exhibits multifunctional electrical properties including dielectric, piezoelectric pyroelectric characteristics. These combined excellent flexibility make PVDF prime candidate material nanogenerators. In nanogenerators, this is capable of efficiently collecting energy. This paper discusses how PVDF's are manifested three types nanogenerators compares performance these addition, strategies to improve output demonstrated, physical chemical modification as well structural optimization such hybrid structures external circuits. It also introduces application natural human harvesting, prospects medical technologies smart home systems. The aim promote use self‐powered sensing, monitoring, thereby providing valuable insights designing more versatile
Language: Английский
Citations
0Journal of Environmental Management, Journal Year: 2025, Volume and Issue: 382, P. 125211 - 125211
Published: April 15, 2025
Language: Английский
Citations
0Inorganic Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: April 29, 2025
Hydrogen production from water using piezo-catalysis is increasingly popular, but it typically requires expensive noble metal cocatalysts to speed up the reactions. In this study, we found that a UV irradiation treatment on piezoelectric material BiOCl enhances its H2 evolution by 6.8 folds, 0.41 2.81 mmol/g/h, even outperforming those loaded with cocatalysts. Our experiments and simulations revealed prompts in situ reduction of lattice Bi3+ BiOCl, creating Bi nanoparticles surface. These serve as cocatalysts, enhancing hydrogen (1) capturing piezo-generated electrons Bi's higher work function; (2) facilitating charge transfer between due their intimate contact; (3) improving kinetics more suitable H* adsorption strength. This UV-enhancement technique can be applied various Bi-based materials (e.g., BiOBr, BiOI, Bi2WO6, etc.) well piezo-catalytic dye degradation reactions, demonstrating versatility potential for broader applications. research provides straightforward cost-effective approach improve performance without need costly
Language: Английский
Citations
0ACS Nano, Journal Year: 2025, Volume and Issue: unknown
Published: May 6, 2025
Mechanically driven catalysis (MDC) has emerged as an effective strategy for environmental remediation, renewable energy conversion, and cancer therapy; this functions by converting mechanical forces to drive catalytic reactions. This review examines four primary mechanisms, namely, piezocatalysis, flexocatalysis, tribocatalysis, sonocatalysis, each involving specific pathways harnessing at the nanoscale. However, significant challenges arise in decoupling effects related individual mechanism order better understand manipulate their synergies. In review, fundamental principles underpinning MDC are systematically interpreted. Beyond mechanistic insights, recent advancements performance enhancement strategies these catalysts highlighted. Potential applications using approaches remediation (pollutant antibiotic degradation microbial disinfection), conversion (hydrogen production greenhouse gas conversion), biomedical treatments (particularly therapy) discussed. Finally, synergies limiting factors explored, addressing overlooked combined of ultrasound activation source, complexities force interactions nanoscale, need targeted application strategies. Additionally, industrial potential processes with consideration scalability practical deployment is evaluated. While remain, provides a roadmap advancing mechanically catalyst design implementation toward real-world applications, offering into its future trajectory transformative impact across numerous fields.
Language: Английский
Citations
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